Feshbach blockade: single-photon nonlinear optics using resonantly enhanced cavity-polariton scattering from biexciton states

We theoretically demonstrate how the resonant coupling between a pair of cavity-polaritons and a biexciton state can lead to a large single-photon Kerr nonlinearity in a semiconductor solid-state system. A fully analytical model of the scattering process between a pair of cavity-polaritons is developed, which explicitly includes the biexcitonic intermediate state. A dramatic enhancement of the polariton-polariton interactions is predicted in the vicinity of the biexciton Feshbach resonance. Application to the generation of non-classical light from polariton dots is discussed

Quantum-dot-spin single-photon interface

Using background-free detection of spin-state-dependent resonance fluorescence from a single-electron charged quantum dot with an efficiency of 0:1%, we realize a single spin-photon interface where the detection of a scattered photon with 300 picosecond time resolution projects the quantum dot spin to a definite spin eigenstate with fidelity exceeding 99%. The bunching of resonantly scattered photons reveals information about electron spin dynamics. High-fidelity fast spin-state initialization heralded by a single photon enables the realization of quantum information processing tasks such as non-deterministic distant spin entanglement. Given that we could suppress the measurement back-action to well below the natural spin-flip rate, realization of a quantum non-demolition measurement of a single spin could be achieved by increasing the fluorescence collection efficiency by a factor exceeding 20 using a photonic nanostructure

Quantum measurement of a mesoscopic spin ensemble

We describe a method for precise estimation of the polarization of a mesoscopic spin ensemble by using its coupling to a single two-level system. Our approach requires a minimal number of measurements on the two-level system for a given measurement precision. We consider the application of this method to the case of nuclear spin ensemble defined by a single electron-charged quantum dot: we show that decreasing the electron spin dephasing due to nuclei and increasing the fidelity of nuclear-spin-based quantum memory could be within the reach of present day experiments.Comment: 8 pages, 2 figures; minor changes, published versio

Nonlinear Optics and Quantum Entanglement of Ultra-Slow Single Photons

Two light pulses propagating with ultra-slow group velocities in a coherently prepared atomic gas exhibit dissipation-free nonlinear coupling of an unprecedented strength. This enables a single-photon pulse to coherently control or manipulate the quantum state of the other. Processes of this kind result in generation of entangled states of radiation field and open up new prospectives for quantum information processing

Polariton Analysis of a Four-Level Atom Strongly Coupled to a Cavity Mode

We present a complete analytical solution for a single four-level atom strongly coupled to a cavity field mode and driven by external coherent laser fields. The four-level atomic system consists of a three-level subsystem in an EIT configuration, plus an additional atomic level; this system has been predicted to exhibit a photon blockade effect. The solution is presented in terms of polaritons. An effective Hamiltonian obtained by this procedure is analyzed from the viewpoint of an effective two-level system, and the dynamic Stark splitting of dressed states is discussed. The fluorescence spectrum of light exiting the cavity mode is analyzed and relevant transitions identified.Comment: 12 pages, 9 figure

Coupled cavities for enhancing the cross-phase modulation in electromagnetically induced transparency

We propose an optical double-cavity resonator whose response to a signal is similar to that of an Electromagnetically Induced Transparency (EIT) medium. A combination of such a device with a four-level EIT medium can serve for achieving large cross-Kerr modulation of a probe field by a signal field. This would offer the possibility of building a quantum logic gate based on photonic qubits. We discuss the technical requirements that are necessary for realizing a probe-photon phase shift of Pi caused by a single-photon signal. The main difficulty is the requirement of an ultra-low reflectivity beamsplitter and to operate a sufficiently dense cool EIT medium in a cavity.Comment: 10 pages, 5 figures, REVTeX, to appear in Phys. Rev. A (v2 - minor changes in discussion of experimental conditions

Cavity-induced coherence effects in spontaneous emission from pre-Selection of polarization

Spontaneous emission can create coherences in a multilevel atom having close lying levels, subject to the condition that the atomic dipole matrix elements are non-orthogonal. This condition is rarely met in atomic systems. We report the possibility of bypassing this condition and thereby creating coherences by letting the atom with orthogonal dipoles to interact with the vacuum of a pre-selected polarized cavity mode rather than the free space vacuum. We derive a master equation for the reduced density operator of a model four level atomic system, and obtain its analytical solution to describe the interference effects. We report the quantum beat structure in the populations.Comment: 6 pages in REVTEX multicolumn format, 5 figures, new references added, journal reference adde

New dinuclear cyanido complexes with amine alcohol ligand: synthesis, characterization and biotechnological application potential

In this study, the cyanido complexes given by the formula [Ni(Abut)Ni(CN)4]·8H2O (C1), [Cu(Abut)2Ni(CN)4]·7H2O (C2), [Zn(Abut)Ni(CN)4]·8H2O (C3) and [Cd(Abut)Ni(CN)4]·7H2O (C4) were obtained by microwave synthesis method. The powder forms of the complexes were characterized by elemental, FT-IR spectroscopy, and thermal analysis. And also antibacterial, antibiofilm and anticancer activities were investigated. The splitting stretching bands of cyanido groups in the FT-IR spectra of C1-C4 indicated the assets of terminal and end cyanido groups. The antibacterial activities of C1-C4 were tested with nine Gram negative and six Gram positive bacteria. The most efficient antibacterial activity of complexes was observed at 1000 µg/ml-1 concentration. Anticancer activity was tested using HeLa cell line and MTT test. The studied cyanide complexes have been shown to decrease the viability of HeLa cells with IC50 values 14.86, 6.5, 7.2 and 19.2 µg/ml for C1, C2, C3 and C4 complex, respectively