465 research outputs found
ab initio frame transformation calculations of direct and indirect dissociative recombination rates of HeH+ + e-
The HeH cation undergoes dissociative recombination with a free electron
to produce neutral He and H fragments. We present calculations using ab initio
quantum defects and Fano's rovibrational frame transformation technique, along
with the methodology of PRL 89, 263003 (2002), to obtain the recombination rate
both in the low-energy (1-300 meV) and high-energy (ca. 0.6 hartree) regions.
We obtain very good agreement with experimental results, demonstrating that
this relatively simple method is able to reproduce observed rates for both
indirect dissociative recombination, driven by rovibrationally autoionizing
states in the low-energy region, and direct dissociative recombination, driven
by electronically autoionizing Rydberg states attached to higher-energy excited
cation channels.Comment: Submitted to Phys Rev
Estimates of rates for dissociative recombination of NO + e via various mechanisms
We estimate rates for the dissociative recombination (DR) of NO +
e. Although accurate excited state potential energy curves for the excited
states of the neutral are not available, we estimate that the 1 {\Phi}
and the 1 {\Pi} states of the neutral may intersect the ground state
cation potential energy surface near its equilibrium geometry. Using fixed
nuclei scattering calculations we estimate the rate for direct DR via these
states and find it to be significant. We also perform approximate calculations
of DR triggered by the indirect mechanism, which suggest that the indirect DR
rate for NO is insignificant compared to the direct rate.Comment: Submitted to Phys Rev
Dissociative electron attachment to the H2O molecule. II. Nuclear dynamics on coupled electronic surfaces within the local complex potential model
We report the results of a first-principles study of dissociative electron
attachment to H2O. The cross sections are obtained from nuclear dynamics
calculations carried out in full dimensionality within the local complex
potential model by using the multi-configuration time-dependent Hartree method.
The calculations employ our previously obtained global, complex-valued,
potential-energy surfaces for the three (doublet B1, doublet A1, and doublet
B2) electronic Feshbach resonances involved in this process. These three
metastable states of H2O- undergo several degeneracies, and we incorporate both
the Renner-Teller coupling between the B1 and A1 states as well as the conical
intersection between the A1 and B2 states into our treatment. The nuclear
dynamics are inherently multidimensional and involve branching between
different final product arrangements as well as extensive excitation of the
diatomic fragment. Our results successfully mirror the qualitative features of
the major fragment channels observed, but are less successful in reproducing
the available results for some of the minor channels. We comment on the
applicability of the local complex potential model to such a complicated
resonant system.Comment: Corrected version of Phys Rev A 75, 012711 (2007
Beyond the Shell Model: The Canonical Nuclear Many-Body Problem as an Effective Theory
We describe a strategy for attacking the canonical nuclear structure problem
---bound-state properties of a system of point nucleons interacting via a
two-body potential---which involves an expansion in the number of particles
scattering at high momenta, but is otherwise exact. The required
self-consistent solutions of the Bloch-Horowitz equation for effective
interactions and operators are obtained by an efficient Green's function method
based on the Lanczos algorithm. We carry out this program for the simplest
nuclei, d and He, to contrast a rigorous effective theory with the shell
model, thereby illustrating several of the uncontrolled approximations in the
latter.Comment: Revtex; two columns; four pages; two figures; submitted to Phys. Rev.
Let
Perturbative Effective Theory in an Oscillator Basis?
The effective interaction/operator problem in nuclear physics is believed to
be highly nonperturbative, requiring extended high-momentum spaces for accurate
solution. We trace this to difficulties that arise at both short and long
distances when the included space is defined in terms of a basis of harmonic
oscillator Slater determinants. We show, in the simplest case of the deuteron,
that both difficulties can be circumvented, yielding highly perturbative
results in the potential even for modest (~6hw) included spaces.Comment: 10 pages, 4 figure
Nuclear Anapole Moments
Nuclear anapole moments are parity-odd, time-reversal-even E1 moments of the
electromagnetic current operator. Although the existence of this moment was
recognized theoretically soon after the discovery of parity nonconservation
(PNC), its experimental isolation was achieved only recently, when a new level
of precision was reached in a measurement of the hyperfine dependence of atomic
PNC in 133Cs. An important anapole moment bound in 205Tl also exists. In this
paper, we present the details of the first calculation of these anapole moments
in the framework commonly used in other studies of hadronic PNC, a meson
exchange potential that includes long-range pion exchange and enough degrees of
freedom to describe the five independent amplitudes induced by
short-range interactions. The resulting contributions of pi-, rho-, and
omega-exchange to the single-nucleon anapole moment, to parity admixtures in
the nuclear ground state, and to PNC exchange currents are evaluated, using
configuration-mixed shell-model wave functions. The experimental anapole moment
constraints on the PNC meson-nucleon coupling constants are derived and
compared with those from other tests of the hadronic weak interaction. While
the bounds obtained from the anapole moment results are consistent with the
broad ``reasonable ranges'' defined by theory, they are not in good agreement
with the constraints from the other experiments. We explore possible
explanations for the discrepancy and comment on the potential importance of new
experiments.Comment: 53 pages; 10 figures; revtex; submitted to Phys Rev
Nuclear electron capture rate in stellar interiors and the case of 7Be
Nuclear electron capture rate from continuum in an astrophysical plasma
environment (like solar core) is calculated using a modified Debye-Huckel
screening potential and the related non-Gaussian q-distribution of electron
momenta. For q=1 the well-known Debye-Huckel results are recovered. The value
of q can be derived from the fluctuation of number of particles and temperature
inside the Debye sphere. For 7Be continuum electron capture in solar core, we
find an increase of 7 -- 10 percent over the rate calculated with standard
Debye-Huckel potential. The consequence of this results is a reduction of the
same percentage of the SSM 8B solar neutrino flux, leaving unchanged the SSM
7Be flux.Comment: 8 pages, 1 figure, IOP macro style, submitted to JP
- …