Thermopower of a Kondo-correlated quantum dot

The thermopower of a Kondo-correlated gate-defined quantum dot is studied using a current heating technique. In the presence of spin correlations the thermopower shows a clear deviation from the semiclassical Mott relation between thermopower and conductivity. The strong thermopower signal indicates a significant asymmetry in the spectral density of states of the Kondo resonance with respect to the Fermi energies of the reservoirs. The observed behavior can be explained within the framework of an Anderson-impurity model. Keywords: Thermoelectric and thermomagnetic effects, Coulomb blockade, single electron tunneling, Kondo-effect PACS Numbers: 72.20.Pa, 73.23.HkComment: 4 pages, 4 figures, revised version, changed figure

Sequential and co-tunneling behavior in the temperature-dependent thermopower of few-electron quantum dots

We have studied the temperature dependent thermopower of gate-defined, lateral quantum dots in the Coulomb blockade regime using an electron heating technique. The line shape of the thermopower oscillations depends strongly on the contributing tunneling processes. Between 1.5 K and 40 mK a crossover from a pure sawtooth- to an intermitted sawtooth-like line shape is observed. The latter is attributed to the increasing dominance of cotunneling processes in the Coulomb blockade regime at low temperatures.Comment: 4 pages, 4 figures, submitted to Phys. Rev.

Energy level shift of quantum systems via the electric Aharonov-Bohm effect

A novel version of the electric Aharonov-Bohm effect is proposed where the quantum system which picks up the Aharonov-Bohm phase is confined to a Faraday cage with a time varying, spatially uniform scalar potential. The electric and magnetic fields in this region are effectively zero for the entire period of the experiment. The observable consequence of this version of the electric Aharonov-Bohmn effect is to shift the energy levels of the quantum system rather than shift the fringes of the 2-slit interference pattern. We show a strong mathematical connection between this version of the scalar electric AB effect and the AC Stark effect.Comment: 14 pages revtex, 4 figures. Added references and changes made to address referee comments. To be published in PR

Measuring Temperature Gradients over Nanometer Length Scales

When a quantum dot is subjected to a thermal gradient, the temperature of electrons entering the dot can be determined from the dot's thermocurrent if the conductance spectrum and background temperature are known. We demonstrate this technique by measuring the temperature difference across a 15 nm quantum dot embedded in a nanowire. This technique can be used when the dot's energy states are separated by many kT and will enable future quantitative investigations of electron-phonon interaction, nonlinear thermoelectric effects, and the effciency of thermoelectric energy conversion in quantum dots.Comment: 6 pages, 5 figure

Spin-dependent thermoelectric transport through double quantum dots

We study thermoelectric transport through double quantum dots system with spin-dependent interdot coupling and ferromagnetic electrodes by means of the non-equilibrium Green function in the linear response regime. It is found that the thermoelectric coefficients are strongly dependent on the splitting of interdot coupling, the relative magnetic configurations and the spin polarization of leads. In particular, the thermoelectric efficiency can achieve considerable value in parallel configuration when the effective interdot coupling and tunnel coupling between QDs and the leads for spin-down electrons are small. Moreover, the thermoelectric efficiency increases with the intradot Coulomb interactions increasing and can reach very high value at an appropriate temperature. In the presence of the magnetic field, the spin accumulation in leads strongly suppresses the thermoelectric efficiency and a pure spin thermopower can be obtained.Comment: 5 figure

Surface Transitions for Confined Associating Mixtures

Thin films of binary mixtures that interact through isotropic forces and directionally specific "hydrogen bonding" are considered through Monte Carlo simulations. We show, in good agreement with experiment, that the single phase of these mixtures can be stabilized or destabilized on confinement. These results resolve a long standing controversy, since previous theories suggest that confinement only stabilizes the single phase of fluid mixtures.Comment: LaTeX document, documentstyle[aps,preprint]{revtex}, psfig.sty, bibtex, 13 pages, 4 figure

Thermal rectification effect of an interacting quantum dot

We investigate nonlinear thermal transport properties of a single interacting quantum dot with two energy levels tunnel-coupled to two electrodes using nonequilibrium Green function method and Hartree-Fock decoupling approximation. In the case of asymmetric tunnel-couplings to two electrodes, for example, when the upper level of the quantum dot is open for transport, whereas the lower level is blocked, our calculations predict a strong asymmetry for the heat (energy) current, which shows that, the quantum dot system may act as a thermal rectifier in this specific situation.Comment: 5 pages, 5 figure

Enhanced sequential carrier capture into individual quantum dots and quantum posts controlled by surface acoustic waves

Individual self-assembled Quantum Dots and Quantum Posts are studied under the influence of a surface acoustic wave. In optical experiments we observe an acoustically induced switching of the occupancy of the nanostructures along with an overall increase of the emission intensity. For Quantum Posts, switching occurs continuously from predominantely charged excitons (dissimilar number of electrons and holes) to neutral excitons (same number of electrons and holes) and is independent on whether the surface acoustic wave amplitude is increased or decreased. For quantum dots, switching is non-monotonic and shows a pronounced hysteresis on the amplitude sweep direction. Moreover, emission of positively charged and neutral excitons is observed at high surface acoustic wave amplitudes. These findings are explained by carrier trapping and localization in the thin and disordered two-dimensional wetting layer on top of which Quantum Dots nucleate. This limitation can be overcome for Quantum Posts where acoustically induced charge transport is highly efficient in a wide lateral Matrix-Quantum Well.Comment: 11 pages, 5 figure

Surface and capillary transitions in an associating binary mixture model

We investigate the phase diagram of a two-component associating fluid mixture in the presence of selectively adsorbing substrates. The mixture is characterized by a bulk phase diagram which displays peculiar features such as closed loops of immiscibility. The presence of the substrates may interfere the physical mechanism involved in the appearance of these phase diagrams, leading to an enhanced tendency to phase separate below the lower critical solution point. Three different cases are considered: a planar solid surface in contact with a bulk fluid, while the other two represent two models of porous systems, namely a slit and an array on infinitely long parallel cylinders. We confirm that surface transitions, as well as capillary transitions for a large area/volume ratio, are stabilized in the one-phase region. Applicability of our results to experiments reported in the literature is discussed.Comment: 12 two-column pages, 12 figures, accepted for publication in Physical Review E; corrected versio

Electrical and thermoelectrical transport in Dirac fermions through a quantum dot

We investigate the conductance and thermopower of massless Dirac fermions through a quantum dot using a pseudogap Anderson model in the non-crossing approximation. When the Fermi level is at the Dirac point, the conductance has a cusp where the thermopower changes its sign. When the Fermi level is away from the Dirac point, the Kondo temperature illustrates a quantum impurity transition between an asymmetric strong coupling Kondo state and a localized moment state. The conductance shows a peak near this transition and reaches the unitary limit at low temperatures. The magnitude of the thermopower exceeds $k_B/e$, and the thermoelectric figure of merit exceeds unity.Comment: 5 pages, 4 figure