2,193 research outputs found
4p states and X-Ray Spectroscopy
The 4p states in transition metals and their compounds usually play minor
roles on their physical quantities. Recent development of resonant x-ray
scattering (RXS) at the K-edge of transition metals, however, casts light on
the 4p states, because the signals on orbital and magnetic superlattice spots
are brought about by the modulation in the 4p states. The 4p states are
extending in solids and thereby sensitive to electronic states at neighboring
sites. This characteristic determines the mechanism of RXS that the intensity
on the orbital superlattice spots are mainly generated by the lattice
distortion and those on magnetic superlattice spots by the coupling of the 4p
states with the orbital polarization in the 3d states at neighboring sites.
Taking up typical examples for orbital and magnetic RXS, we demonstrate these
mechanisms on the basis of the band structure calculation. Finally, we study
the MCD spectra at the K-edge, demonstrating that the same mechanism as the
magnetic RXS is working.Comment: 9 pages, 9 figures, submitted to Physica Scripta (comment
X-Ray Magnetic Circular Dichroism at the K edge of Mn3GaC
We theoretically investigate the origin of the x-ray magnetic circular
dichroism (XMCD) spectra at the K edges of Mn and Ga in the ferromagnetic phase
of Mn3GaC on the basis of an ab initio calculation. Taking account of the
spin-orbit interaction in the LDA scheme, we obtain the XMCD spectra in
excellent agreement with the recent experiment. We have analyzed the origin of
each structure, and thus elucidated the mechanism of inducing the orbital
polarization in the p symmetric states. We also discuss a simple sum rule
connecting the XMCD spectra with the orbital moment in the p symmetric states.Comment: 5 pages, 5 figures, accepted for publication in Physical Review
Spin Excitations and Sum Rules in the Heisenberg Antiferromagnet
Various bounds for the energy of collective excitations in the Heisenberg
antiferromagnet are presented and discussed using the formalism of sum rules.
We show that the Feynman approximation significantly overestimates (by about
30\% in the square lattice) the spin velocity due to the non
negligible contribution of multi magnons to the energy weighted sum rule. We
also discuss a different, Goldstone type bound depending explicitly on the
order parameter (staggered magnetization). This bound is shown to be
proportional to the dispersion of classical spin wave theory with a
q-independent normalization factor. Rigorous bounds for the excitation energies
in the anisotropic Heisenberg model are also presented.Comment: 26 pages, Plain TeX including 1 PostScript figure, UTF-307-10/9
Magnetic Impurity in the two-dimensional Heisenberg Antiferromagnet
We analyze the ground state properties of the two-dimensional quantum
antiferromagnet with a S=1/2 Kondo impurity. Perturbation theory around the
strong Kondo coupling limit is developed and the results compared with studies,
based on exact diagonalization of small clusters. We find that at intermediate
coupling the impurity is partially screened and the magnetization locally
suppressed. A local singlet between the impurity and the host spin is formed
asymptotically.Comment: 12 REVTex pages, 4 Postscript figure
Direct Calculation of the Spin Stiffness in the -- Heisenberg Antiferromagnet
We calculate the spin stiffness for the frustrated
spin- Heisenberg antiferromagnet on a square lattice by exact
diagonalizations on finite clusters of up to sites followed by
extrapolations to the thermodynamic limit. For the non-frustrated case, we find
that , in excellent agreement with the best
results obtained by other means. Turning on frustration, the extrapolated
stiffness vanishes for . In this
intermediate region, the finite-size scaling works poorly -- an additional sign
that their is neither N\'eel nor collinear magnetic order. Using a hydrodynamic
relation, and previous results for the transverse susceptibility, we also
estimate the spin-wave velocity in the N\'eel-ordered region.Comment: 4 pages, uuencoded compressed ps-file (made with uufiles
Energy separation of single-particle and continuum states in a S=1/2 weakly-coupled chains antiferromagnet
Inelastic neutron scattering is used to study transverse-polarized magnetic
excitations in the quasi-one-dimensional S=1/2 antiferromagnet BaCu_2Si_2O_7,
where the saturation value for the N\'eel order parameter is per spin. At low energies the spectrum is totally dominated by
resolution-limited spin wave-like excitations. An excitation continuum sets in
above a well-defined threshold frequency. Experimental results are discussed in
the context of current theories for weakly-interacting quantum half-integer
spin chains.Comment: 4 pages 4 figure
Rare earth contributions to the X-ray magnetic circular dichroism at the Co K edge in rare earth-cobalt compounds investigated by multiple-scattering calculations
The X-ray magnetic circular dichroism (XMCD) has been measured at the Co K
edge in Co-hcp and R-Co compounds (R=La, Tb, Dy). The structure of the
experimental XMCD spectra in the near-edge region has been observed to be
highly sensitive to the magnetic environment of the absorbing site.
Calculations of the XMCD have been carried out at the Co K edge in Co metal,
LaCo and TbCo within the multiple-scattering framework including the
spin-orbit coupling. In the three systems, the XMCD spectra in the near-edge
region are well reproduced. The possibility to separate and quantitatively
estimate the local effects from those due to the neighboring atoms in the XMCD
cross section makes possible a more physical understanding of the spectra. The
present results emphasize the major role played by the states of the Tb
ions in the XMCD spectrum at the Co K edge in the TbCo compound.Comment: 34 pages, revtex, 10 eps figures included with epsf, after referee
revie
Spectral properties of the t-J model in the presence of hole-phonon interaction
We examine the effects of electron-phonon interaction on the dynamics of the
charge carriers doped in two-dimensional (2D) Heisenberg antiferromagnet. The
- model Hamiltonian with a Fr\"ohlich term which couples the holes to a
dispersionless (optical) phonon mode is considered for low doping
concentration. The evolution of the spectral density function, the density of
states, and the momentum distribution function of the holes with an increase of
the hole-phonon coupling constant is studied numerically. As the coupling
to a phonon mode increases the quasiparticle spectral weight decreases and a
``phonon satellite'' feature close to the quasi-particle peak becomes more
pronounced. Furthermore, strong electron-phonon coupling smears the
multi-magnon resonances (``string states'') in the incoherent part of the
spectral function. The jump in the momentum distribution function at the Fermi
surface is reduced without changing the hole pocket volume, thereby providing a
numerical verification of Luttinger theorem for this strongly interacting
system. The vertex corrections due to electron- phonon interaction are
negligible in spite of the fact that the ratio of the phonon frequency to the
effective bandwidth is not small.Comment: REVTeX, 20 pages, 9 figures, to be published in Phys. Rev. B (Nov. 1,
1996
Phase diagram of an impurity in the spin-1/2 chain: two channel Kondo effect versus Curie law
We consider a magnetic s=1/2 impurity in the antiferromagnetic spin chain as
a function of two coupling parameters: the symmetric coupling of the impurity
to two sites in the chain and the coupling between the two sites .
By using field theory arguments and numerical calculations we can identify all
possible fixed points and classify the renormalization flow between them, which
leads to a non-trivial phase diagram. Depending on the detailed choice of the
two (frustrating) coupling strengths, the stable phases correspond either to a
decoupled spin with Curie law behavior or to a non-Fermi liquid fixed point
with a logarithmically diverging impurity susceptibility as in the two channel
Kondo effect. Our results resolve a controversy about the renormalization flow.Comment: 5 pages in revtex format including 4 embedded figures (using epsf).
The latest version in PDF format is available from
http://fy.chalmers.se/~eggert/papers/phase-diagram.pd
Resonant X-Ray Magnetic Scattering from CoO
We analyze the recent experiment [W. Neubeck {\em et al.}, Phys. Rev. B
\vol(60,1999,R9912)] for the resonant x-ray magnetic scattering (RXMS) around
the K edge of Co in the antiferromagnet CoO. We propose a mechanism of the RXMS
to make the states couple to the magnetic order: the intraatomic exchange
interaction between the and the states and the - mixing to the
states of neighboring Co atoms. These couplings induce the orbital moment
in the states and make the scattering tensor antisymmetric. Using a
cluster model, we demonstrate that this modification gives rise to a large RXMS
intensity in the dipole process, in good agreement with the experiment. We also
find that the pre-edge peak is generated by the transition to the states
in the quadrupole process, with negligible contribution of the dipole process.
We also discuss the azimuthal angle dependence of the intensity.Comment: 15 pages, 8 figure
- …