8,712 research outputs found
Temperature dependent d-d excitations in manganites probed by resonant inelastic x-ray scattering
We report the observation of temperature dependent electronic excitations in
various manganites utilizing resonant inelastic x-ray scattering (RIXS) at the
Mn K-edge. Excitations were observed between 1.5 and 16 eV with temperature
dependence found as high as 10 eV. The change in spectral weight between 1.5
and 5 eV was found to be related to the magnetic order and independent of the
conductivity. On the basis of LDA+U and Wannier function calculations, this
dependence is associated with intersite d-d excitations. Finally, the
connection between the RIXS cross-section and the loss function is addressed.Comment: 5 pages, 5 figure
Magnetic and thermodynamic properties of Sr_{2}LaFe_{3}O_{9}
Using a Dirac-Heisenberg Hamiltonian with biquadratic exchange interactions,
we study the effect of iron disproportionation on the magnetic ordering, and
describe the first-order magnetic transition occurring in the perovskite
Sr_{2}LaFe_{3}O_{9}. Upon fitting the experimental data, we give an estimate of
the exchange integrals for the antiferromagntic and ferromagnetic interactions,
in agreement with previous works on kindered compounds. Spin-wave theory yields
a magnon spectrum with a gapless antiferromagnetic mode together with two
gapped ferromagnetic ones.Comment: 8 pages of RevTex, 5 figures (available upon request), submitted to
J. Mag. Mag. Ma
X-ray anomalous scattering investigations on the charge order in -NaVO
Anomalous x-ray diffraction studies show that the charge ordering in
-NaVO is of zig-zag type in all vanadium ladders. We
have found that there are two models of the stacking of layers along
\emph{c-}direction, each of them consisting of 2 degenerated patterns, and that
the experimental data is well reproduced if the 2 patterns appears
simultaneously. We believe that the low temperature structure contains stacking
faults separating regions corresponding to the four possible patterns.Comment: Submitted to Phys. Rev. Lett., 4 pages, 4 eps figures inserted in the
tex
Surface effects on the orbital order in the single layered manganite La0.5Sr1.5MnO4
We report the first observation of `orbital truncation rods' -- the
scattering arising from the termination of bulk orbital order at the surface of
a crystal. The x-ray measurements, performed on a cleaved, single-layered
perovskite, La0.5Sr1.5MnO4, reveal that while the crystallographic surface is
atomically smooth, the orbital `surface' is much rougher, with an r.m.s.
deviation from the average `surface' of ~0.7nm. The temperature dependence of
this scattering shows evidence of a surface-induced second order transition.Comment: 13 pages, 4 figure
Electron quantum optics : partitioning electrons one by one
We have realized a quantum optics like Hanbury Brown and Twiss (HBT)
experiment by partitioning, on an electronic beam-splitter, single elementary
electronic excitations produced one by one by an on-demand emitter. We show
that the measurement of the output currents correlations in the HBT geometry
provides a direct counting, at the single charge level, of the elementary
excitations (electron/hole pairs) generated by the emitter at each cycle. We
observe the antibunching of low energy excitations emitted by the source with
thermal excitations of the Fermi sea already present in the input leads of the
splitter, which suppresses their contribution to the partition noise. This
effect is used to probe the energy distribution of the emitted wave-packets.Comment: 5 pages, 4 figure
The Gamma-Ray Blazar Content of the Northern Sky
Using survey data, we have re-evaluated the correlation of flat spectrum
radio sources with EGRET sources in the Northern sky. A likelihood analysis
incorporating the radio and X-ray properties and the Gamma-ray source
localization is used to gauge the reliability of associations and to search for
counterparts of previously unidentified EGRET sources. Above |b|=10deg, where
the classification is complete, we find that 70% of the Northern EGRET sources
have counterparts similar to the bright EGRET blazars. For several of these we
identify known blazar counterparts more likely than the earlier proposed 3EG
association; for ~20 we have new identifications. Spectroscopic confirmation of
these candidates is in progress and we have found flat spectrum radio quasars
and BL Lac counterparts with redshifts as high as 4. We also find strong
evidence for a set of 28 objects with no plausible counterpart like the known
EGRET Blazars. These thus represent either a new extragalactic population or a
population of Galactic objects with a large scale height. The survey has been
extended into the plane, where we find several new blazar candidates; the bulk
of the sources are, however, Galactic. Looking ahead to the GLAST era we
predict that several of the present 3EG sources are composite and that higher
resolution data will break these into multiple Blazar IDs.Comment: 13 pages, 6 figures, submitted to Ap
Charge-Transfer Excitations in the Model Superconductor HgBaCuO
We report a Cu -edge resonant inelastic x-ray scattering (RIXS) study of
charge-transfer excitations in the 2-8 eV range in the structurally simple
compound HgBaCuO at optimal doping ( K).
The spectra exhibit a significant dependence on the incident photon energy
which we carefully utilize to resolve a multiplet of weakly-dispersive ( eV) electron-hole excitations, including a mode at 2 eV. The observation
of this 2 eV excitation suggests the existence of a charge-transfer pseudogap
deep in the superconducting phase. Quite generally, our data demonstrate the
importance of exploring the incident photon energy dependence of the RIXS cross
section.Comment: 5 pages, 3 figure
Magnetic and electronic Co states in layered cobaltate GdBaCo2O5.5-x
We have performed non-resonant x-ray diffraction, resonant soft and hard
x-ray magnetic diffraction, soft x-ray absorption and x-ray magnetic circular
dichroism measurements to clarify the electronic and magnetic states of the
Co3+ ions in GdBaCo2O5.5. Our data are consistent with a 3+ Py Co HS state at
the pyramidal sites and a 3+ Oc Co LS state at the octahedral sites. The
structural distortion, with a doubling of the a axis (2ap x 2ap x 2ap cell),
shows alternating elongations and contractions of the pyramids and indicates
that the metal-insulator transition is associated with orbital order in the t2g
orbitals of the 3+ Py Co HS state. This distortion corresponds to an
alternating ordering of xz and yz orbitals along the a and c axes for the 3+ Py
Co . The orbital ordering and pyramidal distortion lead to deformation of the
octahedra, but the 3+ Oc Co LS state does not allow an orbital order to occur
for the 3+ Oc Co ions. The soft x-ray magnetic diffraction results indicate
that the magnetic moments are aligned in the ab plane but are not parallel to
the crystallographic a or b axes. The orbital order and the doubling of the
magnetic unit cell along the c axis support a non-collinear magnetic structure.
The x-ray magnetic circular dichroism data indicate that there is a large
orbital magnetic contribution to the total ordered Co moment
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