180 research outputs found
Temperature-induced pair correlations in clusters and nuclei
The pair correlations in mesoscopic systems such as -size superconducting
clusters and nuclei are studied at finite temperature for the canonical
ensemble of fermions in model spaces with a fixed particle number: i) a
degenerate spherical shell (strong coupling limit), ii) an equidistantly spaced
deformed shell (weak coupling limit). It is shown that after the destruction of
the pair correlations at T=0 by a strong magnetic field or rapid rotation,
heating can bring them back. This phenomenon is a consequence of the fixed
number of fermions in the canonical ensemble
High frequency resonant experiments in Fe molecular clusters
Precise resonant experiments on Fe magnetic clusters have been
conducted down to 1.2 K at various tranverse magnetic fields, using a
cylindrical resonator cavity with 40 different frequencies between 37 GHz and
110 GHz. All the observed resonances for both single crystal and oriented
powder, have been fitted by the eigenstates of the hamiltonian . We have identified the
resonances corresponding to the coherent quantum oscillations for different
orientations of spin S = 10.Comment: to appear in Phys.Rev. B (August 2000
Feedback Effect on Landau-Zener-Stueckelberg Transitions in Magnetic Systems
We examine the effect of the dynamics of the internal magnetic field on the
staircase magnetization curves observed in large-spin molecular magnets. We
show that the size of the magnetization steps depends sensitively on the
intermolecular interactions, even if these are very small compared to the
intra-molecular couplings.Comment: 4 pages, 3 Postscript figures; paper reorganized, conclusions
modifie
Quantum Step Heights in Hysteresis Loops of Molecular Magnets
We present an analytical theory on the heights of the quantum steps observed
in the hysteresis loops of molecular magnets. By considering the dipolar
interaction between molecular spins, our theory successfully yields the step
heights measured in experiments, and reveals a scaling law for the dependence
of the heights on the sweeping rates hidden in the experiment data on Fe
and Mn. With this theory, we show how to accurately determine the tunnel
splitting of a single molecular spin from the step heights.Comment: 4 pages, 5 figure
Characterization of the S = 9 excited state in Fe8Br8 by Electron Paramagnetic Resonance
High Frequency electron paramagnetic resonance has been used to observe the
magnetic dipole, M = 1, transitions in the excited
state of the single molecule magnet FeBr. A Boltzmann analysis of the
measured intensities locates it at 24 2 K above the ground
state, while the line positions yield its magnetic parameters D = -0.27 K, E =
0.05 K, and B = -1.3 10 K. D is thus smaller by 8%
and E larger by 7% than for . The anisotropy barrier for is
estimated as 22 K,which is 25% smaller than that for (29 K). These
data also help assign the spin exchange constants(J's) and thus provide a basis
for improved electronic structure calculations of FeBr.Comment: 7 pages, Figs included in text, submitted to PR
Inter- and Intragranular Effects in Superconducting Compacted Platinum Powders
Compacted platinum powders exhibit a sharp onset of diamagnetic screening at
mK in zero magnetic field in all samples investigated. This
sharp onset is interpreted in terms of the intragranular transition into the
superconducting state. At lower temperatures, the magnetic ac susceptibility
strongly depends on the ac field amplitude and reflects the small intergranular
critical current density . This critical current density shows a strong
dependence on the packing fraction f of the granular samples. Surprisingly,
increases significantly with decreasing f ( A/cm for f = 0.67 and A/cm for f
= 0.50). The temperature dependence of shows strong positive curvature
over a wide temperature range for both samples. The phase diagrams of inter-
and intragranular superconductivity for different samples indicate that the
granular structure might play the key role for an understanding of the origin
of superconductivity in the platinum compacts.Comment: 11 pages including 9 figures. To appear in Phys. Rev. B in Nov. 0
Role of dipolar and exchange interactions in the positions and widths of EPR transitions for the single-molecule magnets Fe8 and Mn12
We examine quantitatively the temperature dependence of the linewidths and
line shifts in electron paramagnetic resonance experiments on single crystals
of the single-molecule magnets Fe and Mn, at fixed frequency, with
an applied magnetic field along the easy axis. We include inter-molecular
spin-spin interactions (dipolar and exchange) and distributions in both the
uniaxial anisotropy parameter and the Land\'{e} -factor. The temperature
dependence of the linewidths and the line shifts are mainly caused by the
spin-spin interactions. For Fe and Mn, the temperature dependence of
the calculated line shifts and linewidths agrees well with the trends of the
experimental data. The linewidths for Fe reveal a stronger temperature
dependence than those for Mn, because for Mn a much wider
distribution in overshadows the temperature dependence of the spin-spin
interactions. For Fe, the line-shift analysis suggests two competing
interactions: a weak ferromagnetic exchange coupling between neighboring
molecules and a longer-ranged dipolar interaction. This result could have
implications for ordering in Fe at low temperatures.Comment: published versio
Dislocation-induced spin tunneling in Mn-12 acetate
Comprehensive theory of quantum spin relaxation in Mn-12 acetate crystals is
developed, that takes into account imperfections of the crystal structure and
is based upon the generalization of the Landau-Zener effect for incoherent
tunneling from excited energy levels. It is shown that linear dislocations at
plausible concentrations provide the transverse anisotropy which is the main
source of tunneling in Mn-12. Local rotations of the easy axis due to
dislocations result in a transverse magnetic field generated by the field
applied along the c-axis of the crystal, which explains the presence of odd
tunneling resonances. Long-range deformations due to dislocations produce a
broad distribution of tunnel splittings. The theory predicts that at subkelvin
temperatures the relaxation curves for different tunneling resonances can be
scaled onto a single master curve. The magnetic relaxation in the thermally
activated regime follows the stretched-exponential law with the exponent
depending on the field, temperature, and concentration of defects.Comment: 17 pages, 14 figures, 1 table, submitted to PR
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