Large X-ray Flares from LMC X-4: Discovery of Milli-hertz Quasi-periodic Oscillations and QPO-modulated Pulsations

We report the discovery of milli-hertz (mHz) quasi-periodic oscillations (QPOs) and QPO-modulated pulsations during large X-ray flares from the high-mass X-ray binary pulsar LMC X-4 using data from the Rossi X-Ray Timing Explorer (RXTE). The lightcurves of flares show that, in addition to ~74 mHz coherent pulsations, there exist two more time-varying temporal structures at frequencies of ~0.65-1.35 and ~2-20 mHz. These relatively long-term structures appear in the power density spectra as mHz QPOs and as well-developed sidebands around the coherent pulse frequency as well, indicating that the amplitudes of the coherent pulsation is modulated by those of the mHz QPOs. One interesting feature is that, while the first flare shows symmetric sidebands around the coherent pulse frequency, the second flare shows significant excess emission in the lower-frequency sidebands due to the ~2-20 mHz QPOs. We discuss the origin of the QPOs using a combination of the beat-frequency model and a modified version of the Keplerian-frequency model. According to our discussion, it seems to be possible to attribute the origin of the ~0.65-1.35 and ~2-20 mHz QPOs to the beating between the rotational frequency of the neutron star and the Keplerian frequency of large accreting clumps near the corotation radius and to the orbital motion of clumps at Keplerian radii of 2-10 times 10^9 cm, respectively.Comment: 12 pages, including 4 figures; accepted by ApJ Letter

Broadband Ferromagnetic Resonance Linewidth Measurement of Magnetic Tunnel Junction Multilayers

The broadband ferromagnetic resonance (FMR) linewidth of the free layer of magnetic tunnel junctions is used as a simple diagnostic of the quality of the magnetic structure. The FMR linewidth increases near the field regions of free layer reversal and pinned layer reversal, and this increase correlates with an increase in magnetic hysteresis in unpatterned films, low frequency noise in patterned devices, and previous observations of magnetic domain ripple by use of Lorentz microscopy. Postannealing changes the free layer FMR linewidth indicating that considerable magnetic disorder, originating in the exchange-biased pinned layer, is transferred to the free layer.Comment: 13 pages, 4 figure

Excited-state dynamics of [Ru(S–Sbpy)(bpy)2]2+to form long-lived localized triplet states

The novel photosensitizer [Ru( S−S bpy)(bpy) 2 ] 2+ harbors two distinct sets of excited states in the UV/Vis region of the absorption spectrum located on either bpy or S−S bpy ligands. Here, we address the question of whether following excitation into these two types of states could lead to the formation of different long-lived excited states from where energy transfer to a reactive species could occur. Femtosecond transient absorption spectros- copy identifies the formation of the final state within 80 fs for both excitation wavelengths. The recorded spectra hint at very similar dynamics following excitation toward either the parent or sulfur- decorated bpy ligands, indicating ultrafast interconversion into a unique excited-state species regardless of the initial state. Non-adiabatic surface hopping dynamics simulations show that ultrafast spin−orbit-mediated mixing of the states within less than 50 fs strongly increases the localization of the excited electron at the S−S bpy ligand. Extensive structural relaxation within this sulfurated ligand is possible, via S−S bond cleavage that results in triplet state energies that are lower than those in the analogue [Ru(bpy)3 ]2+ . This structural relaxation upon localization of the charge on S−S bpy is found to be the reason for the formation of a single long-lived species independent of the excitation wavelength

Growth and characterization of sputtered BSTO/BaM multilayers

Multilayers of Ba0.5Sr0.5TiO3 (BSTO) and BaFe12O19 (BaM), with tunable permeability and permittivity are attractive systems for radio frequency and microwave applications. We have grown multilayers of BSTO and BaM using magnetron sputtering on Al2O3 substrates. Film growth conditions such as sputtering parameters were optimized to obtain high quality multilayers. X-ray diffraction established that both BSTO and BaM were formed and cross-sectional SEM studies showed sharp interfaces between BSTO and BaM layers. Magnetization showed a large coercivity (similar to 2000 Oe) consistent with the hexaferrite component. The hysteresis loops also revealed the distinct influence of magnetocrystalline and shape anisotropies at different temperatures

Multifrequency Observations of the Virgo Blazars 3C 273 and 3C 279 in CGRO Cycle 8

We report first observational results of multifrequency campaigns on the prominent Virgo blazars 3C 273 and 3C 279 which were carried out in January and February 1999. Both blazars are detected from radio to gamma-ray energies. We present the measured X- to gamma-ray spectra of both sources, and for 3C 279 we compare the 1999 broad-band (radio to gamma-ray) spectrum to measured previous ones.Comment: 5 pages including 3 figures, latex2e, to appear in: 'Proc. of the 5th Compton Symposium', AIP, in pres

Switching Distributions for Perpendicular Spin-Torque Devices within the Macrospin Approximation

We model "soft" error rates for writing (WSER) and for reading (RSER) for perpendicular spin-torque memory devices by solving the Fokker-Planck equation for the probability distribution of the angle that the free layer magnetization makes with the normal to the plane of the film. We obtain: (1) an exact, closed form, analytical expression for the zero-temperature switching time as a function of initial angle; (2) an approximate analytical expression for the exponential decay of the WSER as a function of the time the current is applied; (3) comparison of the approximate analytical expression for the WSER to numerical solutions of the Fokker-Planck equation; (4) an approximate analytical expression for the linear increase in RSER with current applied for reading; (5) comparison of the approximate analytical formula for the RSER to the numerical solution of the Fokker-Planck equation; and (6) confirmation of the accuracy of the Fokker-Planck solutions by comparison with results of direct simulation using the single-macrospin Landau-Lifshitz-Gilbert (LLG) equations with a random fluctuating field in the short-time regime for which the latter is practical

Orbital and Super-Orbital Periods of 1E 1740.7-2942 and GRS 1758-258

Five years of Rossi X-ray Timing Explorer (RXTE) observations of the Galactic black-hole candidates 1E 1740.7-2942 and GRS 1758-258 show a periodic modulation with amplitude 3-4% in each source at 12.73 +/- 0.05 dy and 18.45 +/- 0.10 dy, respectively. We interpret the modulations as orbital, suggesting that the objects have red-giant companions. Combining the RXTE data with earlier data (Zhang, Harmon & Liang 1997) from the Burst and Transient Source Experiment on the Compton Gamma-Ray Observatory, we find a long period or quasi-period of about 600 dy in 1E 1740.7-2942, and a suggestion of a similar 600-dy period in GRS 1758-258. These timescales are longer than any yet found for either precessing systems like Her X-1 and SS 433 or binaries like LMC X-3 and Cyg X-1 with more irregular long periods.Comment: 13 pages, 5 figures, accepted by The Astrophysical Journal Letter

Intermolecular London Dispersion Interactions of Azobenzene Switches for Tuning Molecular Solar Thermal Energy Storage Systems

The performance of molecular solar thermal energy storage systems (MOST) depends amongst others on the amount of energy stored. Azobenzenes have been investigated as high-potential materials for MOST applications. In the present study it could be shown that intermolecular attractive London dispersion interactions stabilize the (E)-isomer in bisazobenzene that is linked by different alkyl bridges. Differential scanning calorimetry (DSC) measurements revealed, that this interaction leads to an increased storage energy per azo-unit of more than 3 kcal/mol compared to the parent azobenzene. The origin of this effect has been supported by computation as well as X-ray analysis. In the solid state structure attractive London dispersion interactions between the C−H of the alkyl bridge and the π-system of the azobenzene could be clearly assigned. This concept will be highly useful in designing more effective MOST systems in the future