Electronic states of metallic and semiconducting carbon nanotubes with bond and site disorder

Disorder effects on the density of states in carbon nanotubes are analyzed by a tight binding model with Gaussian bond or site disorder. Metallic armchair and semiconducting zigzag nanotubes are investigated. In the strong disorder limit, the conduction and valence band states merge, and a finite density of states appears at the Fermi energy in both of metallic and semiconducting carbon nanotubes. The bond disorder gives rise to a huge density of states at the Fermi energy differently from that of the site disorder case. Consequences for experiments are discussed.Comment: Phys. Rev. B: Brief Reports (to be published). Related preprints can be found at http://www.etl.go.jp/~harigaya/NEW.htm

Universality of electron correlations in conducting carbon nanotubes

Effective low-energy Hamiltonian of interacting electrons in conducting single-wall carbon nanotubes with arbitrary chirality is derived from the microscopic lattice model. The parameters of the Hamiltonian show very weak dependence on the chiral angle, which makes the low energy properties of conducting chiral nanotubes universal. The strongest Mott-like electron instability at half filling is investigated within the self-consistent harmonic approximation. The energy gaps occur in all modes of elementary excitations and estimate at $0.01-0.1$ eV.Comment: 4 pages, 2 figure

Localized and Delocalized Charge Transport in Single-Wall Carbon-Nanotube Mats

We measured the complex dielectric constant in mats of single-wall carbon-nanotubes between 2.7 K and 300 K up to 0.5 THz. The data are well understood in a Drude approach with a negligible temperature dependence of the plasma frequency (omega_p) and scattering time (tau) with an additional contribution of localized charges. The dielectric properties resemble those of the best ''metallic'' polypyrroles and polyanilines. The absence of metallic islands makes the mats a relevant piece in the puzzle of the interpretation of tau and omega_p in these polymers.Comment: 4 pages including 4 figure

Superconductor-ferromagnet junction phase qubit

We propose a scheme for a phase qubit in an SIFIS junction, consisting of bulk superconductors (S), a proximity-induced ferromagnet (F), and insulating barriers (I). The qubit state is constituted by 0 and $\pi$ phase states of the junction, in which the charging energy of the junction leads to the superposition of the two states. The qubit is operated by the gate voltage applied to the ferromagnet, and insensitive to the decoherence sources existing in other superconducting qubits. We discuss a scalable scheme for qubit measurement and tunable two-qubit coupling.Comment: 3 pages, 3 figure

Oscillator Strength of Metallic Carbon Nanotubes

Based on the tight binding method with hopping integral between the nearest-neighbor atoms, an oscillator strength \int_0^{\infty} \d \omega {\rm Re} \sigma (\omega) is discussed for armchair and metallic zigzag carbon nanotubes. The formulae of the oscillator strength are derived for both types of nanotubes and are compared with the result obtained by a linear chain model. In addition, the doping dependence is investigated in the absence of Coulomb interaction. It is shown that the oscillator strength of each carbon nanotube shows qualitatively the same doping dependence, but the fine structure is different due to it's own peculiar band structure. Some relations independent of the radius of the tube are derived, and a useful formula for determining the amount of doping is proposed.Comment: 4 pages, 4 figures, submitted to J. Phys. Soc. Jpn. at June 30, 200

One-Dimensional Energy Dispersion of Single-Walled Carbon Nanotubes by Resonant Electron Scattering

We characterized the energy band dispersion near the Fermi level in single-walled carbon nanotubes using low-temperature scanning tunneling microscopy. Analysis of energy dependent standing wave oscillations, which result from quantum interference of electrons resonantly scattered by defects, yield a linear energy dispersion near EF, and indicate the importance of parity in scattering for armchair single-walled carbon nanotubes. Additionally, these data provide values of the tight-binding overlap integral and Fermi wavevector in good agreement with previous work, but indicate that the electron coherence length is substantially shortened.Comment: 5 pages, 3 figure

O(N) algorithms in tight-binding molecular-dynamics simulations of the electronic structure of carbon nanotubes

The O(N) and parallelization techniques have been successfully applied in tight-binding molecular-dynamics simulations of single-walled carbon nanotubes (SWNTs) of various chiralities. The accuracy of the O(N) description is found to be enhanced by the use of basis functions of neighboring atoms (buffer). The importance of buffer size in evaluating the simulation time, total energy, and force values together with electronic temperature has been shown. Finally, through the local density of state results, the metallic and semiconducting behavior of (10x10) armchair and (17x0) zigzag SWNT s, respectively, has been demonstrated.Comment: 15 pages, 10 figure

New metallic allotropes of planar and tubular carbon

We propose a new family of layered sp2-like carbon crystals, incorporating five-, six-, and seven-membered rings in 2D Bravais lattices. These periodic sheets can be rolled so as to generate nanotubes of different diameter and chirality. We demonstrate that these sheets and tubes are metastable and more favorable than C60, and it is also shown that their mechanical properties are similar to those of graphene. Density of states calculations of all structures revealed an intrinsic metallic behavior, independent of orientation, tube diameter, and chirality