Combined scanning force microscopy and scanning tunneling spectroscopy of an electronic nano-circuit at very low temperature

We demonstrate the combination of scanning force microscopy and scanning tunneling spectroscopy in a local probe microscope operating at very low temperature (60 mK). This local probe uses a quartz tuning fork ensuring high tunnel junction stability. We performed the spatially-resolved spectroscopic study of a superconducting nano-circuit patterned on an insulating substrate. Significant deviations from the BCS prediction are observed.Comment: 4 page

Josephson Coupling in the Dissipative State of a Thermally Hysteretic μ\mu-SQUID

Micron-sized superconducting interference devices ($\mu$-SQUIDs) based on constrictions optimized for minimizing thermal runaway are shown to exhibit voltage oscillations with applied magnetic flux despite their hysteretic behavior. We explain this remarkable feature by a significant supercurrent contribution surviving deep into the resistive state, due to efficient heat evacuation. A resistively shunted junction model, complemented by a thermal balance determining the amplitude of the critical current, describes well all experimental observations, including the flux modulation of the (dynamic) retrapping current and voltage by introducing a single dimensionless parameter. Thus hysteretic $\mu$-SQUIDs can be operated in the voltage read-out mode with a faster response. The quantitative modeling of this regime incorporating both heating and phase dynamics paves the way for further optimization of $\mu$-SQUIDs for nano-magnetism.Comment: 10 pages, 11 figures, Revise

A subKelvin scanning probe microscope for the electronic spectroscopy of an individual nano-device

We present a combined scanning force and tunneling microscope working in a dilution refrigerator that is optimized for the study of individual electronic nano-devices. This apparatus is equipped with commercial piezo-electric positioners enabling the displacement of a sample below the probe over several hundred microns at very low temperature, without excessive heating. Atomic force microscopy based on a tuning fork resonator probe is used for cryogenic precise alignment of the tip with an individual device. We demonstrate the local tunneling spectroscopy of a hybrid Josephson junction as a function of its current bias

Spatially-Correlated Microstructure and Superconductivity in Polycrystalline Boron-Doped Diamond

Scanning tunneling spectroscopies are performed below 100~mK on nano-crystalline boron-doped diamond films characterized by Transmission Electron Microscopy and transport measurements. We demonstrate a strong correlation between the local superconductivity strength and the granular structure of the films. The study of the spectral shape, amplitude and temperature dependence of the superconductivity gap enables us to differentiate intrinsically superconducting grains that follow the BCS model, from grains showing a different behavior involving the superconducting proximity effect

Sub-Gap Structure in the Conductance of a Three-Terminal Josephson Junction

Three-terminal superconductor (S) - normal metal (N) - superconductor (S) Josephson junctions are investigated. In a geometry where a T-shape normal metal is connected to three superconducting reservoirs, new sub-gap structures appear in the differential resistance for specific combinations of the superconductor chemical potentials. Those correspond to a correlated motion of Cooper pairs within the device that persist well above the Thouless energy and is consistent with the prediction of quartets formed by two entangled Cooper pairs. A simplified nonequilibrium Keldysh Green's function calculation is presented that supports this interpretation.Comment: To appear in Physical Review

Modulating charge density and inelastic optical response in graphene by atmospheric pressure localized intercalation through wrinkles

The intercalation of an oxide barrier between graphene and its metallic substrate for chem- ical vapor deposition is a contamination-free alternative to the transfer of graphene to dielectric supports, usually needed for the realization of electronic devices. Low-cost pro- cesses, especially at atmospheric pressure, are desirable but whether they are achievable remains an open question. Combining complementary microscopic analysis, providing structural, electronic, vibrational, and chemical information, we demonstrate the spontaneous reactive intercalation of 1.5 nm-thick oxide ribbons between graphene and an iridium substrate, at atmospheric pressure and room temperature. We discover that oxygen-containing molecules needed for forming the ribbons are supplied through the graphene wrinkles, which act as tunnels for the efficient diffusion of molecules entering their free end. The intercalated oxide ribbons are found to modify the graphene-support interaction, leading to the formation of quasi-free-standing high quality graphene whose charge density is modulated in few 10-100 nm-wide ribbons by a few 10^12 cm-2, where the inelastic optical response is changed, due to a softening of vibrational modes - red-shifts of Raman G and 2D bands by 6 and 10 cm-1, respectively.Comment: Carbon (2013) available onlin

Hybrid superconducting nanostructures: very low temperature local probing and noise

International audienceWe review the topic of hybrid superconducting nanostructures by introducing the basic physical concepts and describing recent key experimental results. We discuss the superconductivity nucleation in mesoscopic structures, the vortex lattice imaging in doped diamond films, the superconducting proximity effect, multiple Andreev reflection in Josephson junctions and the electronic micro-cooling in hybrid tunnel junctions. An emphasis is put on very low temperature local probes and noise measurement techniques developed in Grenoble

Quasiparticle diffusion based heating in superconductor tunneling micro-coolers

In a hybrid Superconductor - Insulator - Normal metal tunnel junction biased just below the gap, the extraction of hot electrons out of the normal metal results in electronic cooling effect. The quasiparticles injected in the superconductor accumulate near the tunnel interface, thus increasing the effective superconductor temperature. We propose a simple model for the diffusion of excess quasiparticles in a superconducting strip with an additional trap junction. This diffusion model has a complete analytic solution, which depends on experimentally accessible parameters. We find that the accumulated quasiparticles near the junction reduce the efficiency of the device. This study is also relevant to more general situations making use of superconducting tunnel junctions, as low temperature detectors.Comment: 4 pages, 3 figure

Superconducting cascade electron refrigerator

The design and operation of an electronic cooler based on a combination of superconducting tunnel junctions is described. The cascade extraction of hot-quasiparticles, which stems from the energy gaps of two different superconductors, allows for a normal metal to be cooled down to about 100 mK starting from a bath temperature of 0.5 K. We discuss the practical implementation, potential performance and limitations of such a device

Etching suspended superconducting hybrid junctions from a multilayer

A novel method to fabricate large-area superconducting hybrid tunnel junctions with a suspended central normal metal part is presented. The samples are fabricated by combining photo-lithography and chemical etch of a superconductor - insulator - normal metal multilayer. The process involves few fabrication steps, is reliable and produces extremely high-quality tunnel junctions. Under an appropriate voltage bias, a significant electronic cooling is demonstrated