2,314 research outputs found
Temperature Dependent Polarized XANES Spectra for Zn-doped LSCO system
The cuprates seem to exhibit statistics, dimensionality and phase transitions
in novel ways. The nature of excitations [i.e. quasiparticle or collective],
spin-charge separation, stripes [static and dynamics], inhomogeneities,
psuedogap, effect of impurity dopings [e.g. Zn, Ni] and any other phenomenon in
these materials must be consistently understood. Zn-doped LSCO single crystal
were grown by TSFZ technique. Temperature dependent Polarized XANES [near edge
local structure] spectra were measured at the BL13-B1 [Photon Factory] in the
Flourescence mode from 10 K to 300 K. Since both stripes and nonmagnetic Zn
impurities substituted for Cu give rise to inhomogeneous charge and spin
distribution it is interesting to understand the interplay of Zn impurities and
stripes. To understand these points we have used Zn-doping and some of the
results obtained are as follows: The spectra show a strong dependence with
respect to the polarization angle, , as is evident at any temperature
by comparing the spectra where the electric field vector is parallel with
ab-plane to the one where it is parallel to the c-axis. By using the XANES
[temperature] difference spectra we have determined T* [experimentally we find,
T* 160-170 K] for this sample. The XANES difference spectra shows
that the changes in XANES features are larger in the ab-plane than the c-axis,
this trend is expected since zinc is doped in the ab-plane at the copper site.
Our study also complements the results in literature namely that zinc doping
does not affect the c-axis transport.Comment: To appear in Physica C [ISS2001 Special Issue], related talk
presented at ISS2001 as PC-16, 10 pages revtex and 7 pages of figures (pdf
Ordering of localized moments in Kondo lattice models
We describe the transition from a ferromagnetic phase, to a disordered para-
magnetic phase, which occurs in one-dimensional Kondo lattice models with
partial conduction band filling. The transition is the quantum order-disorder
transition of the transverse-field Ising chain, and reflects double-exchange
ordered regions of localized spins being gradually destroyed as the coupling to
the conduction electrons is reduced. For incommensurate conduction band
filling, the low-energy properties of the localized spins near the transition
are dominated by anomalous ordered (disordered) regions of localized spins
which survive into the paramagnetic (ferromagnetic) phase. Many interesting
properties follow, including a diverging susceptibility for a finite range of
couplings into the paramagnetic phase. Our critical line equation, together
with numerically determined transition points, are used to determine the range
of the double-exchange interaction. Models we consider are the spin 1/2 Kondo
lattices with antiferromagnetic (Kondo) coupling, with ferromagnetic (Hund's
rule) coupling, and the Kondo lattice with repulsive interactions between the
conduction electrons.Comment: 18 pages, 6 embedded eps figures. To appear in Phys Rev
Tunneling and rattling in clathrate crystal
We present tunneling and rattling motions of an off-center guest atom in cage
referring to a clathrate crystal La_3Pd_{20}Ge_6. The elastic constant C_{44}
of La_3Pd_{20}Ge_6 shows a Debye-type dispersion around 20 K obeying a
relaxation time tau = tau_0exp(E/k_{B}T) with an attempt time tau_0 =
2.0*10^{-12} sec and an activation energy E = 197 K. At low temperatures below
3 K down to 20 mK, the C_{44} shows a softening of C_{44} =
C_{44}^0(T-T_C^0)/(T-Theta) with T_C^0 = -337.970 mK and Theta = -338.044 mK.
These facts are attributed to two different types of the off-center motions
with Gamma_5 symmetry in 4a-site cage of La_3Pd_{20}Ge_6, a thermally activated
rattling motion over the potential hill and a tunneling motion through the
potential hill at low temperatures.Comment: 5 pages, 4 figures, to be published Phys. Rev.
Phase transition in the one-dimensional Kondo lattice model with attractive electron-electron interaction
The one-dimensional Kondo lattice model with attractive interaction among the
conduction electrons is analyzed in the case of half-filling. It is shown that
there are three distinct phases depending on the coupling constants of the
model. Two phases have a spin and charge gap. While one shows a clear
separation of the spin and charge excitation spectrum the other phase may be
characterized as a band insulator type where both excitations are due to
two-particle states. The third phase is gapless in both channels and has quasi
long-range order in the spin and charge density wave correlation. In this phase
the spin and charge excitations have again a clearly separated spectrum. For
the analysis we discuss first two limiting cases. Then a density matrix
renormalization group calculation on finite systems is applied to determine the
phase diagram and the correlation functions in the gapped and gapless phase for
general couplding constants.Comment: 9 pages, 7 Postscript figures, REVTe
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