A Single Atom as a Mirror of an Optical Cavity

By tightly focussing a laser field onto a single cold ion trapped in front of a far-distant dielectric mirror, we could observe a quantum electrodynamic effect whereby the ion behaves as the optical mirror of a Fabry-P\'erot cavity. We show that the amplitude of the laser field is significantly altered due to a modification of the electromagnetic mode structure around the atom in a novel regime in which the laser intensity is already changed by the atom alone. e propose a direct application of this system as a quantum memory for single photons.Comment: 7 pages, 3 figures, to appear in Physical Review Letter

Infrared spectroscopic studies on unoriented single-walled carbon nanotube films under hydrostatic pressure

The electronic properties of as-prepared and purified unoriented single-walled carbon nanotube films were studied by transmission measurements over a broad frequency range (far-infrared up to visible) as a function of temperature (15 K - 295 K) and external pressure (up to 8 GPa). Both the as-prepared and the purified SWCNT films exhibit nearly temperature-independent properties. With increasing pressure the low-energy absorbance decreases suggesting an increasing carrier localization due to pressure-induced deformations. The energy of the optical transitions in the SWCNTs decreases with increasing pressure, which can be attributed to pressure-induced hybridization and symmetry-breaking effects. We find an anomaly in the pressure-induced shift of the optical transitions at $\sim$2 GPa due to a structural phase transition.Comment: 13 pages, 15 figure

Vacuum-Stimulated Raman Scattering based on Adiabatic Passage in a High-Finesse Optical Cavity

We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by means of an adiabatic passage technique based on a counter-intuitive interaction sequence between pump laser and cavity field. This photon leaves the cavity through the less-reflecting mirror. The emission rate shows a characteristic dependence on the cavity and pump detuning, and the observed spectra have a sub-natural linewidth. The results are in excellent agreement with numerical simulations.Comment: 4 pages, 5 figure

Quantum Beat of Two Single Photons

The interference of two single photons impinging on a beam splitter is measured in a time-resolved manner. Using long photons of different frequencies emitted from an atom-cavity system, a quantum beat with a visibility close to 100% is observed in the correlation between the photodetections at the output ports of the beam splitter. The time dependence of the beat amplitude reflects the coherence properties of the photons. Most remarkably, simultaneous photodetections are never observed, so that a temporal filter allows one to obtain perfect two-photon coalescence even for non-perfect photons.Comment: 4 pages, 3 figure

QED with a spherical mirror

We investigate the Quantum-Electro-Dynamic properties of an atomic electron close to the focus of a spherical mirror. We first show that the spontaneous emission and excited state level shift of the atom can be fully suppressed with mirror-atom distances of many wavelengths. A three-dimensional theory predicts that the spectral density of vacuum fluctuations can indeed vanish within a volume $\lambda^3$ around the atom, with the use of a far distant mirror covering only half of the atomic emission solid angle. The modification of these QED atomic properties is also computed as a function of the mirror size and large effects are found for only moderate numerical apertures. We also evaluate the long distance ground state energy shift (Casimir-Polder shift) and find that it scales as $(\lambda/R)^2$ at the focus of a hemi-spherical mirror of radius $R$, as opposed to the well known $(\lambda/R)^4$ scaling law for an atom at a distance $R$ from an infinite plane mirror. Our results are relevant for investigations of QED effects, and also free space coupling to single atoms using high-numerical aperture lenses.Comment: 12 pages, 4 figure