3,081 research outputs found
Kondo-like behaviors in magnetic and thermal properties of single crystal Tm5Si2Ge2
We grew the single crystal of stoichiometric Tm5Si2.0Ge2.0 using a Bridgeman
method and performed XRD, EDS, magnetization, ac and dc magnetic
susceptibilities, specific heat, electrical resistivity and XPS experiments. It
crystallizes in orthorhombic Sm5Ge4-type structure. The mean valence of Tm ions
in Tm5Si2.0Ge2.0 is almost trivalent. The 4f states is split by the crystalline
electric field. The ground state exhibits the long range antiferromagnetic
order with the ferromagnetically coupled magnetic moments in the ac plane below
8.01 K, while the exited states exhibit the reduction of magnetic moment and
magnetic entropy and -log T-behaviors observed in Kondo materials.Comment: 8 pages, 13 figure
Comparative Analysis of Non-thermal Emissions and Study of Electron Transport in a Solar Flare
We study the non-thermal emissions in a solar flare occurring on 2003 May 29
by using RHESSI hard X-ray (HXR) and Nobeyama microwave observations. This
flare shows several typical behaviors of the HXR and microwave emissions: time
delay of microwave peaks relative to HXR peaks, loop-top microwave and
footpoint HXR sources, and a harder electron energy distribution inferred from
the microwave spectrum than from the HXR spectrum. In addition, we found that
the time profile of the spectral index of the higher-energy (\gsim 100 keV)
HXRs is similar to that of the microwaves, and is delayed from that of the
lower-energy (\lsim 100 keV) HXRs. We interpret these observations in terms
of an electron transport model called {\TPP}. We numerically solved the
spatially-homogeneous {\FP} equation to determine electron evolution in energy
and pitch-angle space. By comparing the behaviors of the HXR and microwave
emissions predicted by the model with the observations, we discuss the
pitch-angle distribution of the electrons injected into the flare site. We
found that the observed spectral variations can qualitatively be explained if
the injected electrons have a pitch-angle distribution concentrated
perpendicular to the magnetic field lines rather than isotropic distribution.Comment: 32 pages, 12 figures, accepted for publication in The Astronomical
Journa
Nature of the insulating phases in the half-filled ionic Hubbard model
We investigate the ground-state phase diagram of the one-dimensional "ionic"
Hubbard model with an alternating periodic potential at half-filling by
numerical diagonalization of finite systems with the Lanczos and density matrix
renormalization group (DMRG) methods. We identify an insulator-insulator phase
transition from a band to a correlated insulator with simultaneous charge and
bond-charge order. The transition point is characterized by the vanishing of
the optical excitation gap while simultaneously the charge and spin gaps remain
finite and equal. Indications for a possible second transition into a
Mott-insulator phase are discussed.Comment: final for
Development of biomimetic catalytic oxidation methods and non-salt methods using transition metal-based acid and base ambiphilic catalysts
This review focuses on the development of ruthenium and flavin catalysts for environmentally benign oxidation reactions based on mimicking the functions of cytochrome P-450 and flavoenzymes, and low valent transition-metal catalysts that replace conventional acids and bases. Several new concepts and new types of catalytic reactions based on these concepts are described
Crossover from Kondo assisted suppression to co-tunneling enhancement of tunneling magnetoresistance via ferromagnetic nanodots in MgO tunnel barriers
Recently, it has been shown that magnetic tunnel junctions with thin MgO
tunnel barriers exhibit extraordinarily high tunneling magnetoresistance (TMR)
values at room temperature1, 2. However, the physics of spin dependent
tunneling through MgO barriers is only beginning to be unravelled. Using planar
magnetic tunnel junctions in which ultra-thin layers of magnetic metals are
deposited in the middle of a MgO tunnel barrier here we demonstrate that the
TMR is strongly modified when these layers are discontinuous and composed of
small pancake shaped nanodots. At low temperatures, in the Coulomb blockade
regime, for layers less than ~1 nm thick, the conductance of the junction is
increased at low bias consistent with Kondo assisted tunneling. In the same
regime we observe a suppression of the TMR. For slightly thicker layers, and
correspondingly larger nanodots, the TMR is enhanced at low bias, consistent
with co-tunneling.Comment: Nano Letters (in press
Excitation Spectrum of One-dimensional Extended Ionic Hubbard Model
We use Perturbative Continuous Unitary Transformations (PCUT) to study the
one dimensional Extended Ionic Hubbard Model (EIHM) at half-filling in the band
insulator region. The extended ionic Hubbard model, in addition to the usual
ionic Hubbard model, includes an inter-site nearest-neighbor (n.n.) repulsion,
. We consider the ionic potential as unperturbed part of the Hamiltonian,
while the hopping and interaction (quartic) terms are treated as perturbation.
We calculate total energy and ionicity in the ground state. Above the ground
state, (i) we calculate the single particle excitation spectrum by adding an
electron or a hole to the system. (ii) the coherence-length and spectrum of
electron-hole excitation are obtained. Our calculations reveal that for V=0,
there are two triplet bound state modes and three singlet modes, two anti-bound
states and one bound state, while for finite values of there are four
excitonic bound states corresponding to two singlet and two triplet modes. The
major role of on-site Coulomb repulsion is to split singlet and triplet
collective excitation branches, while tends to pull the singlet branches
below the continuum to make them bound states.Comment: 10 eps figure
Quantum Size Effect transition in percolating nanocomposite films
We report on unique electronic properties in Fe-SiO2 nanocomposite thin films
in the vicinity of the percolation threshold. The electronic transport is
dominated by quantum corrections to the metallic conduction of the Infinite
Cluster (IC). At low temperature, mesoscopic effects revealed on the
conductivity, Hall effect experiments and low frequency electrical noise
(random telegraph noise and 1/f noise) strongly support the existence of a
temperature-induced Quantum Size Effect (QSE) transition in the metallic
conduction path. Below a critical temperature related to the geometrical
constriction sizes of the IC, the electronic conductivity is mainly governed by
active tunnel conductance across barriers in the metallic network. The high 1/f
noise level and the random telegraph noise are consistently explained by random
potential modulation of the barriers transmittance due to local Coulomb
charges. Our results provide evidence that a lowering of the temperature is
somehow equivalent to a decrease of the metal fraction in the vicinity of the
percolation limit.Comment: 21 pages, 8 figure
Why male orangutans do not kill infants
Infanticide is widespread among mammals, is particularly common in primates, and has been shown to be an adaptive male strategy under certain conditions. Although no infanticides in wild orangutans have been reported to date, several authors have suggested that infanticide has been an important selection pressure influencing orangutan behavior and the evolution of orangutan social systems. In this paper, we critically assess this suggestion. We begin by investigating whether wild orangutans have been studied for a sufficiently long period that we might reasonably expect to have detected infanticide if it occurs. We consider whether orangutan females exhibit counterstrategies typically employed by other mammalian females. We also assess the hypothesis that orangutan females form special bonds with particular “protector males” to guard against infanticide. Lastly, we discuss socioecological reasons why orangutan males may not benefit from infanticide. We conclude that there is limited evidence for female counterstrategies and little support for the protector male hypothesis. Aspects of orangutan paternity certainty, lactational amenorrhea, and ranging behavior may explain why infanticide is not a strategy regularly employed by orangutan males on Sumatra or Borneo
An event of extreme relativistic and ultra-relativistic electron enhancements following the arrival of consecutive corotating interaction regions: coordinated observations by Van Allen Probes, Arase, THEMIS and Galileo satellites
[During July to October of 2019, a sequence of isolated Corotating Interaction Regions (CIRs) impacted the magnetosphere, for four consecutive solar rotations, without any interposed Interplanetary Coronal Mass Ejections. Even though the series of CIRs resulted in relatively weak geomagnetic storms, the net effect of the outer radiation belt during each disturbance was different, depending on the electron energy. During the August-September CIR group, significant multi-MeV electron enhancements occurred, up to ultra-relativistic energies of 9.9 MeV in the heart of the outer Van Allen radiation belt. These characteristics deemed this time period a fine case for studying the different electron acceleration mechanisms. In order to do this, we exploited coordinated data from the Van Allen Probes, the Time History of Events and Macroscale Interactions during Substorms Mission (THEMIS), Arase and Galileo satellites, covering seed, relativistic and ultra-relativistic electron populations, investigating their Phase Space Density (PSD) profile dependence on the values of the second adiabatic invariant K, ranging from near-equatorial to off equatorial mirroring populations. Our results indicate that different acceleration mechanisms took place for different electron energies. The PSD profiles were dependent not only on the μ value, but also on the K value, with higher K values corresponding to more pronounced local acceleration by chorus waves. The 9.9 MeV electrons were enhanced prior to the 7.7 MeV, indicating that different mechanisms took effect on different populations. Finally, all ultra-relativistic enhancements took place below geosynchronous orbit, emphasizing the need for more Medium Earth Orbit (MEO) missions.]80NSSC19K0845 - NASAPublished versio
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