Adhesion in soft contacts is minimum beyond a critical shear displacement

The most direct measurement of adhesion is the pull-off force, i.e. the tensile force necessary to separate two solids in contact. For a given interface, it depends on various experimental parameters, including separation speed, contact age and maximum loading force. Here, using smooth contacts between elastomer spheres and rigid plates, we show that the pull-off force also varies if the contact is sheared prior to separation. For shear displacements below a critical valueabout 10% of that necessary to yield gross sliding, the pull-off force steadily decreases as shear increases. For larger shear, the pull-off force remains constant, at a residual value 10%--15% of its initial value. Combining force measurements and in situ imaging, we show how the unloading path leading to contact separation is modified by the initial shear. In particular, we find that the residual pull-off force prevails if the contact reaches full sliding during unloading. Based on those observations, a first modeling attempt of the critical shear displacement is proposed,involving a competition between jump instability and transition to sliding. Overall, those results offer new insights into the interplay between adhesion and friction, provide new constraints on adhesion measurements and challenge existing adhesive models. They will be useful wherever soft contacts undergo both normal and shear stresses, including tire grip, soft robotics, haptics and animal locomotion

Understanding fast macroscale fracture from microcrack post mortem patterns

Dynamic crack propagation drives catastrophic solid failures. In many amorphous brittle materials, sufficiently fast crack growth involves small-scale, high-frequency microcracking damage localized near the crack tip. The ultra-fast dynamics of microcrack nucleation, growth and coalescence is inaccessible experimentally and fast crack propagation was therefore studied only as a macroscale average. Here, we overcome this limitation in polymethylmethacrylate, the archetype of brittle amorphous materials: We reconstruct the complete spatio-temporal microcracking dynamics, with micrometer / nanosecond resolution, through post mortem analysis of the fracture surfaces. We find that all individual microcracks propagate at the same low, load-independent, velocity. Collectively, the main effect of microcracks is not to slow down fracture by increasing the energy required for crack propagation, as commonly believed, but on the contrary to boost the macroscale velocity through an acceleration factor selected on geometric grounds. Our results emphasize the key role of damage-related internal variables in the selection of macroscale fracture dynamics.Comment: 9 pages, 5 figures + supporting information (15 pages

Anomalously slow spin dynamics and short-range correlations in the quantum spin ice systems Yb2Ti2O7 and Yb2Sn2O7

We report a positive muon spin relaxation and rotation (\muSR) study of the quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field response. In agreement with earlier reports, data recorded in small longitudinal fields evidence anomalously slow spin dynamics in the microsecond range below the temperature T_c at which the specific heat displays an intense peak, namely T_c = 0.24 K and 0.15 K, respectively, for the two systems. We found that slow dynamics extends above T_c up to at least 0.7 K for both compounds. The conventional dynamical Gaussian Kubo-Toyabe model describes the \muSR spectra recorded above T_c. At lower temperatures a published analytical extension of the Gaussian Kubo-Toyabe model provides a good description, consistent with the existence of short-range magnetic correlations. While the physical response of the two systems is qualitatively the same, Yb2Ti2O7 exhibits a much larger local magnetic susceptibility than Yb2Sn2O7 below T_c. Considering previously reported ac susceptibility, neutron scattering and \muSR results, we suggest the existence of anomalously slow spin dynamics to be a common physical property of pyrochlore magnetic materials. The possibility of molecular spin substructures to be associated to the slow dynamics and therefore the short-range correlations is mentioned. The slow spin dynamics observed under field does not exclude the presence of much faster dynamics detected in extremely low or zero field.Comment: 11 pages, 10 figure

2D Kagome Ordering in the 3D Frustrated Spinel Li2Mn2O4

muSR experiments on the geometrically frustrated spinel oxide, Li2Mn2O4, show the development of spin correlations over a range of length scales with decreasing temperature. Increased relaxation below 150 K is consistent with the onset of spin correlations. Below 50 K, spin order on a length scale, which is long range for the muSR probe, appears abruptly in temperature, consistent with prior neutron diffraction results. The oscillations in the zero field asymmetry are analyzed using a three frequency model. By locating the muon site this is shown to be consistent with the unexpected 2D q = root 3 x root 3 structure on the Kagome planes proposed originally from neutron data. Longitudinal field data demonstrate that some spin dynamics persist even at 2 K. Thus, a very complex magnetic ground state, featuring the co-existence of long length scale 2D ordering and significant spin dynamics, is proposed. This is unusual considering the 3D topology of the Mn3+ spins in this material.Comment: 9 pages, 9 figures, to be submitted to J. Phys. Cond. Mat

Comparison of different methods for analyzing μ\muSR line shapes in the vortex state of type-II superconductors

A detailed analysis of muon-spin rotation ($\mu$SR) spectra in the vortex state of type-II superconductors using different theoretical models is presented. Analytical approximations of the London and Ginzburg-Landau (GL) models, as well as an exact solution of the GL model were used. The limits of the validity of these models and the reliability to extract parameters such as the magnetic penetration depth $\lambda$ and the coherence length $\xi$ from the experimental $\mu$SR spectra were investigated. The analysis of the simulated $\mu$SR spectra showed that at high magnetic fields there is a strong correlation between obtained $\lambda$ and $\xi$ for any value of the Ginzburg-Landau parameter $\kappa = \lambda/\xi$. The smaller the applied magnetic field is, the smaller is the possibility to find the correct value of $\xi$. A simultaneous determination of $\lambda$ and $\xi$ without any restrictions is very problematic, independent of the model used to describe the vortex state. It was found that for extreme type-II superconductors and low magnetic fields, the fitted value of $\lambda$ is practically independent of $\xi$. The second-moment method frequently used to analyze $\mu$SR spectra by means of a multi-component Gaussian fit, generally yields reliable values of $\lambda$ in the whole range of applied fields $H_{c1} \ll H \lesssim H_{c2}$ ($H_{c1}$ and $H_{c2}$ are the first and second critical fields, respectively). These results are also relevant for the interpretation of small-angle neutron scattering (SANS) experiments of the vortex state in type-II superconductors.Comment: 17 pages, 19 figure

Comparação entre essências florestais nativas e exóticas em Quedas do Iguacu, PR - resultados preliminares.

bitstream/item/215524/1/circ-tec15.pd

Muon spin rotation and relaxation in magnetic materials

A review of the muon spin rotation and relaxation ($\mu$SR) studies on magnetic materials published from July 1993 is presented. It covers the investigation of magnetic phase diagrams, of spin dynamics and the analysis of the magnetic properties of superconductors. We have chosen to focus on selected experimental works in these different topics. In addition, a list of published works is provided.Comment: Review article, 59 pages, LaTeX with IoP macro

Evidence for a two component magnetic response in UPt3

The magnetic response of the heavy fermion superconductor UPt_3 has been investigated on a microscopic scale by muon Knight shift studies. Two distinct and isotropic Knight shifts have been found for the field in the basal plane. While the volume fractions associated with the two Knight shifts are approximately equal at low and high temperatures, they show a dramatic and opposite temperature dependence around T_N. Our results are independent on the precise muon localization site. We conclude that UPt_3 is characterized by a two component magnetic response.Comment: 5 pages, 4 figure