2,539 research outputs found
Neutron diffraction, magnetization and ESR studies of pseudocubic Nd(0.75)Ba(0.25)MnO3 and its unusual critical behavior above Tc
Results of structural neutron diffraction study, magnetization and ESR
measure-ments are presented for insulating Nd0.75Ba0.25MnO3, Tc = 129 K. The
crystal structure is refined in the range 4.2-300 K. The compound is found to
exhibit the Jahn-Teller (JT) transition at 250 K. The field cooled (FC)
magnetization data are in a reasonable agreement with the predictions for a 3D
isotropic ferromagnet above Tc. However, these measurements reveal a difference
between the FC and zero FC data in the paramagnetic region. ESR results are
also in a correspondence with behavior of a cubic ferromagnet above T* = 143 K.
It is shown that an anisotropic exchange coupling of the Mn and Nd magnetic
moments can give a substantial contribution in ESR linewidth masking its
critical enhan-cement. The different temperature treatments of the sample
reveal a temperature hysteresis of the ESR spectra below T* indicating an
anomalous response in the paramagnetic region. The study of phase transition in
this manganite suggests change in its character from the second to first order
at T*. The conventional free energy including the magnetization and magnetic
field is not found to describe the first order transition. This suggests that
the charge, orbital and JT phonon degrees of freedom, in addition to
magnetization, may be the critical variables, the unusual character of the
transition being determined by their coupling. Unconventional critical behavior
is attributed to orbital liquid metallic phase that coexists with the initial
orbital ordered phase below T*.Comment: 18 pages, 5 figures, submitted to Phys. Rev.
Low-temperature kinetics of exciton-exciton annihilation of weakly localized one-dimensional Frenkel excitons
We present results of numerical simulations of the kinetics of
exciton-exciton annihilation of weakly localized one-dimensional Frenkel
excitons at low temperatures. We find that the kinetics is represented by two
well-distinguished components: a fast short-time decay and a very slow
long-time tail. The former arises from excitons that initially reside in states
belonging to the same localization segment of the chain, while the slow
component is caused by excitons created on different localization segments. We
show that the usual bi-molecular theory fails in the description of the
behavior found. We also present a qualitative analytical explanation of the
non-exponential behavior observed in both the short- and the long-time decay
components.Comment: Published in J. Chem. Phys. 114, 1 April (2001
Giant oscillations of energy levels in mesoscopic superconductors
The interplay of geometrical and Andreev quantization in mesoscopic
superconductors leads to giant mesoscopic oscillations of energy levels as
functions of the Fermi momentum and/or sample size. Quantization rules are
formulated for closed quasiparticle trajectories in the presence of normal
scattering at the sample boundaries. Two generic examples of mesoscopic systems
are studied: (i) one dimensional Andreev states in a quantum box, (ii) a single
vortex in a mesoscopic cylinder.Comment: 4 pages, 3 figure
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