Electronic structure of Ca1−x_{1-x}Srx_xVO3_3: a tale of two energy-scales

We investigate the electronic structure of Ca$_{1-x}$Sr$_x$VO$_3$ using photoemission spectroscopy. Core level spectra establish an electronic phase separation at the surface, leading to distinctly different surface electronic structure compared to the bulk. Analysis of the photoemission spectra of this system allowed us to separate the surface and bulk contributions. These results help us to understand properties related to two vastly differing energy-scales, namely the low energy-scale of thermal excitations (~$k_{B}T$) and the high-energy scale related to Coulomb and other electronic interactions.Comment: 4 pages and 3 figures. Europhysics Letters (appearing

Fermi Surface of 3d^1 Perovskite CaVO3 Near the Mott Transition

We present a detailed de Haas van Alphen effect study of the perovskite CaVO3, offering an unprecedented test of electronic structure calculations in a 3d transition metal oxide. Our experimental and calculated Fermi surfaces are in good agreement -- but only if we ignore large orthorhombic distortions of the cubic perovskite structure. Subtle discrepancies may shed light on an apparent conflict between the low energy properties of CaVO3, which are those of a simple metal, and high energy probes which reveal strong correlations that place CaVO3 on the verge of a metal-insulator transition.Comment: 4 pages, 4 figures (REVTeX

Giant Intrinsic Spin and Orbital Hall Effects in Sr2MO4 (M=Ru,Rh,Mo)

We investigate the intrinsic spin Hall conductivity (SHC) and the d-orbital Hall conductivity (OHC) in metallic d-electron systems, by focusing on the t_{2g}-orbital tight-binding model for Sr2MO4 (M=Ru,Rh,Mo). The conductivities obtained are one or two orders of magnitude larger than predicted values for p-type semiconductors with 5% hole doping. The origin of these giant Hall effects is the ``effective Aharonov-Bohm phase'' that is induced by the d-atomic angular momentum in connection with the spin-orbit interaction and the inter-orbital hopping integrals. The huge SHC and OHC generated by this mechanism are expected to be ubiquitous in multiorbital transition metal complexes, which pens the possibility of realizing spintronics as well as orbitronics devices.Comment: 5 pages, accepted for publication in PR

A mechanism for unipolar resistance switching in oxide non-volatile memory devices

Building on a recently introduced model for non-volatile resistive switching, we propose a mechanism for unipolar resistance switching in metal-insulator-metal sandwich structures. The commutation from the high to low resistance state and back can be achieved with successive voltage sweeps of the same polarity. Electronic correlation effects at the metal-insulator interface are found to play a key role to produce a resistive commutation effect in qualitative agreement with recent experimental reports on binary transition metal oxide based sandwich structures.Comment: 4 pages, 2 figure

Tunnel magnetoresistance and interfacial electronic state

We study the relation between tunnel magnetoresistance (TMR) and interfacial electronic states modified by magnetic impurities introduced at the interface of the ferromagnetic tunnel junctions, by making use of the periodic Anderson model and the linear response theory. It is indicated that the TMR ratio is strongly reduced depending on the position of the $d$-levels of impurities, based on reduction in the spin-dependent $s$-electron tunneling in the majority spin state. The results are compared with experimental results for Cr-dusted ferromagnetic tunnel junctions, and also with results for metallic multilayers for which similar reduction in giant magnetoresistance has been reported.Comment: 5 pages, 4 figures, 2 column revtex4 format, ICMFS 2002 (Kyoto

Charge transport in two dimensional electron gas/superconductor junctions with Rashba spin-orbit coupling

We have studied the tunneling conductance in two dimensional electron gas / insulator / superconductor junctions in the presence of Rashba spin-orbit coupling (RSOC). It is found that for low insulating barrier the tunneling conductance is suppressed by the RSOC while for high insulating barrier it is almost independent of the RSOC. We also find the reentrant behavior of the conductance at zero voltage as a function of RSOC for intermediate insulating barrier strength. The results are essentially different from those predicted in ferromagnet / superconductor junctions. The present derivation of the conductance is applicable to arbitrary velocity operator with off-diagonal components.Comment: 8 pages, 6 figure

Correlation Inequalities for Quantum Spin Systems with Quenched Centered Disorder

It is shown that random quantum spin systems with centered disorder satisfy correlation inequalities previously proved (arXiv:cond-mat/0612371) in the classical case. Consequences include monotone approach of pressure and ground state energy to the thermodynamic limit. Signs and bounds on the surface pressures for different boundary conditions are also derived for finite range potentials.Comment: 4 page

Perturbation theory for localized solutions of sine-Gordon equation: decay of a breather and pinning by microresistor

We develop a perturbation theory that describes bound states of solitons localized in a confined area. External forces and influence of inhomogeneities are taken into account as perturbations to exact solutions of the sine-Gordon equation. We have investigated two special cases of fluxon trapped by a microresistor and decay of a breather under dissipation. Also, we have carried out numerical simulations with dissipative sine-Gordon equation and made comparison with the McLaughlin-Scott theory. Significant distinction between the McLaughlin-Scott calculation for a breather decay and our numerical result indicates that the history dependence of the breather evolution can not be neglected even for small damping parameter

Extrinsic Entwined with Intrinsic Spin Hall Effect in Disordered Mesoscopic Bars

We show that pure spin Hall current, flowing out of a four-terminal phase-coherent two-dimensional electron gas (2DEG) within inversion asymmetric semiconductor heterostructure, contains contributions from both the extrinsic mechanisms (spin-orbit dependent scattering off impurities) and the intrinsic ones (due to the Rashba coupling). While the extrinsic contribution vanishes in the weakly and strongly disordered limits, and the intrinsic one dominates in the quasiballistic limit, in the crossover transport regime the spin Hall conductance, exhibiting sample-to-sample large fluctuations and sign change, is not simply reducible to either of the two mechanisms, which can be relevant for interpretation of experiments on dirty 2DEGs [V. Sih et al., Nature Phys. 1, 31 (2005)].Comment: 5 pages, 3 color EPS figure

Band-width control in a perovskite-type 3d^1 correlated metal Ca_1-xSr_xVO_3. II. Optical spectroscopy investigation

Optical conductivity spectra of single crystals of Ca_1-xSr_xVO_3 have been studied to elucidate how the electronic behavior depends on the strength of the electron correlation without changing the nominal number of electrons per vanadium atom. The effective mass deduced by the analysis of the Drude-like contribution do not show critical enhancement, even though the system is close to the Mott transition. Besides the Drude-like contribution, two anomalous features were observed in the optical conductivity spectra of the intraband transition within the 3d band. These features can be assigned to transitions involving the incoherent and coherent bands near the Fermi level. The large spectral weight redistribution in this system, however, does not involve a large mass enhancement.Comment: 12 pages in a Phys. Rev. B camera-ready format with 16 EPS figures embedded. LaTeX 2.09 source file using "camera.sty" and "prbplug.sty" provided by N. Shirakawa. For OzTeX (Macintosh), use "ozfig.sty" instead of "psfig.sty". "ozfig.sty" can be also obtained by e-mail request to N. Shirakawa: . Submitted to Phys. Rev. B. See "Part I (by Inoue et al.)" at cond-mat/980107