Strong orientational effect of stretched aerogel on the 3He order parameter

Deformation of aerogel strongly modifies the orientation of the order parameter of superfluid 3He confined in aerogel. We used a radial squeezing of aerogel to keep the orbital angular momentum of the 3He Cooper pairs in the plane perpendicular to the magnetic field. We did not find strong evidence for a "polar" phase, with a nodal line along the equator of the Fermi surface, predicted to occur at large radial squeezing. Instead we observed 3He-A with a clear experimental evidence of the destruction of the long-range order by random anisotropy -- the Larkin-Imry-Ma effect. In 3He-B we observed and identified new modes of NMR, which are impossible to obtain in bulk 3He-B. One of these modes is characterized by a repulsive interaction between magnons, which is suitable for the magnon Bose-Einstein condensation (BEC).Comment: 4 pages, 3 figures, revtex, submitted to PR

Vortex core transitions in superfluid 3He in globally anisotropic aerogels

Core structures of a single vortex in A-like and B-like phases of superfluid 3He in uniaxially compressed and stretched aerogels are studied by numerically solving Ginzburg-Landau equations derived microscopically. It is found that, although any uniaxial deformation leads to a wider A-like phase with the axial pairing in the pressure-temperature phase diagram, the vortex core states in the two phases in aerogel depend highly on the type of deformation. In a compressed aerogel, the first-order vortex core transition (VCT) previously seen in the bulk B phase appears at any pressure in the B-like phase while no strange vortex core is expected in the corresponding A-like phase. By contrast, in a stretched aerogel, the VCT in the B-like phase is lost while another VCT is expected to occur between a nonunitary core and a polar one in the A-like phase. Experimental search for these results is hoped to understand correlation between superfluid 3He and aerogel structure.Comment: 7 pages, 6 figures Text was changed. Resubmitted versio

Bolometric calibration of a superfluid 3^3He detector for Dark Matter search: direct measurement of the scintillated energy fraction for neutron, electron and muon events

We report on the calibration of a superfluid $^3$He bolometer developed for the search of non-baryonic Dark Matter. Precise thermometry is achieved by the direct measurement of thermal excitations using Vibrating Wire Resonators (VWRs). The heating pulses for calibration were produced by the direct quantum process of quasiparticle generation by other VWRs present. The bolometric calibration factor is analyzed as a function of temperature and excitation level of the sensing VWR. The calibration is compared to bolometric measurements of the nuclear neutron capture reaction and heat depositions by cosmic muons and low energy electrons. The comparison allows a quantitative estimation of the ultra-violet scintillation rate of irradiated helium, demonstrating the possibility of efficient electron recoil event rejection.Comment: 17 pages, submitted to Nuc. Instr. Meth.

NMR in Superfluid A-like Phase of 3^3He Confined in Globally Deformed Aerogel in Tilted Magnetic Field

NMR spectra in superfluid A-like phases confined in axially deformed aerogel in presence of a magnetic field inclined with respect to deformation axis is considered. The characteristic features of dipole frequency shift in axially compressed and axially stretched cases are compared. In particular, it is shown that in axially stretched aerogel environment the stability region of coherently spin precessing mode is rather narrow due to the U(1)LIM effect.Comment: 8 pages, 2 figure

New Chiral Phases of Superfluid 3He Stabilized by Anisotropic Silica Aerogel

A rich variety of Fermi systems condense by forming bound pairs, including high temperature [1] and heavy fermion [2] superconductors, Sr2RuO4 [3], cold atomic gases [4], and superfluid 3He [5]. Some of these form exotic quantum states having non-zero orbital angular momentum. We have discovered, in the case of 3He, that anisotropic disorder, engineered from highly porous silica aerogel, stabilizes a chiral superfluid state that otherwise would not exist. Additionally, we find that the chiral axis of this state can be uniquely oriented with the application of a magnetic field perpendicular to the aerogel anisotropy axis. At suffciently low temperature we observe a sharp transition from a uniformly oriented chiral state to a disordered structure consistent with locally ordered domains, contrary to expectations for a superfluid glass phase [6].Comment: 6 pages, 4 figure, and Supplementary Informatio

Mass coupling and Q−1ofimpurity−limitednormalQ^{-1} of impurity-limited normal ^3$He in a torsion pendulum

We present results of the $Q^{-1}$ and period shift, $\Delta P$, for $^3$He confined in a 98% nominal open aerogel on a torsion pendulum. The aerogel is compressed uniaxially by 10% along a direction aligned to the torsion pendulum axis and was grown within a 400 $\mu$m tall pancake (after compression) similar to an Andronikashvili geometry. The result is a high $Q$ pendulum able to resolve $Q^{-1}$ and mass coupling of the impurity-limited $^3$He over the whole temperature range. After measuring the empty cell background, we filled the cell above the critical point and observe a temperature dependent period shift, $\Delta P$, between 100 mK and 3 mK that is 2.9$$ of the period shift (after filling) at 100 mK. The $Q^{-1}$ due to the $^3$He decreases by an order of magnitude between 100 mK and 3 mK at a pressure of $0.14\pm0.03$ bar. We compare the observable quantities to the corresponding calculated $Q^{-1}$ and period shift for bulk $^3$He.Comment: 8 pages, 3 figure

Orbital glass and spin glass states of 3He-A in aerogel

Glass states of superfluid A-like phase of 3He in aerogel induced by random orientations of aerogel strands are investigated theoretically and experimentally. In anisotropic aerogel with stretching deformation two glass phases are observed. Both phases represent the anisotropic glass of the orbital ferromagnetic vector l -- the orbital glass (OG). The phases differ by the spin structure: the spin nematic vector d can be either in the ordered spin nematic (SN) state or in the disordered spin-glass (SG) state. The first phase (OG-SN) is formed under conventional cooling from normal 3He. The second phase (OG-SG) is metastable, being obtained by cooling through the superfluid transition temperature, when large enough resonant continuous radio-frequency excitation are applied. NMR signature of different phases allows us to measure the parameter of the global anisotropy of the orbital glass induced by deformation.Comment: 7 pages, 6 figures, Submitted to Pis'ma v ZhETF (JETP Letters

Electrospray Ionization with High-Resolution Mass Spectrometry as a Tool for Lignomics: Lignin Mass Spectrum Deconvolution

Capability to characterize lignin, lignocellulose, and their degradation products is essential for development of new renewable feedstocks. Electrospray ionization high-resolution time-offlight mass spectrometry (ESI HR TOF MS) method was developed expanding the lignomics toolkit while targeting the simultaneous detection of low and high molecular weight (MW) lignin species. The effect of a broad range of electrolytes and various ionization conditions on ion formation and ionization effectiveness was studied using a suite of mono-, di- and triarene lignin model compounds as well as intact lignin. Contrary to the previous studies, the positive ionization mode was found to be more effective for methoxy-substituted arenes and polyphenols, i.e., species of a broadly varied MW structurally similar to the native lignin. For the first time, we report an effective formation of multiply charged species of lignin with the subsequent mass spectrum deconvolution in the presence of 100 mmol·L-1 formic acid in the positive ESI mode. The developed method enabled the detection of lignin species with an MW between 150 and 9,000 Da or higher, depending on the mass analyzer. The obtained Mn and Mw values of 1,500 and 2,500 Da, respectively, were in good agreement with those determined by gel permeation chromatography. Furthermore, the deconvoluted ESI mass spectrum was similar to that obtained with matrixassisted laser desorption/ionization (MALDI) TOF MS, yet featuring a higher signal-to-noise ratio. The formation of multiply charged species was confirmed with ESI ion mobility HR Q-TOF MS