2,699 research outputs found
Equilibrium ion distribution in the presence of clearing electrodes and its influence on electron dynamics
Here we compute the ion distribution produced by an electron beam when
ion-clearing electrodes are installed. This ion density is established as an
equilibrium between gas ionization and ion clearing. The transverse ion
distributions are shown to strongly peak in the beam's center, producing very
nonlinear forces on the electron beam. We will analyze perturbations to the
beam properties by these nonlinear fields. To obtain reasonable simulation
speeds, we develop fast algorithms that take advantage of adiabatic invariants
and scaling properties of Maxwell's equations and the Lorentz force.
Our results are very relevant for high current Energy Recovery Linacs, where
ions are produced relatively quickly, and where clearing gaps in the electron
beam cannot easily be used for ion elimination. The examples in this paper
therefore use parameters of the Cornell Energy Recovery Linac project. For
simplicity we only consider the case of a circular electron beam of changing
diameter. However, we parameterize this model to approximate non-round beams
well. We find suitable places for clearing electrodes and compute the
equilibrium ion density and its effect on electron-emittance growth and halo
development. We find that it is not sufficient to place clearing electrodes
only at the minimum of the electron beam potential where ions are accumulated
Synthesis, Structure, and Applications of Pyridiniophosphines
A new family of cationic ligands, N-alkyl/aryl pyridiniophosphines, has been synthesized through a short, scalable, and highly modular route. Evaluation of their electronic properties evidenced weak σ-donor and quite strong π-acceptor character when used as ancillary ligands. These attributes confer a substantially enhanced π-acidity to the PtII and AuI complexes thereof derived and, as result, they depict an improved ability to activate alkynes towards nucleophilic attack. This superior performance has been demonstrated along several mechanistically diverse PtII- and AuI-catalyzed transformations
Effect of dopants on thermal stability and self-diffusion in iron nitride thin films
We studied the effect of dopants (Al, Ti, Zr) on the thermal stability of
iron nitride thin films prepared using a dc magnetron sputtering technique.
Structure and magnetic characterization of deposited samples reveal that the
thermal stability together with soft magnetic properties of iron nitride thin
films get significantly improved with doping. To understand the observed
results, detailed Fe and N self-diffusion measurements were performed. It was
observed that N self-diffusion gets suppressed with Al doping whereas Ti or Zr
doping results in somewhat faster N diffusion. On the other hand Fe
self-diffusion seems to get suppressed with any dopant of which heat of nitride
formation is significantly smaller than that of iron nitride. Importantly, it
was observed that N self-diffusion plays only a trivial role, as compared to Fe
self-diffusion, in affecting the thermal stability of iron nitride thin films.
Based on the obtained results effect of dopants on self-diffusion process is
discussed.Comment: 10 pages, 9 fig
Short- and long-term health consequences of sleep disruption
Sleep plays a vital role in brain function and systemic physiology across many body systems. Problems with sleep are widely prevalent and include deficits in quantity and quality of sleep; sleep problems that impact the continuity of sleep are collectively referred to as sleep disruptions. Numerous factors contribute to sleep disruption, ranging from lifestyle and environmental factors to sleep disorders and other medical conditions. Sleep disruptions have substantial adverse short-and long-term health consequences. A literature search was conducted to provide a nonsystematic review of these health consequences (this review was designed to be nonsystematic to better focus on the topics of interest due to the myriad parameters affected by sleep). Sleep disruption is associated with increased activity of the sympathetic nervous system and hypothalamic-pituitary-adrenal axis, metabolic effects, changes in circadian rhythms, and proinflammatory responses. In otherwise healthy adults, short-term consequences of sleep disruption include increased stress responsivity, somatic pain, reduced quality of life, emotional distress and mood disorders, and cognitive, memory, and performance deficits. For adolescents, psychosocial health, school performance, and risk-taking behaviors are impacted by sleep disruption. Behavioral problems and cognitive functioning are associated with sleep disruption in children. Long-term consequences of sleep disruption in otherwise healthy individuals include hypertension, dyslipidemia, cardiovascular disease, weight-related issues, metabolic syndrome, type 2 diabetes mellitus, and colorectal cancer. All-cause mortality is also increased in men with sleep disturbances. For those with underlying medical conditions, sleep disruption may diminish the health-related quality of life of children and adolescents and may worsen the severity of common gastrointestinal disorders. As a result of the potential consequences of sleep disruption, health care professionals should be cognizant of how managing underlying medical conditions may help to optimize sleep continuity and consider prescribing interventions that minimize sleep disruption
Intensity interferometry of single x-ray pulses from a synchrotron storage ring
We report on measurements of second-order intensity correlations at the high
brilliance storage ring PETRA III using a prototype of the newly developed
Adaptive Gain Integrating Pixel Detector (AGIPD). The detector recorded
individual synchrotron radiation pulses with an x-ray photon energy of 14.4 keV
and repetition rate of about 5 MHz. The second-order intensity correlation
function was measured simultaneously at different spatial separations that
allowed to determine the transverse coherence length at these x-ray energies.
The measured values are in a good agreement with theoretical simulations based
on the Gaussian Schell-model.Comment: 16 pages, 6 figures, 42 reference
Spin waves and spin-state transitions in a ruthenate high-temperature antiferromagnet
Ruthenium compounds play prominent roles in materials research ranging from
oxide electronics to catalysis, and serve as a platform for fundamental
concepts such as spin-triplet superconductivity, Kitaev spin-liquids, and
solid-state analogues of the Higgs mode in particle physics. However, basic
questions about the electronic structure of ruthenates remain unanswered,
because several key parameters (including the Hund's-rule, spin-orbit, and
exchange interactions) are comparable in magnitude, and their interplay is
poorly understood - partly due to difficulties in synthesizing sizable single
crystals for spectroscopic experiments. Here we introduce a resonant inelastic
x-ray scattering (RIXS) technique capable of probing collective modes in
microcrystals of -electron materials. We present a comprehensive set of
data on spin waves and spin-state transitions in the honeycomb antiferromagnet
SrRuO, which possesses an unusually high N\'eel temperature. The
new RIXS method provides fresh insight into the unconventional magnetism of
SrRuO, and enables momentum-resolved spectroscopy of a large class
of transition-metal compounds.Comment: The original submitted version of the published manuscript.
https://www.nature.com/articles/s41563-019-0327-
- …