Photothermal effects in ultra-precisely stabilized tunable microcavities

We study the mechanical stability of a tunable high-finesse microcavity under ambient conditions and investigate light-induced effects that can both suppress and excite mechanical fluctuations. As an enabling step, we demonstrate the ultra-precise electronic stabilization of a microcavity. We then show that photothermal mirror expansion can provide high-bandwidth feedback and improve cavity stability by almost two orders of magnitude. At high intracavity power, we observe self-oscillations of mechanical resonances of the cavity. We explain the observations by a dynamic photothermal instability, leading to parametric driving of mechanical motion. For an optimized combination of electronic and photothermal stabilization, we achieve a feedback bandwidth of $500\,$kHz and a noise level of $1.1 \times 10^{-13}\,$m rms

Cavity-enhanced Raman Microscopy of Individual Carbon Nanotubes

Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement of Raman scattering in a tunable high-finesse microcavity, and utilize it for molecular diagnostics by combined Raman and absorption imaging. Studying individual single-wall carbon nanotubes, we identify crucial structural parameters such as nanotube radius, electronic structure and extinction cross-section. We observe a 320-times enhanced Raman scattering spectral density and an effective Purcell factor of 6.2, together with a collection efficiency of 60%. Potential for significantly higher enhancement, quantitative signals, inherent spectral filtering and absence of intrinsic background in cavity-vacuum stimulated Raman scattering render the technique a promising tool for molecular imaging. Furthermore, cavity-enhanced Raman transitions involving localized excitons could potentially be used for gaining quantum control over nanomechanical motion and open a route for molecular cavity optomechanics

Cavity-enhanced optical detection of carbon nanotube Brownian motion

Optical cavities with small mode volume are well-suited to detect the vibration of sub-wavelength sized objects. Here we employ a fiber-based, high-finesse optical microcavity to detect the Brownian motion of a freely suspended carbon nanotube at room temperature under vacuum. The optical detection resolves deflections of the oscillating tube down to 50pm/Hz^1/2. A full vibrational spectrum of the carbon nanotube is obtained and confirmed by characterization of the same device in a scanning electron microscope. Our work successfully extends the principles of high-sensitivity optomechanical detection to molecular scale nanomechanical systems.Comment: 14 pages, 11 figure

On the nature of the fast moving star S2 in the Galactic Center

We analyze the properties of the star S2 orbiting the supermassive black hole at the center of the Galaxy. A high quality SINFONI H and K band spectrum obtained from coadding 23.5 hours of observation between 2004 and 2007 reveals that S2 is an early B dwarf (B0-2.5V). Using model atmospheres, we constrain its stellar and wind properties. We show that S2 is a genuine massive star, and not the core of a stripped giant star as sometimes speculated to resolve the problem of star formation so close to the supermassive black hole. We give an upper limit on its mass loss rate, and show that it is He enriched, possibly because of the presence of a magnetic field.Comment: 4 pages, 5 figures, ApJ letters accepte

On the origin of the extremely different solubilities of polyethers in water

The solubilities of polyethers are surprisingly counter-intuitive. The best-known example is the difference between polyethylene glycol ([–CH2–CH2–O–]n) which is infinitely soluble, and polyoxymethylene ([–CH2–O–]n) which is completely insoluble in water, exactly the opposite of what one expects from the C/O ratios of these molecules. Similar anomalies exist for oligomeric and cyclic polyethers. To solve this apparent mystery, we use femtosecond vibrational and GHz dielectric spectroscopy with complementary ab initio calculations and molecular dynamics simulations. We find that the dynamics of water molecules solvating polyethers is fundamentally different depending on their C/O composition. The ab initio calculations and simulations show that this is not because of steric effects (as is commonly believed), but because the partial charge on the O atoms depends on the number of C atoms by which they are separated. Our results thus show that inductive effects can have a major impact on aqueous solubilities

Self-localization of magnon Bose-Einstein condensates in the ground state and on excited levels: from harmonic to box-like trapping potential

Long-lived coherent spin precession of 3He-B at low temperatures around 0.2 Tc is a manifestation of Bose-Einstein condensation of spin-wave excitations or magnons in a magnetic trap which is formed by the order-parameter texture and can be manipulated experimentally. When the number of magnons increases, the orbital texture reorients under the influence of the spin-orbit interaction and the profile of the trap gradually changes from harmonic to a square well, with walls almost impenetrable to magnons. This is the first experimental example of Bose condensation in a box. By selective rf pumping the trap can be populated with a ground-state condensate or one at any of the excited energy levels. In the latter case the ground state is simultaneously populated by relaxation from the exited level, forming a system of two coexisting condensates.Comment: 4 pages, 5 figure