811 research outputs found
Synergic Extraction of Rare Earth Elements with Thenoyltrifluoroacetone and Neutral Bidentate Ligands
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Substoichiometric Isotope Dilution Analysis of Vanadium by Synergistic Extraction
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Solvent Extraction of Lanthanoid(III) with 18-Crown-6 and Trichloroacetate Ion
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Full counting statistics for transport through a molecular quantum dot magnet
Full counting statistics (FCS) for the transport through a molecular quantum
dot magnet is studied theoretically in the incoherent tunneling regime. We
consider a model describing a single-level quantum dot, magnetically coupled to
an additional local spin, the latter representing the total molecular spin s.
We also assume that the system is in the strong Coulomb blockade regime, i.e.,
double occupancy on the dot is forbidden. The master equation approach to FCS
introduced in Ref. [12] is applied to derive a generating function yielding the
FCS of charge and current. In the master equation approach, Clebsch-Gordan
coefficients appear in the transition probabilities, whereas the derivation of
generating function reduces to solving the eigenvalue problem of a modified
master equation with counting fields. To be more specific, one needs only the
eigenstate which collapses smoothly to the zero-eigenvalue stationary state in
the limit of vanishing counting fields. We discovered that in our problem with
arbitrary spin s, some quartic relations among Clebsch-Gordan coefficients
allow us to identify the desired eigenspace without solving the whole problem.
Thus we find analytically the FCS generating function in the following two
cases: i) both spin sectors lying in the bias window, ii) only one of such spin
sectors lying in the bias window. Based on the obtained analytic expressions,
we also developed a numerical analysis in order to perform a similar
contour-plot of the joint charge-current distribution function, which have
recently been introduced in Ref. [13], here in the case of molecular quantum
dot magnet problem.Comment: 17 pages, 5 figure
Discontinuous Transition from a Real Bound State to Virtual Bound State in a Mixed-Valence State of SmS
Golden SmS is a paramagnetic, mixed-valence system with a pseudogap. With
increasing pressure across a critical pressure Pc, the system undergoes a
discontinuous transition into a metallic, anti-ferromagnetically ordered state.
By using a combination of thermodynamic, transport, and magnetic measurements,
we show that the pseudogap results from the formation of a local bound state
with spin singlet. We further argue that the transition Pc is regarded as a
transition from an insulating electron-hole gas to a Kondo metal, i.e., from a
spatially bound state to a Kondo virtually bound state between 4f and
conduction electrons.Comment: 5 pages, 5 figure
Liquid-Liquid Partition Coefficients of Nickel (II) and Copper (II) Thenoyltrifluoroacetonates and Dimethyldithiocarbamates
開始ページ、終了ページ: 冊子体のページ付
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