351 research outputs found
Anisotropic Superparamagnetism of Monodispersive Cobalt-Platinum Nanocrystals
Based on the high-temperature organometallic route (Sun et al. Science 287,
1989 (2000)), we have synthesized powders containing CoPt_3 single crystals
with mean diameters of 3.3(2) nm and 6.0(2) nm and small log-normal widths
sigma=0.15(1). In the entire temperature range from 5 K to 400 K, the
zero-field cooled susceptibility chi(T) displays significant deviations from
ideal superparamagnetism. Approaching the Curie temperature of 450(10) K, the
deviations arise from the (mean-field) type reduction of the ferromagnetic
moments, while below the blocking temperature T_b, chi(T) is suppressed by the
presence of energy barriers, the distributions of which scale with the particle
volumes obtained from transmission electron microscopy (TEM). This indication
for volume anisotropy is supported by scaling analyses of the shape of the
magnetic absorption chi''(T,omega) which reveal distribution functions for the
barriers being also consistent with the volume distributions observed by TEM.
Above 200 K, the magnetization isotherms M(H,T) display Langevin behavior
providing 2.5(1) mu_B per CoPt_3 in agreement with reports on bulk and thin
film CoPt_3. The non-Langevin shape of the magnetization curves at lower
temperatures is for the first time interpreted as anisotropic
superparamagnetism by taking into account an anisotropy energy of the
nanoparticles E_A(T). Using the magnitude and temperature variation of E_A(T),
the mean energy barriers and 'unphysical' small switching times of the
particles obtained from the analyses of chi''(T,omega) are explained. Below T_b
hysteresis loops appear and are quantitatively described by a blocking model,
which also ignores particle interactions, but takes the size distributions from
TEM and the conventional field dependence of E_A into account.Comment: 12 pages with 10 figures and 1 table. Version accepted for
publication in Phys. Rev. B . Two-column layou
Enhancement of the magnetic anisotropy of nanometer-sized Co clusters: influence of the surface and of the inter-particle interactions
We study the magnetic properties of spherical Co clusters with diameters
between 0.8 nm and 5.4 nm (25 to 7500$ atoms) prepared by sequential sputtering
of Co and Al2O3. The particle size distribution has been determined from the
equilibrium susceptibility and magnetization data and it is compared to
previous structural characterizations. The distribution of activation energies
was independently obtained from a scaling plot of the ac susceptibility.
Combining these two distributions we have accurately determined the effective
anisotropy constant Keff. We find that Keff is enhanced with respect to the
bulk value and that it is dominated by a strong anisotropy induced at the
surface of the clusters. Interactions between the magnetic moments of adjacent
layers are shown to increase the effective activation energy barrier for the
reversal of the magnetic moments. Finally, this reversal is shown to proceed
classically down to the lowest temperature investigated (1.8 K).Comment: 13 figures submitted to Phys. Rev.
Is the Sun Embedded in a Typical Interstellar Cloud?
The physical properties and kinematics of the partially ionized interstellar
material near the Sun are typical of warm diffuse clouds in the solar vicinity.
The interstellar magnetic field at the heliosphere and the kinematics of nearby
clouds are naturally explained in terms of the S1 superbubble shell. The
interstellar radiation field at the Sun appears to be harder than the field
ionizing ambient diffuse gas, which may be a consequence of the low opacity of
the tiny cloud surrounding the heliosphere. The spatial context of the Local
Bubble is consistent with our location in the Orion spur.Comment: "From the Outer Heliosphere to the Local Bubble", held at
International Space Sciences Institute, October 200
Predicting therapy response to mycophenolic acid using UGT1A9 genotyping: towards personalized medicine in atopic dermatitis
Atopic dermatitis (AD) is a very common chronic inflammatory skin disease requiring long-term treatment. Mycophenolic acid (MPA) is used off-label in treatment of patients with severe AD failing Cyclosporin A (CsA) treatment, however clinical efficacy is observed in only half of the AD patients. In blood, MPA levels are known to have a large interindividual variability. Low MPA exposure and increased enzyme activity correlates with the presence of UGT1A9 polymorphisms. In this retrospective study, 65 adult AD patients treated with MPA were classified as responder or non-responder to MPA treatment. UGT1A9 polymorphisms were determined using PCR. A significantly higher number of UGT1A9 polymorphisms was found in the group that did not respond to MPA treatment. Of the patients that carried a UGT1A9 polymorphism, 85.7% were non-responsive to MPA treatment. This implies that non-responsiveness in AD patients is more likely to occur in carriers of a UGT1A9 polymorphism. In a binary logistic regression analysis the odds ratio (OR) was 8.65 (95% confidence interval: 0.93–80.17). Our results show that UGT1A9 polymorphisms can be used to identify patients with non-responsiveness to MPA. Patients with UGT1A9 polymorphisms might benefit from higher MPA dosage
Nucleon Spin-Polarisabilities from Polarisation Observables in Low-Energy Deuteron Compton Scattering
We investigate the dependence of polarisation observables in elastic deuteron
Compton scattering below the pion production threshold on the spin-independent
and spin-dependent iso-scalar dipole polarisabilities of the nucleon. The
calculation uses Chiral Effective Field Theory with dynamical Delta(1232)
degrees of freedom in the Small Scale Expansion at next-to-leading order.
Resummation of the NN intermediate rescattering states and including the Delta
induces sizeable effects. The analysis considers cross-sections and the
analysing power of linearly polarised photons on an unpolarised target, and
cross-section differences and asymmetries of linearly and circularly polarised
beams on a vector-polarised deuteron. An intuitive argument helps one to
identify kinematics in which one or several polarisabilities do not contribute.
Some double-polarised observables are only sensitive to linear combinations of
two of the spin-polarisabilities, simplifying a multipole-analysis of the data.
Spin-polarisabilities can be extracted at photon energies \gtrsim 100 MeV,
after measurements at lower energies of \lesssim 70 MeV provide high-accuracy
determinations of the spin-independent ones. An interactive Mathematica 7.0
notebook of our findings is available from [email protected]: 30 pages LaTeX2e, including 22 figures as 66 .eps file embedded with
includegraphicx; three errors in initial submission corrected. This
submission includes ot the erratum to be published in EPJA (2012) and the
corrections in the tex
Short communication: Detection of yeast DNA in omasal digesta of dairy cows consuming dried distillers grains and solubles
Nucleon Polarizabilities from Deuteron Compton Scattering within a Green's-Function Hybrid Approach
We examine elastic Compton scattering from the deuteron for photon energies
ranging from zero to 100 MeV, using state-of-the-art deuteron wave functions
and NN-potentials. Nucleon-nucleon rescattering between emission and absorption
of the two photons is treated by Green's functions in order to ensure gauge
invariance and the correct Thomson limit. With this Green's-function hybrid
approach, we fulfill the low-energy theorem of deuteron Compton scattering and
there is no significant dependence on the deuteron wave function used.
Concerning the nucleon structure, we use Chiral Effective Field Theory with
explicit \Delta(1232) degrees of freedom within the Small Scale Expansion up to
leading-one-loop order. Agreement with available data is good at all energies.
Our 2-parameter fit to all elastic data leads to values for the
static isoscalar dipole polarizabilities which are in excellent agreement with
the isoscalar Baldin sum rule. Taking this value as additional input, we find
\alpha_E^s= (11.3+-0.7(stat)+-0.6(Baldin)) x 10^{-4} fm^3 and \beta_M^s =
(3.2-+0.7(stat)+-0.6(Baldin)) x 10^{-4} fm^3 and conclude by comparison to the
proton numbers that neutron and proton polarizabilities are essentially the
same.Comment: 47 pages LaTeX2e with 20 figures in 59 .eps files, using graphicx.
Minor modifications; extended discussion of theoretical uncertainties of
polarisabilities extraction. Version accepted for publication in EPJ
Early carboniferous brachiopod faunas from the Baoshan block, west Yunnan, southwest China
38 brachiopod species in 27 genera and subgenera are described from the Yudong Formation in the Shidian-Baoshan area, west Yunnan, southwest China. New taxa include two new subgenera: Unispirifer (Septimispirifer) and Brachythyrina (Longathyrina), and seven new species: Eomarginifera yunnanensis, Marginatia cylindrica, Unispirifer (Unispirifer) xiangshanensis, Unispirifer (Septimispirifer) wafangjieensis, Brachythyrina (Brachythyrina) transversa, Brachythyrina (Longathyrina) baoshanensis, and Girtyella wafangjieensis. Based on the described material and constraints from associated coral and conodont faunas, the age of the brachiopod fauna from the Yudon Formation is considered late Tournaisian (Early Carboniferous), with a possibility extending into earlyViseacutean.<br /
Cosmological parameters from SDSS and WMAP
We measure cosmological parameters using the three-dimensional power spectrum
P(k) from over 200,000 galaxies in the Sloan Digital Sky Survey (SDSS) in
combination with WMAP and other data. Our results are consistent with a
``vanilla'' flat adiabatic Lambda-CDM model without tilt (n=1), running tilt,
tensor modes or massive neutrinos. Adding SDSS information more than halves the
WMAP-only error bars on some parameters, tightening 1 sigma constraints on the
Hubble parameter from h~0.74+0.18-0.07 to h~0.70+0.04-0.03, on the matter
density from Omega_m~0.25+/-0.10 to Omega_m~0.30+/-0.04 (1 sigma) and on
neutrino masses from <11 eV to <0.6 eV (95%). SDSS helps even more when
dropping prior assumptions about curvature, neutrinos, tensor modes and the
equation of state. Our results are in substantial agreement with the joint
analysis of WMAP and the 2dF Galaxy Redshift Survey, which is an impressive
consistency check with independent redshift survey data and analysis
techniques. In this paper, we place particular emphasis on clarifying the
physical origin of the constraints, i.e., what we do and do not know when using
different data sets and prior assumptions. For instance, dropping the
assumption that space is perfectly flat, the WMAP-only constraint on the
measured age of the Universe tightens from t0~16.3+2.3-1.8 Gyr to
t0~14.1+1.0-0.9 Gyr by adding SDSS and SN Ia data. Including tensors, running
tilt, neutrino mass and equation of state in the list of free parameters, many
constraints are still quite weak, but future cosmological measurements from
SDSS and other sources should allow these to be substantially tightened.Comment: Minor revisions to match accepted PRD version. SDSS data and ppt
figures available at http://www.hep.upenn.edu/~max/sdsspars.htm
Genetic characterization of a brangus-ibage cattle population: biochemical polymorphisms and reproductive efficiency
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