Is perpendicular magnetic anisotropy essential to all-optical ultrafast spin reversal in ferromagnets?

All-optical spin reversal presents a new opportunity for spin manipulations, free of a magnetic field. Most of all-optical-spin-reversal ferromagnets are found to have a perpendicular magnetic anisotropy (PMA), but it has been unknown whether PMA is necessary for the spin reversal. Here we theoretically investigate magnetic thin films with either PMA or in-plane magnetic anisotropy (IMA). Our results show that the spin reversal in IMA systems is possible, but only with a longer laser pulse and within a narrow laser parameter region. The spin reversal does not show a strong helicity dependence where the left- and right-circularly polarized light lead to the identical results. By contrast, the spin reversal in PMA systems is robust, provided both the spin angular momentum and laser field are strong enough while the magnetic anisotropy itself is not too strong. This explains why experimentally the majority of all-optical spin-reversal samples are found to have strong PMA and why spins in Fe nanoparticles only cant out of plane. It is the laser-induced spin-orbit torque that plays a key role in the spin reversal. Surprisingly, the same spin-orbit torque results in laser-induced spin rectification in spin-mixed configuration, a prediction that can be tested experimentally. Our results clearly point out that PMA is essential to the spin reversal, though there is an opportunity for in-plane spin reversal.Comment: 20 pages, 4 figures and one tabl

Switching ferromagnetic spins by an ultrafast laser pulse: Emergence of giant optical spin-orbit torque

Faster magnetic recording technology is indispensable to massive data storage and big data sciences. {All-optical spin switching offers a possible solution}, but at present it is limited to a handful of expensive and complex rare-earth ferrimagnets. The spin switching in more abundant ferromagnets may significantly expand the scope of all-optical spin switching. Here by studying 40,000 ferromagnetic spins, we show that it is the optical spin-orbit torque that determines the course of spin switching in both ferromagnets and ferrimagnets. Spin switching occurs only if the effective spin angular momentum of each constituent in an alloy exceeds a critical value. Because of the strong exchange coupling, the spin switches much faster in ferromagnets than weakly-coupled ferrimagnets. This establishes a paradigm for all-optical spin switching. The resultant magnetic field (65 T) is so big that it will significantly reduce high current in spintronics, thus representing the beginning of photospintronics.Comment: 12 page2, 6 figures. Accepted to Europhysics Letters (2016). Extended version with the supplementary information. Contribution from Indiana State University,Europhysics Letters (2016

Quasi-particle random phase approximation with quasi-particle-vibration coupling: application to the Gamow-Teller response of the superfluid nucleus 120^{120}Sn

We propose a self-consistent quasi-particle random phase approximation (QRPA) plus quasi-particle-vibration coupling (QPVC) model with Skyrme interactions to describe the width and the line shape of giant resonances in open-shell nuclei, in which the effect of superfluidity should be taken into account in both the ground state and the excited states. We apply the new model to the Gamow-Teller resonance in the superfluid nucleus $^{120}$Sn, including both the isoscalar spin-triplet and the isovector spin-singlet pairing interactions. The strength distribution in $^{120}$Sn is well reproduced and the underlying microscopic mechanisms, related to QPVC and also to isoscalar pairing, are analyzed in detail.Comment: 32 pages, 11 figures, 4 table

Magnetic spin moment reduction in photoexcited ferromagnets through exchange interaction quenching: Beyond the rigid band approximation

The exchange interaction among electrons is one of the most fundamental quantum mechanical interactions in nature and underlies any magnetic phenomena from ferromagnetic ordering to magnetic storage. The current technology is built upon a thermal or magnetic field, but a frontier is emerging to directly control magnetism using ultrashort laser pulses. However, little is known about the fate of the exchange interaction. Here we report unambiguously that photoexcitation is capable of quenching the exchange interaction in all three $3d$ ferromagnetic metals. The entire process starts with a small number of photoexcited electrons which build up a new and self-destructive potential that collapses the system into a new state with a reduced exchange splitting. The spin moment reduction follows a Bloch-like law as $M_z(\Delta E)=M_z(0)(1-{\Delta E}/{\Delta E_0})^{\frac{1}{\beta}}$, where $\Delta E$ is the absorbed photon energy and $\beta$ is a scaling exponent. A good agreement is found between the experimental and our theoretical results. Our findings may have a broader implication for dynamic electron correlation effects in laser-excited iron-based superconductors, iron borate, rare-earth orthoferrites, hematites and rare-earth transition metal alloys.Comment: 16 pages, 3 figures, one supplementary material fil

Multi-wavelength variability properties of Fermi blazar S5 0716+714

S5 0716+714 is a typical BL Lacertae object. In this paper we present the analysis and results of long term simultaneous observations in the radio, near-infrared, optical, X-ray and $\gamma$-ray bands, together with our own photometric observations for this source. The light curves show that the variability amplitudes in $\gamma$-ray and optical bands are larger than those in the hard X-ray and radio bands and that the spectral energy distribution (SED) peaks move to shorter wavelengths when the source becomes brighter, which are similar to other blazars, i.e., more variable at wavelengths shorter than the SED peak frequencies. Analysis shows that the characteristic variability timescales in the 14.5 GHz, the optical, the X-ray, and the $\gamma$-ray bands are comparable to each other. The variations of the hard X-ray and 14.5 GHz emissions are correlated with zero-lag, so are the V band and $\gamma$-ray variations, which are consistent with the leptonic models. Coincidences of $\gamma$-ray and optical flares with a dramatic change of the optical polarization are detected. Hadronic models do not have the same nature explanation for these observations as the leptonic models. A strong optical flare correlating a $\gamma$-ray flare whose peak flux is lower than the average flux is detected. Leptonic model can explain this variability phenomenon through simultaneous SED modeling. Different leptonic models are distinguished by average SED modeling. The synchrotron plus synchrotron self-Compton (SSC) model is ruled out due to the extreme input parameters. Scattering of external seed photons, such as the hot dust or broad line region emission, and the SSC process are probably both needed to explain the $\gamma$-ray emission of S5 0716+714.Comment: 43 pages, 13 figures, 3 tables, to be appeared in Ap

First-principles and model simulation of all-optical spin reversal

All-optical spin switching is a potential trailblazer for information storage and communication at an unprecedented fast rate and free of magnetic fields. However, the current wisdom is largely based on semiempirical models of effective magnetic fields and heat pulses, so it is difficult to provide high-speed design protocols for actual devices. Here, we carry out a massively parallel first-principles and model calculation for thirteen spin systems and magnetic layers, free of any effective field, to establish a simpler and alternative paradigm of laser-induced ultrafast spin reversal and to point out a path to a full-integrated photospintronic device. It is the interplay of the optical selection rule and sublattice spin orderings that underlines seemingly irreconcilable helicity-dependent/independent switchings. Using realistic experimental parameters, we predict that strong ferrimagnets, in particular, Laves phase C15 rare-earth alloys, meet the telecommunication energy requirement of 10 fJ, thus allowing a cost-effective subpicosecond laser to switch spin in the GHz region.Comment: 23 pages, 6 figures and one tabl

Generating high-order optical and spin harmonics from ferromagnetic monolayers

High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far has missed an important group. HHG in magnetic materials should have profound impact on future magnetic storage technology advances. Here we introduce and demonstrate HHG in ferromagnetic monolayers. We find that HHG carries spin information and sensitively depends on the relativistic spin-orbit coupling; and if they are dispersed into the crystal momentum ${\bf k}$ space, harmonics originating from real transitions can be ${\bf k}$-resolved and carry the band structure information. Geometrically, the HHG signal is sensitive to spatial orientations of monolayers. Different from the optical counterpart, the spin HHG, though probably weak, only appears at even orders, a consequence of SU(2) symmetry. Our findings open an unexplored frontier -- magneto-high-order harmonic generation.Comment: 19 pages, 4 figure