Quantum integrability and nonintegrability in the spin-boson model

We study the spectral properties of a spin-boson Hamiltonian that depends on two continuous parameters $0\leq\Lambda<\infty$ (interaction strength) and $0\leq\alpha\leq\pi/2$ (integrability switch). In the classical limit this system has two distinct integrable regimes, $\alpha=0$ and $\alpha=\pi/2$. For each integrable regime we can express the quantum Hamiltonian as a function of two action operators. Their eigenvalues (multiples of $\hbar$) are the natural quantum numbers for the complete level spectrum. This functional dependence cannot be extended into the nonintegrable regime $(0<\alpha<\pi/2)$. Here level crossings are prohibited and the level spectrum is naturally described by a single (energy sorting) quantum number. In consequence, the tracking of individual eigenstates along closed paths through both regimes leads to conflicting assignments of quantum numbers. This effect is a useful and reliable indicator of quantum chaos -- a diagnostic tool that is independent of any level-statistical analysis

Writing electronic ferromagnetic states in a high-temperature paramagnetic nuclear spin system

In this paper we use the Nuclear Magnetic Resonance (NMR) to write eletronic states of a ferromagnetic system into a high-temperature paramagnetic nuclear spins. Through the control of phase and duration of radiofrequency pulses we set the NMR density matrix populations, and apply the technique of quantum state tomography to experimentally obtain the matrix elements of the system, from which we calculate the temperature dependence of magnetization for different magnetic fields. The effects of the variation of temperature and magnetic field over the populations can be mapped in the angles of spins rotations, carried out by the RF pulses. The experimental results are compared to the Brillouin functions of ferromagnetic ordered systems in the mean field approximation for two cases: the mean field is given by (i) $B=B_0+\lambda M$ and (ii) $B=B_0+\lambda M + \lambda^\prime M^3$, where $B_0$ is the external magnetic field, and $\lambda, \lambda^\prime$ are mean field parameters. The first case exhibits second order transition, whereas the second case has first order transition with temperature hysteresis. The NMR simulations are in good agreement with the magnetic predictions

Dynamic properties of quantum spin chains: Simple route to complex behavior

We examine dynamic structure factors of spin-1/2 chains with nearest-neighbor interactions of XX and Dzyaloshinskii-Moriya type, and with periodic and random changes in the sign of these interactions. This special kind of inhomogeneity can be eliminated from the Hamiltonian by suitable transformation of the spin variables. As a result, the dynamic structure factors of periodic or random chains can be computed from those of the uniform chains. Using the exact analytical and precise numerical results available for the uniform systems we illustrate the effects of regular alternation or random disorder on dynamic structure factors of quantum spin chains

VI3 - a new layered ferromagnetic semiconductor

Two-dimensional (2D) materials are promising candidates for next-generation electronic devices. In this regime, insulating 2D ferromagnets, which remain rare, are of special importance due to their potential for enabling new device architectures. Here we report the discovery of ferromagnetism in a layered van der Waals semiconductor, VI3, which is based on honeycomb vanadium layers separated by an iodine-iodine van der Waals gap. It has a BiI3-type structure (R-3, No.148) at room temperature, and our experimental evidence suggests that it may undergo a subtle structural phase transition at 78 K. VI3 becomes ferromagnetic at 49 K, below which magneto-optical Kerr effect imaging clearly shows ferromagnetic domains, which can be manipulated by the applied external magnetic field. The optical band gap determined by reflectance measurements is 0.6 eV, and the material is highly resistive

Charge and spin dynamics in the one-dimensional t−Jzt-J_z and t−Jt-J models

The impact of the spin-flip terms on the (static and dynamic) charge and spin correlations in the Luttinger-liquid ground state of the 1D $t-J$ model is assessed by comparison with the same quantities in the 1D $t-J_z$ model, where spin-flip terms are absent. We employ the recursion method combined with a weak-coupling or a strong-coupling continued-fraction analysis. At $J_z/t=0^+$ we use the Pfaffian representation of dynamic spin correlations. The changing nature of the dynamically relevant charge and spin excitations on approach of the transition to phase separation is investigated in detail. The $t-J_z$ charge excitations (but not the spin excitations) at the transition have a single-mode nature, whereas charge and spin excitations have a complicated structure in the $t-J$ model. In the $t-J_z$ model, phase separation is accompanied by N\'eel long-range order, caused by the condensation of electron clusters with an already existing alternating up-down spin configuration (topological long-range order). In the $t-J$ model, by contrast, the spin-flip processes in the exchange coupling are responsible for continued strong spin fluctuations (dominated by 2-spinon excitations) in the phase-separated state.Comment: 11 pages (RevTex). 14 Figures available from author

Dynamics of spin correlations in the spin-1/2 isotropic XY chain in a transverse field

Dynamic xx spin pair correlation functions for the isotropic spin-1/2 XY chain are calculated numerically for long open chains in the presence of a transverse magnetic field at finite temperature. As an application we discuss the temperature dependence of the spin-spin relaxation time in PrCl_3.Comment: 2 pages, latex, 2 figures, abstract of the paper presented at Ampere Summer School ``Applications of Magnetic Resonance in Novel Materials'' Nafplion, Greece, 3-9 September, 2000, partially published in J. Phys. A: Math. Gen. 33, 3063 (2000

Random antiferromagnetic quantum spin chains: Exact results from scaling of rare regions

We study XY and dimerized XX spin-1/2 chains with random exchange couplings by analytical and numerical methods and scaling considerations. We extend previous investigations to dynamical properties, to surface quantities and operator profiles, and give a detailed analysis of the Griffiths phase. We present a phenomenological scaling theory of average quantities based on the scaling properties of rare regions, in which the distribution of the couplings follows a surviving random walk character. Using this theory we have obtained the complete set of critical decay exponents of the random XY and XX models, both in the volume and at the surface. The scaling results are confronted with numerical calculations based on a mapping to free fermions, which then lead to an exact correspondence with directed walks. The numerically calculated critical operator profiles on large finite systems (L<=512) are found to follow conformal predictions with the decay exponents of the phenomenological scaling theory. Dynamical correlations in the critical state are in average logarithmically slow and their distribution show multi-scaling character. In the Griffiths phase, which is an extended part of the off-critical region average autocorrelations have a power-law form with a non-universal decay exponent, which is analytically calculated. We note on extensions of our work to the random antiferromagnetic XXZ chain and to higher dimensions.Comment: 19 pages RevTeX, eps-figures include