728 research outputs found

    Probing spin dynamics and quantum relaxation in LiY0.998Ho0.002F4 via 19F NMR

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    We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is found to depend on the coupling with the diluted rare-earth (RE) moments. Depending on the temperature range, a fast spin diffusion regime or a diffusion limited regime is encountered. In both cases we find it possible to use the 19F nucleus as a probe of the rare-earth spin dynamics. The results for 1/T1 show a behavior similar to that observed in molecular nanomagnets, a result which we attribute to the discreteness of the energy levels in both cases. At intermediate temperatures the lifetime broadening of the crystal field split RE magnetic levels follows a T3 power law. At low temperature the field dependence of 1/T1 shows peaks in correspondence to the critical magnetic fields for energy level crossings (LC). The results can be explained by inelastic scattering between the fluorine nuclear spins and the RE magnetic levels. A key result of this study is that the broadening of the levels at LC is found to be become extremely small at low temperatures, about 1.7 mT, a value which is comparable to the weak dipolar fields at the RE lattice positions. Thus, unlike the molecular magnets, decoherence effects are strongly suppressed, and it may be possible to measure directly the level repulsions at avoided level crossings.Comment: 21 pages, 5 figure

    19F nuclear spin relaxation and spin diffusion effects in the single ion magnet LiYF4:Ho3+

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    Temperature and magnetic field dependences of the 19F nuclear spin-lattice relaxation in a single crystal of LiYF4 doped with holmium are described by an approach based on a detailed consideration of the magnetic dipole-dipole interactions between nuclei and impurity paramagnetic ions and nuclear spin diffusion processes. The observed non-exponential long time recovery of the nuclear magnetization after saturation at intermediate temperatures is in agreement with predictions of the spin-diffusion theory in a case of the diffusion limited relaxation. At avoided level crossings in the spectrum of electron-nuclear states of the Ho3+ ion, rates of nuclear spin-lattice relaxation increase due to quasi-resonant energy exchange between nuclei and paramagnetic ions, in contrast to the predominant role played by electronic cross-relaxation processes in the low-frequency ac-susceptibility.Comment: 27 pages total, 5 figures, accepted for publication, Eur. Phys. J.

    Spin dynamics in hole-doped two-dimensional S=1/2 Heisenberg antiferromagnets: ^{63}Cu NQR relaxation in La_{2-x}Sr_xCuO_4 for x0.04x\leq 0.04

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    The effects on the correlated Cu^{2+} S = 1/2 spin dynamics in the paramagnetic phase of La_{2-x}Sr_xCuO_4 (for x0.04x \lesssim 0.04) due to the injection of holes are studied by means of ^{63}Cu NQR spin-lattice relaxation time T_1 measurements. The results are discussed in the framework of the connection between T_1 and the in-plane magnetic correlation length ξ2D(x,T)\xi_{2D}(x,T). It is found that at high temperatures the system remains in the renormalized classical regime, with a spin stiffness constant ρs(x)\rho_s(x) reduced by small doping to an extent larger than the one due to Zn doping. For x0.02x\gtrsim 0.02 the effect of doping on ρs(x)\rho_s(x) appears to level off. The values for ρs(x)\rho_s(x) derived from T_1 for T500T\gtrsim 500 K are much larger than the ones estimated from the temperature behavior of sublattice magnetization in the ordered phase (TTNT\leq T_N). It is argued that these features are consistent with the hypothesis of formation of stripes of microsegregated holes.Comment: 10 pages, 3 figure

    Dynamics of Magnetic Defects in Heavy Fermion LiV2O4 from Stretched Exponential 7Li NMR Relaxation

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    7Li NMR measurements on LiV2O4 from 0.5 to 4.2 K are reported. A small concentration of magnetic defects within the structure drastically changes the 7Li nuclear magnetization relaxation versus time from a pure exponential as in pure LiV2O4 to a stretched exponential, indicating glassy behavior of the magnetic defects. The stretched exponential function is described as arising from a distribution of 7Li nuclear spin-lattice relaxation rates and we present a model for the distribution in terms of the dynamics of the magnetic defects. Our results explain the origin of recent puzzling 7Li NMR literature data on LiV2O4 and our model is likely applicable to other glassy systems.Comment: Four typeset pages including four figure

    High-Resolution Topography along Surface Rupture of the 16 October 1999 Hector Mine, California, Earthquake (M_w 7.1) from Airborne Laser Swath Mapping

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    In order to document surface rupture associated with the Hector Mine earthquake, in particular, the area of maximum slip and the deformed surface of Lavic Lake playa, we acquired high-resolution data using relatively new topographic-mapping methods. We performed a raster-laser scan of the main surface breaks along the entire rupture zone, as well as along an unruptured portion of the Bullion fault. The image of the ground surface produced by this method is highly detailed, comparable to that obtained when geologists make particularly detailed site maps for geomorphic or paleoseismic studies. In this case, however, for the first time after a surface-rupturing earthquake, the detailed mapping is along the entire fault zone rather than being confined to selected sites. These data are geodetically referenced, using the Global Positioning System, thus enabling more accurate mapping of the rupture traces. In addition, digital photographs taken along the same flight lines can be overlaid onto the precise topographic data, improving terrain visualization. We demonstrate the potential of these techniques for measuring fault-slip vectors

    Magnetoresistance Anomalies in Antiferromagnetic YBa_2Cu_3O_{6+x}: Fingerprints of Charged Stripes

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    We report novel features in the in-plane magnetoresistance (MR) of heavily underdoped YBa_2Cu_3O_{6+x}, which unveil a developed ``charged stripe'' structure in this system. One of the striking features is an anisotropy of the MR with a "d-wave" symmetry upon rotating the magnetic field H within the ab plane, which is caused by the rotation of the stripes with the external field. With decreasing temperature, a hysteresis shows up below ~20 K in the MR curve as a function of H and finally below 10 K the magnetic-field application produces a persistent change in the resistivity. This "memory effect" is caused by the freezing of the directionally-ordered stripes.Comment: 4 pages, 6 figures, final version, to appear in 4 October 1999 issue of PR

    ^{17}O and ^{51}V NMR for the zigzag spin-1 chain compound CaV2O4

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    51^{51}V NMR studies on CaV2O4 single crystals and 17^{17}O NMR studies on 17^{17}O-enriched powder samples are reported. The temperature dependences of the 17^{17}O NMR line width and nuclear spin-lattice relaxation rate give strong evidence for a long-range antiferromagnetic transition at Tn = 78 K in the powder. Magnetic susceptibility measurements show that Tn = 69 K in the crystals. A zero-field 51^{51}V NMR signal was observed at low temperatures (f \approx 237 MHz at 4.2 K) in the crystals. The field swept spectra with the field in different directions suggest the presence of two antiferromagnetic substructures. Each substructure is collinear, with the easy axes of the two substructures separated by an angle of 19(1) degree, and with their average direction pointing approximately along the b-axis of the crystal structure. The two spin substructures contain equal number of spins. The temperature dependence of the ordered moment, measured up to 45 K, shows the presence of an energy gap Eg in the antiferromagnetic spin wave excitation spectrum. Antiferromagnetic spin wave theory suggests that Eg lies between 64 and 98 K.Comment: 11 pages, 14 figures. v2: 2 new figures; version published in Phys. Rev.

    Coordinated X-ray and Optical observations of Star-Planet Interaction in HD 17156

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    The large number of close-in Jupiter-size exoplanets prompts the question whether star-planet interaction (SPI) effects can be detected. We focused our attention on the system HD 17156, having a Jupiter-mass planet in a very eccentric orbit. Here we present results of the XMM-Newton observations and of a five months coordinated optical campaign with the HARPS-N spectrograph. We observed HD 17156 with XMM-Newton when the planet was approaching the apoastron and then at the following periastron passage, quasi simultaneously with HARPS-N. We obtained a clear (5.5σ\approx 5.5\sigma) X-ray detection only at the periastron visit, accompanied by a significant increase of the RHKR'_{\rm HK} chromospheric index. We discuss two possible scenarios for the activity enhancement: magnetic reconnection and flaring or accretion onto the star of material tidally stripped from the planet. In any case, this is possibly the first evidence of a magnetic SPI effect caught in action

    Implications of Charge Ordering for Single-Particle Properties of High-Tc Superconductors

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    The consequences of disordered charge stripes and antiphase spin domains for the properties of the high-temperature superconductors are studied. We focus on angle-resolved photoemission spectroscopy and optical conductivity, and show that the many unusual features of the experimentally observed spectra can be understood naturally in this way. This interpretation of the data, when combined with evidence from neutron scattering and NMR, suggests that disordered and fluctuating stripe phases are a common feature of high-temperature superconductors.Comment: 4 pages, figures by fax or mai
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