131 research outputs found
Influence of higher d-wave gap harmonics on the dynamical magnetic susceptibility of high-temperature superconductors
Using a fermiology approach to the computation of the magnetic susceptibility
measured by neutron scattering in hole-doped high-Tc superconductors, we
estimate the effects on the incommensurate peaks caused by higher d-wave
harmonics of the superconducting order parameter induced by underdoping. The
input parameters for the Fermi surface and d-wave gap are taken directly from
angle resolved photoemission (ARPES) experiments on Bi{2}Sr{2}CaCu{2}O{8+x}
(Bi2212). We find that higher d-wave harmonics lower the momentum dependent
spin gap at the incommensurate peaks as measured by the lowest spectral edge of
the imaginary part in the frequency dependence of the magnetic susceptibility
of Bi2212. This effect is robust whenever the fermiology approach captures the
physics of high-Tc superconductors. At energies above the resonance we observe
diagonal incommensurate peaks. We show that the crossover from parallel
incommensuration below the resonance energy to diagonal incommensuration above
it is connected to the values and the degeneracies of the minima of the
2-particle energy continuum.Comment: 13 pages, 7 figure
Evidence for an incommensurate magnetic resonance in La(2-x)Sr(x)CuO(4)
We study the effect of a magnetic field (applied along the c-axis) on the
low-energy, incommensurate magnetic fluctuations in superconducting
La(1.82)Sr(0.18)CuO(4). The incommensurate peaks at 9 meV, which in zero-field
were previously shown to sharpen in q on cooling below T_c [T. E. Mason et al.,
Phys. Rev. Lett. 77, 1604 (1996)], are found to broaden in q when a field of 10
T is applied. The applied field also causes scattered intensity to shift into
the spin gap. We point out that the response at 9 meV, though occurring at
incommensurate wave vectors, is comparable to the commensurate magnetic
resonance observed at higher energies in other cuprate superconductors.Comment: 8 pages, including 4 figure
Charge ordering, stripes and phase separation in manganese perovskite oxides: an STM/STS study
A microscopic characterisation of the phase transitions associated with
colossal magnetoresistance (CMR) in manganese perovskite oxides is a very
important ingredient in the quest of understanding its underlying mechanism.
Scanning tunneling microscopy (STM) is most suitable to investigate some of
their reported hallmarks, including charge ordering, lattice distortions, and
electronic phase separation. Here we investigate Bi1-XCaXMnO3 (BCMO) with
x=0.76. At this composition, BCMO develops an insulating charge-ordered phase
upon cooling, whose study as a function of temperature will allow identifying
atomic scale characteristics of the metal-insulator phase transition (MIT). We
observe distinct atomic scale phases at temperatures above and below the MIT,
with very different electronic and structural characteristics. Combining STM
micrographs and current-voltage tunneling characteristics, we find that charge
ordering correlates both with the local conduction state (metallic or
insulating) and the local structural order. Furthermore, STM shows coexistence
of these phases as expected for a first order phase transition.Comment: Materials Science and Engineering C, (2005). In Pres
Possible spin-orbit driven spin-liquid ground state in the double perovskite phase of Ba3YIr2O9
We report the structural transformation of hexagonal Ba3YIr2O9 to a cubic
double perovskite form (stable in ambient conditions) under an applied pressure
of 8GPa at 1273K. While the ambient pressure (AP) synthesized sample undergoes
long-range magnetic ordering at 4K, the high pressure(HP) synthesized sample
does not order down to 2K as evidenced from our susceptibility, heat capacity
and nuclear magnetic resonance (NMR) measurements. Further, for the HP sample,
our heat capacity data have the form gamma*T+beta*T3 in the temperature (T)
range of 2-10K with the Sommerfeld coefficient gamma=10mJ/mol-Ir K2. The 89Y
NMR shift has no T-dependence in the range of 4-120K and its spin-lattice
relaxation rate varies linearly with T in the range of 8-45K (above which it is
T-independent). Resistance measurements of both the samples confirm that they
are semiconducting. Our data provide evidence for the formation of a 5d based,
gapless, quantum spin-liquid (QSL) in the cubic (HP) phase of Ba3YIr2O9. In
this picture, the T term in the heat capacity and the linear variation of 89Y
1/T1 arises from excitations out of a spinon Fermi surface. Our findings lend
credence to the theoretical suggestion [G. Chen, R. Pereira, and L. Balents,
Phys. Rev. B 82, 174440 (2010)] that strong spin-orbit coupling can enhance
quantum fluctuations and lead to a QSL state in the double perovskite lattice.Comment: 6 pages 5 figure
Pair Correlations, Short Range Order and Dispersive Excitations in the Quasi-Kagome Quantum Magnet Volborthite
We present spatial and dynamic information on the s=1/2 distorted kagome
antiferromagnet volborthite, Cu3V2O7(OD)2.2D2O, obtained by polarized and
inelastic neutron scattering. The instantaneous structure factor, S(Q), is
dominated by nearest neighbor pair correlations, with short range order at wave
vectors Q1=0.65(3) {\AA}^-1 and Q2=1.15(5) {\AA}^-1 emerging below 5 K. The
excitation spectrum, S(Q,{\omega}), reveals two steep branches dispersing from
Q1 and Q2, and a flat mode at {\omega}=5.0(2) meV. The results allow us to
identify the cross-over at T*=1 K in 51V NMR and specific heat measurements as
the build-up of correlations at Q_1. We compare our data to theoretical models
proposed for volborthite, and demonstrate that the excitation spectrum can be
explained by spin-wave-like excitations with anisotropic exchange parameters,
as also suggested by recent local density calculations.Comment: Rewritten article resubmitted to Phys. Rev. Lett. 021
Orbital occupancies and the putative jeff = 1/2 groundstate in Ba2IrO4: a combined oxygen K edge XAS and RIXS study
The nature of the electronic groundstate of Ba2IrO4 has been addressed using
soft X-ray absorption and inelastic scattering techniques in the vicinity of
the oxygen K edge. From the polarization and angular dependence of XAS we
deduce an approximately equal superposition of xy, yz and zx Ir4+ 5d orbitals.
By combining the measured orbital occupancies, with the value of the spin-orbit
coupling provided by RIXS, we estimate the crystal field splitting associated
with the tetragonal distortion of the IrO6 octahedra to be small, \Delta=50(50)
meV. We thus conclude definitively that Ba2IrO4 is a close realization of a
spin-orbit Mott insulator with a jeff = 1/2 groundstate, thereby overcoming
ambiguities in this assignment associated with the interpretation of X-ray
resonant scattering experiments.Comment: 5 pages, 5 figure
Site dilution of quantum spins in the honeycomb lattice
We discuss the effect of site dilution on both the magnetization and the
density of states of quantum spins in the honeycomb lattice, described by the
antiferromagnetic Heisenberg spin-S model. For this purpose a real-space
Bogoliubov-Valatin transformation is used. In this work we show that for the
S>1/2 the system can be analyzed in terms of linear spin wave theory. For spin
S=1/2, however, the linear spin wave approximation breaks down. In this case,
we have studied the effect of dilution on the staggered magnetization using the
Stochastic Series Expansion Monte Carlo method. Two main results are to be
stressed from the Monte Carlo method: (i) a better value for the staggered
magnetization of the undiluted system, m=0.2677(6); (ii) a finite value of the
staggered magnetization of the percolating cluster at the classical percolation
threshold, showing that there is no quantum critical transition driven by
dilution in the Heisenberg model. In the solution of the problem using linear
the spin wave method we pay special attention to the presence of zero energy
modes. Using a combination of linear spin wave analysis and the recursion
method we were able to obtain the thermodynamic limit behavior of the density
of states for both the square and the honeycomb lattices. We have used both the
staggered magnetization and the density of states to analyze neutron scattering
experiments and Neel temperature measurements on quasi-two- -dimensional
honeycomb systems. Our results are in quantitative agreement with experimental
results on Mn_pZn_{1-p}PS_3 and on the Ba(Ni_pMg_{1-p})_2V_2O_8.Comment: 21 pages (REVTEX), 16 figure
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