201 research outputs found
Electrical control of the exciton-biexciton splitting in a single self-assembled InGaAs quantum dots
We report on single InGaAs quantum dots embedded in a lateral electric field
device. By applying a voltage we tune the neutral exciton transition into
resonance with the biexciton using the quantum confined Stark effect. The
results are compared to theoretical calculations of the relative energies of
exciton and biexciton. Cascaded decay from the manifold of single
exciton-biexciton states has been predicted to be a new concept to generate
entangled photon pairs on demand without the need to suppress the fine
structures splitting of the neutral exciton
Ion beam synthesis of nanothermochromic diffraction gratings with giant switching contrast at telecom wavelengths
Nanothermochromic diffraction gratings based on the metal-insulator
transition of are fabricated by site-selective ion beam
implantation in a matrix. Gratings were defined either (i)
directly by spatially selective ion beam synthesis or (ii) by site-selective
deactivation of the phase transition by ion beam induced defects. The strongest
increase of the diffracted light intensities was observed at a wavelength of
1550\,nm exceeding a factor of 20 for the selectively deactivated gratings. The
observed pronounced thermal hysteresis extending down close to room temperature
makes this system ideally suited for optical memory applications.Comment: 4 pages, 3 figures, 1 table - corrected Figure
Vertical quantum wire realized with double cleaved-edge overgrowth
A quantum wire is fabricated on (001)-GaAs at the intersection of two
overgrown cleaves. The wire is contacted at each end to n+ GaAs layers via
two-dimensional (2D) leads. A sidegate controls the density of the wire
revealing conductance quantization. The step height is strongly reduced from
2e^2/h due to the 2D-lead series resistance. We characterize the 2D density and
mobility for both cleave facets with four-point measurements. The density on
the first facet is modulated by the substrate potential, depleting a 2um wide
strip that defines the wire length. Micro-photoluminescence shows an extra peak
consistent with 1D electron states at the corner.Comment: 4 pages, 4 figure
Optically Probing Spin and Charge Interactions in an Tunable Artificial Molecule
We optically probe and electrically control a single artificial molecule
containing a well defined number of electrons. Charge and spin dependent
inter-dot quantum couplings are probed optically by adding a single
electron-hole pair and detecting the emission from negatively charged exciton
states. Coulomb and Pauli blockade effects are directly observed and
hybridization and electrostatic charging energies are independently measured.
The inter-dot quantum coupling is confirmed to be mediated predominantly by
electron tunneling. Our results are in excellent accord with calculations that
provide a complete picture of negative excitons and few electron states in
quantum dot molecules.Comment: shortened version: 6 pages, 3 figures, 1 table, to appear in Phys.
Rev. Let
Direct observation of acoustic phonon mediated relaxation between coupled exciton states in a single quantum dot molecule
We probe acoustic phonon mediated relaxation between tunnel coupled exciton
states in an individual quantum dot molecule in which the inter-dot quantum
coupling and energy separation between exciton states is continuously tuned
using static electric field. Time resolved and temperature dependent optical
spectroscopy are used to probe inter-level relaxation around the point of
maximum coupling. The radiative lifetimes of the coupled excitonic states can
be tuned from ~2 ns to ~10 ns as the spatially direct and indirect character of
the wavefunction is varied by detuning from resonance. Acoustic phonon mediated
inter-level relaxation is shown to proceed over timescales comparable to the
direct exciton radiative lifetime, indicative of a relaxation bottleneck for
level spacings in the range $\Delta E\$ ~3-6 meV.Comment: 6 pages, 4 figures, submitted for publicatio
Enhanced sequential carrier capture into individual quantum dots and quantum posts controlled by surface acoustic waves
Individual self-assembled Quantum Dots and Quantum Posts are studied under
the influence of a surface acoustic wave. In optical experiments we observe an
acoustically induced switching of the occupancy of the nanostructures along
with an overall increase of the emission intensity. For Quantum Posts,
switching occurs continuously from predominantely charged excitons (dissimilar
number of electrons and holes) to neutral excitons (same number of electrons
and holes) and is independent on whether the surface acoustic wave amplitude is
increased or decreased. For quantum dots, switching is non-monotonic and shows
a pronounced hysteresis on the amplitude sweep direction. Moreover, emission of
positively charged and neutral excitons is observed at high surface acoustic
wave amplitudes. These findings are explained by carrier trapping and
localization in the thin and disordered two-dimensional wetting layer on top of
which Quantum Dots nucleate. This limitation can be overcome for Quantum Posts
where acoustically induced charge transport is highly efficient in a wide
lateral Matrix-Quantum Well.Comment: 11 pages, 5 figure
Direct Observation of Controlled Coupling in an Individual Quantum Dot Molecule
We report the direct observation of quantum coupling in individual quantum
dot molecules and its manipulation using static electric fields. A pronounced
anti-crossing of different excitonic transitions is observed as the electric
field is tuned. Comparison of our experimental results with theory shows that
the observed anti-crossing occurs between excitons with predominant spatially
\emph{direct} and \emph{indirect} character. The electron component of the
exciton wavefunction is shown to have molecular character at the anti-crossing
and the quantum coupling strength is deduced optically. In addition, we
determine the dependence of the coupling strength on the inter-dot separation
and identify a field driven transition of the nature of the molecular ground
state.Comment: 11 pages, 4 figures submitted to Physical Review Letter
Cascaded exciton emission of an individual strain-induced quantum dot
Single strain-induced quantum dots are isolated for optical experiments by
selective removal of the inducing InP islands from the sample surface.
Unpolarized emission of single, bi- and triexciton transitions are identified
by power-dependent photoluminescence spectroscopy. Employing time-resolved
experiments performed at different excitation powers we find a pronounced shift
of the rise and decay times of these different transitions as expected from
cascaded emission. Good agreement is found for a rate equation model for a
three step cascade
Site-selective ion beam synthesis and optical properties of individual CdSe nanocrystal quantum dots in a SiO2 matrix
Cadmium selenide nanocrystal quantum dots (NC-QDs) are site-selectively
synthesized by sequential ion beam implantation of selenium and cadmium ions in
a SiO2 matrix through sub-micron apertures followed by a rapid thermal
annealing step. The size, areal density and optical emission energy of the
NC-QDs are controlled by the ion fluence during implantation and the diameter
of implantation aperture. For low fluences and small apertures the emission of
these optically active emitters is blue-shifted compared to that of the bulk
material by due to quantum confinement. The emission exhibits
spectral diffusion and blinking on a second timescales as established also for
solution synthesized NC-QDs
Growth and optical properties of self-assembled InGaAs Quantum Posts
We demonstrate a method to grow height controlled, dislocation-free InGaAs
quantum posts (QPs) on GaAs by molecular beam epitaxy (MBE) which is confirmed
by structural investigations. The optical properties are compared to realistic
8-band k.p calculations of the electronic structure which fully account for
strain and the structural properties of the QP. Using QPs embedded in n-i-p
junctions we find wide range tunability of the interband spectrum and giant
static dipole moments.Comment: Proccedings paper for MSS-13, 7 pages, 4 figure
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