Ultrafast helicity control of surface currents in topological insulators with near-unity fidelity

In recent years, a class of solid state materials, called three-dimensional topological insulators, has emerged. In the bulk, a topological insulator behaves like an ordinary insulator with a band gap. At the surface, conducting gapless states exist showing remarkable properties such as helical Dirac dispersion and suppression of backscattering of spin-polarized charge carriers. The characterization and control of the surface states via transport experiments is often hindered by residual bulk contributions yet at cryogenic temperatures. Here, we show that surface currents in Bi2Se3 can be controlled by circularly polarized light on a picosecond time scale with a fidelity near unity even at room temperature. We re-veal the temporal separation of such ultrafast helicity-dependent surface currents from photo-induced thermoelectric and drift currents in the bulk. Our results uncover the functionality of ultrafast optoelectronic devices based on surface currents in topological insulators.Comment: 19 pages, 4 figures, supplementary informatio

Covalently Binding the Photosystem I to Carbon Nanotubes

We present a chemical route to covalently couple the photosystem I (PS I) to carbon nanotubes (CNTs). Small linker molecules are used to connect the PS I to the CNTs. Hybrid systems, consisting of CNTs and the PS I, promise new photo-induced transport phenomena due to the outstanding optoelectronic properties of the robust cyanobacteria membrane protein PS I

Optoelectronic sensitization of carbon nanotubes by CdTe nanocrystals

We investigate the photoconductance of single-walled carbon nanotube-nanocrystal hybrids. The nanocrystals are bound to the nanotubes via molecular recognition. We find that the photoconductance of the hybrids can be adjusted by the absorption characteristics of the nanocrystals. In addition, the photoconductance of the hybrids surprisingly exhibits a slow time constant of about 1 ms after excitation of the nanocrystals. The data are consistent with a bolometrically induced current increase in the nanotubes caused by photon absorption in the nanocrystals

Dicke effect in a quantum wire with side-coupled quantum dots

A system of an array of side-coupled quantum-dots attached to a quantum wire is studied theoretically. Transport through the quantum wire is investigated by means of a noninteracting Anderson tunneling Hamiltonian. Analytical expressions of the transmission probability and phase are given. The transmission probability shows an energy spectrum with forbidden and allowed bands that depends on the up-down asymmetry of the system. In up-down symmetry only the gap survives, and in up-down asymmetry an allowed band is formed. We show that the allowed band arises by the indirect coupling between the up and down quantum dots. In addition, the band edges can be controlled by the degree of asymmetry of the quantum dots. We discuss the analogy between this phenomenon with the Dicke effect in optics.Comment: 11 pages, 5 figures. To appear in Physica