266 research outputs found
Enhancement of the upper critical field in codoped iron-arsenic high-temperature superconductors
We present the first study of codoped iron-arsenide superconductors of the
122 family (Sr/Ba)_(1-x)K_xFe_(2-y)Co_yAs_2 with the purpose to increase the
upper critical field H_c2 compared to single doped (Sr/Ba)Fe_2As_2 materials.
H_c2 was investigated by measuring the magnetoresistance in high pulsed
magnetic fields up to 64 T. We find, that H_c2 extrapolated to T = 0 is indeed
enhanced significantly to ~ 90 T for polycrystalline samples of
Ba_0.55K_0.45Fe_1.95Co_0.05As_2 compared to ~75 T for Ba_0.55K_0.45Fe_2As_2 and
BaFe_1.8Co_0.2As_2 single crystals. Codoping thus is a promising way for the
systematic optimization of iron-arsenic based superconductors for
magnetic-field and high-current applications.Comment: 7 pages, 5 figures, submitted to Journal of Applied Physic
Competition of local-moment ferromagnetism and superconductivity in Co-substituted EuFe2As2
In contrast to SrFe2As2, where only the iron possesses a magnetic moment, in
EuFe2As2 an additional large, local magnetic moment is carried by Eu2+. Like
SrFe2As2, EuFe2As2 exhibits a spin-density wave transition at high
temperatures, but in addition the magnetic moments of the Eu2+ order at around
20 K. The interplay of pressure-induced superconductivity and the Eu2+ order
leads to a behavior which is reminiscent of re-entrant superconductivity as it
was observed, for example, in the ternary Chevrel phases or in the rare-earth
nickel borocarbides. Here, we study the delicate interplay of the ordering of
the Eu2+ moments and superconductivity in EuFe1.9Co0.1As2, where application of
external pressure makes it possible to sensitively tune the ratio of the
magnetic (T_C) and the superconducting (T_{c,onset}) critical temperatures. We
find that superconductivity disappears once T_C > T_{c,onset}.Comment: 4 pages, 4 figures, submitted to the proceedings of SCES201
Superconductivity in SrFe_(2-x)Co_xAs_2: Internal Doping of the Iron Arsenide Layers
In the electron doped compounds SrFe_(2-x)Co_xAs_2 superconductivity with T_c
up to 20 K is observed for 0.2 < x < 0.4. Results of structure determination,
magnetic susceptibility, electrical resistivity, and specific heat are
reported. The observation of bulk superconductivity in all thermodynamic
properties -- despite strong disorder in the Fe-As layer -- favors an itinerant
picture in contrast to the cuprates and renders a p- or d-wave scenario
unlikely. DFT calculations find that the substitution of Fe by Co (x > 0.3)
leads to the suppression of the magnetic ordering present in SrFe_2As_2 due to
a rigid down-shift of the Fe-3d_(x^2-y^2) related band edge in the density of
states.Comment: 5 pages, 3 figure
High spin polarization in the ferromagnetic filled skutterudites KFe4Sb12 and NaFe4Sb12
The spin polarization of ferromagnetic alkali-metal iron antimonides KFe4Sb12
and NaFe4Sb12 is studied by point-contact Andreev reflection using
superconducting Nb and Pb tips. From these measurements an intrinsic transport
spin polarization Pt of 67% and 60% for the K and Na compound, respectively, is
inferred which establishes these materials as a new class of highly spin
polarized ferromagnets. The results are in accord with band structure
calculations within the local spin density approximation (LSDA) that predict
nearly 100% spin polarization in the density of states. We discuss the impact
of calculated Fermi velocities and spin fluctuations on Pt.Comment: Pdf file with fi
Field dependence of the Eu2+ spin relaxation in EuFe(2-x)CoxAs2
The layered compound EuFe2As2 is an interesting model system to investigate
the effects of well defined local Eu2+ 4f states on the itinerant electronic
and magnetic properties of the FeAs layers. To address this subject, we
investigated the series EuFe2-xCoxAs2 (0.1 <= x <=0.75) by electron spin
resonance (ESR) of Eu2+ to probe the spin dynamics of the itinerant subsystem.
We relate the results to dc-susceptibility measurements and band structure
calculations. As a consequence of the weak coupling between the local and
itinerant subsystems we found that the spin relaxation is well understood in
terms of the exchange coupling among the local Eu2+ spins. A pronounced field
dependence of the Eu2+ spin relaxation demonstrates the direct influence of
magnetic fluctuations at the Fe2-xCoxAs2 layers.Comment: 13 pages, 5 figure
Superconductivity in SrFe2As2 with Pt Doping
We have synthesized polycrystalline samples of Pt-substituted SrFe2As2 and
measured the temperature dependence of magnetization and electrical
resistivity. We have observed the superconducting transition at Tc = 17 K with
the maximum shielding volume fraction at x = 0.125 in Sr(Fe1-xPtx)2As2. It is
found that the maximum Tc depends on the substituted element, so it is
important to substitute various elements to explore new iron-based
superconductors with higher Tc.Comment: 2 pages, 1 figure, to appear in J. Phys. Soc. Jpn. Vol. 79 No. 9
(2010
On Electron Transport in ZrB12, ZrB2 and MgB2
We report on measurements of the temperature dependence of resistivity,
, for single crystal samples of ZrB, ZrB and
polycrystalline samples of MgB. It is shown that cluster compound
ZrB behaves like a simple metal in the normal state, with a typical
Bloch -- Gr\"uneisen dependence. However, the resistive Debye
temperature, , is three times smaller than obtained from
specific heat data. We observe the term in of these borides,
which could be interpreted as an indication of strong electron-electron
interaction. Although the dependence of ZrB reveals a sharp
superconductive transition at , no superconductivity was observed
for single crystal samples of ZrB down to .Comment: 5 pages, 4 figure
Distinct transport behaviors of LaFe1-yCoyAsO1-xFx (x=0.11) between the superconducting and nonsuperconducting metallic y regions divided by y ~ 0.05
Electrical resistivities, Hall coefficients and thermoelectric powers have
been measured for polycrystalline samples of LaFe1-yCoyAsO1-xFx (x=0.11) with
various values of y. The results show that there exists clear distinction of
these transport behaviors between the superconducting and nonsuperconducting
metallic regions of y divided by the boundary value yc~0.05. We have found that
the behaviors in both regions are very similar to those of high-Tc Cu oxides in
the corresponding phases. If they reflect, as in the case of Cu oxides, effects
of strong magnetic fluctuations, the energy scale of the fluctuations is
considered to be smaller than that of the high Cu oxides by a factor of ~1/2.
Arguments on the electronic nature and superconducting symmetry are presented
on the basis of the observed small rate of the Tc suppression rate by the Co
doping.Comment: 8 pages, 4 figures, submitted to J. Phys. Soc. Jp
Effect of Impurities with Internal Structure on Multiband Superconductors - Possible Enhancement of Transition Temperature -
We study inelastic (dynamical) impurity scattering effects in two-band
superconductors with the same ( wave) or different ( wave) sign
order parameters. We focus on the enhancement of the superconducting transition
temperature by magnetic interband scattering with the interchange
of crystal-field singlet ground and multiplet excited states. Either the
-wave or -wave state is favored by the impurity-mediated
pairing, which depends on the magnetic and nonmagnetic scattering strengths
derived from the hybridization of the impurity states with the conduction
bands. The details are examined for the singlet-triplet configuration that is
suggestive of Pr impurities in the skutterudite superconductor
LaOsSb.Comment: 14 pages, 5 figures, to appear in J. Phys. Soc. Jpn. Vol. 79, No. 9
(2010
Muon-spin rotation and magnetization studies of chemical and hydrostatic pressure effects in EuFe_{2}(As_{1-x}P_{x})_{2}
The magnetic phase diagram of EuFe(AsP) was
investigated by means of magnetization and muon-spin rotation studies as a
function of chemical (isovalent substitution of As by P) and hydrostatic
pressure. The magnetic phase diagrams of the magnetic ordering of the Eu and Fe
spins with respect to P content and hydrostatic pressure are determined and
discussed. The present investigations reveal that the magnetic coupling between
the Eu and the Fe sublattices strongly depends on chemical and hydrostatic
pressure. It is found that chemical and hydrostatic pressure have a similar
effect on the Eu and Fe magnetic order.Comment: 11 pages, 10 figure
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