2,180 research outputs found
Anomalous Spin Dynamics in Doped Quantum Antiferromagnets
Finite-temperature spin dynamics in planar t-J model is studied using the
method based on the Lanczos diagonalization of small systems. Dynamical spin
structure factor at moderate dopings shows the coexistence of free-fermion-like
and spin-fluctuation timescales. At T<J, the low-frequency and static
susceptibility show pronounced T dependence, supporting a scenario, related to
the marginal Fermi-liquid one, for the explanation of neutron-scattering and
NMR-relaxation experiments in cuprates. Calculated NMR relaxation rates
reasonably reproduce experimental ones.Comment: 10 pages + 4 figures, Postscript in uuencoded compressed tar file,
IJS-TP-94/2
Three-dimensional (3D) Fast Neutron Tomography at the Low Energy Neutron Source (LENS)
AbstractWe have constructed a neutron imaging station at the Low Energy Neutron Source (LENS), located within the Center for the Exploration of Energy and Matter at Indiana University. In contrast to many existing neutron imaging stations, we utilize a broad range of neutron energies, extending into the fast neutron regime, to take advantage of the higher fluxes and larger penetrating power of these high-energy neutrons. The imaging station consists of a collimator to define the beam, a rotating sample stage, and a cooled charge-coupled device camera (Alta U6) using a scintillator. A LiF + ZnS screen is used to produce scintillation light. Typical image collection times are a few seconds for a aperture to sample distance ratio of 100, yielding a spatial resolution of 0.2 × 0.2 mm2. Examples of the scanned and calculated image are presented
Target Performance at the Low Energy Neutron Source
AbstractThe Indiana University Low Energy Neutron Source (LENS) production target was recently upgraded to handle the high power 13 MeV proton pulsed beam. The target, a 2 inch diameter beryllium disk, is 1.2 millimeters thick allowing the 13 MeV protons to pass completely through the target and stop in the cooling water eliminating the buildup of protons inside the beryllium. This change along with upgrading the cooling water system has produced the most reliable target to date for LENS operations. Details about the failure modes will be presented
Spin diffusion of the t-J model
The spin-diffusion constant of the 2D model is calculated for the first
time using an analytical approach at high temperatures and a recently-developed
numerical method based on the Lanczos technique combined with random sampling
in the intermediate temperature regime. A simple relation, ,
between spin conductivity and spin diffusion is established and used to
calculate the latter. In the high-temperature and low-doping limit the
calculated diffusion constant agrees with known results for the Heisenberg
model. At small hole doping, increases approximately linearly with
doping, which leads us to an important conclusion that hopping processes
enhance spin diffusion at high temperatures. At modest hole doping, , diffusion exhibits a nonmonotonic temperature dependence, which
indicates anomalous spin dynamics at small frequencies.Comment: 12 pages with figure
NMR relaxation in half-integer antiferromagnetic spin chains
Nuclear relaxation in half-integer spin chains at low temperatures (T << J,
the antiferromagnetic exchange constant) is dominated by dissipation from a gas
of thermally-excited, overdamped, spinons. The universal low temperature
dependence of the relaxation rates and is computed.Comment: 7 pages, 1 uuencoded postscript figure appende
Quantum Disordered Regime and Spin Gap in the Cuprate Superconductors
We discuss the crossover from the quantum critical, , to the quantum
disordered regime in high-T materials in relation to the experimental data
on the nuclear relaxation, bulk susceptibility, and inelastic neutron
scattering. In our scenario, the spin excitations develop a gap
well above T, which is supplemented by the
quasiparticle gap below T. The above experiments yield consistent estimates
for the value of the spin gap, which increases as the correlation length
decreases.Comment: 14 pages, REVTeX v3.0, PostScript file for 3 figures is attached,
UIUC-P-93-07-06
Spin Dynamics of La_2CuO_4 and the Two-Dimensional Heisenberg Model
The spin-lattice relaxation rate and the spin echo decay rate
for the 2D Heisenberg model are calculated using quantum Monte Carlo
and maximum entropy analytic continuation. The results are compared to recent
experiments on LaCuO, as well as predictions based on the non-linear
-model.Comment: Compressed & uuencoded Postscript file (4 pages with figures
Bulk and Surface Contributions to Ionisation Potentials of Metal Oxides
Determining the absolute band edge positions in solid
materials is crucial for optimising their performance in wide-ranging applications including photocatalysis and electronic devices. However, obtaining absolute energies is challenging, as seen in CeO2, where experimental measurements show substantial discrepancies in the ionisation potential (IP). Here, we have combined several theoretical approaches, from classical electrostatics to quantum mechanics, to elucidate the bulk and surface contributions to the IP of metal oxides. We have determined a theoretical bulk contribution to the IP of stoichiometric CeO2 of only 5.38 eV, while surface orientation results in intrinsic IP variations from 4.2 eV to 8.2 eV. Highly tuneable IPs were also found in TiO2, ZrO2, and HfO2, in which surface polarisation plays a pivotal role in long-range energy level shifting. Our analysis, in addition to rationalising the observed range of experimental results, provides a firm basis for future interpretations of experimental and computational studies of oxide band structures
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