Polarized Neutron Inelastic Scattering Study of the Anisotropic Magnetic Fluctuations in the Quasi-1D Ising-like Antiferromagnet TlCoCl3_3

Polarized neutron inelastic scattering experiments have been carried out in the quasi-1D Ising-like antiferromagnet TlCoCl$_3$. We observed the longitudinal magnetic fluctuation $S_{zz} (Q, \omega)$ for the spin-wave excitation continuum, which has not been observed in the unpolarized neutron inelastic scattering experiments of the quasi-1D Ising-like antiferromagnets CsCoCl$_3$ and TlCoCl$_3$ so far, together with the transverse magnetic fluctuation $S_{xx} (Q, \omega)$. We compared both obtained intensities of $S_{xx} (Q, \omega)$ and $S_{zz} (Q, \omega)$ with the perturbation theory from the pure Ising limit by Ishimura and Shiba, and a semi-quantitative agreement was found.Comment: 5 pages, 5 figures, jpsj2.cls, to be published in J. Phys. Soc. Jpn. Vol. 75 (2006) No.

A design method of broadband metalens using time-domain topology optimization

Flat metalenses have attracted attention due to an increasing demand for compact electromagnetic devices. For such applications, broadband metalenses are highly desirable; however, conventional metalenses show relatively narrow band operation. Here, we propose a design method of free-form metalenses using topology optimization to operate with enhanced bandwidths. In contrast with preceding reports of topology optimization methods for metalenses, we developed a topology optimization method based on the time domain formulation to deal with broadband frequencies simultaneously. For this purpose, a group delay of optical pulses in the time domain, which is equivalent to the broadband phase matching condition in the frequency domain, is employed in the objective function. A level set based topology optimization method is applied to obtain a clear optimal configuration. To demonstrate the effectiveness of the proposed method, we provide design examples of metalens unit cells at millimeter frequency. We confirm that optimized unit cells of metalenses show superior performance compared to the conventional unit cells for both transmittance efficiency and phase error in broadband wavelength

Magnetic Excitations in the Quasi-1D Ising-like Antiferromagnet TlCoCl3_3

Neutron inelastic scattering measurements have been performed in order to investigate the magnetic excitations in the quasi-1D Ising-like antiferromagnet TlCoCl$_3$. We observed the magnetic excitation, which corresponds to the spin-wave excitation continuum corresponding to the domain-wall pair excitation in the 1D Ising-like antiferromagnet. According to the Ishimura-Shiba theory, we analyzed the observed spin-wave excitation, and the exchange constant $2J$ and the anistropy $\epsilon$ were estimated as 14.7 meV and 0.14 in TlCoCl$_3$, respectively.Comment: 2 pages, 3 figures, jpsj2.cls, to be published in J. Phys. Soc. Jpn. Vol.75 (2006) No.

Quantification of Crack Formation Using Image Analysis and its Relationship with Permeability

In this study a relationship between permeability of concrete and fractal dimension of crack is established. For this purpose four series of specimens of fiber reinforced cementitious composites are prepared. Specimens are subjected to uniaxial tension in order to create targeted damage (cracking) prior to permeability test. Image analysis is done on the cracked surface and fractal dimension of cracks are calculated using box counting method. Maximum crack width is found to have correlation with the coefficient of permeability. However, such correlation was observed neither between coefficient of permeability and crack area nor between coefficient of permeability and crack density. Relationships of fractal dimension of cracks is established with the maximum crack width, crack area and crack density. Trilateral relationship among coefficient of permeability, the maximum crack width and fractal dimension are established

Sulfur-Mediated Palladium Catalyst Immobilized on a GaAs Surface

We present a hard x-ray photoelectron spectroscopy study on the preparation process of palladium catalyst immobilized on an S-terminated GaAs(100) surface. It is revealed that Pd(II) species are reduced on the GaAssurface and yield Pd nanoparticles during the process of Pd immobilization and the subsequent heat treatment. A comparison with the results on GaAs without S-termination suggests that the reduction of Pd is promoted by hydroxy groups during the Pd immobilization and by S during the heat treatment

Mechanism of Anomalous Tunneling in Condensed Bose System

We clarify the origin of anomalous tunneling [Yu. Kagan et al. Phys. Rev. Lett. 90 (2003) 130402] i.e. the perfect transmission at low energy limit of tunneling of phonon excitations across the potential barrier separating two Bose condensates. The perfect transmission is a consequence of the coincidence of the wave function of the excited state at low energy limit and the macroscopic wave function of the condensate. We show that the perfect transmission at low energy occurs even at finite temperatures within the scheme of Popov approximation.Comment: 4 pages 1 figur

Intramolecular Regulation of Phosphorylation Status of the Circadian Clock Protein KaiC

KaiC, a central clock protein in cyanobacteria, undergoes circadian oscillations between hypophosphorylated and hyperphosphorylated forms in vivo and in vitro. Structural analyses of KaiC crystals have identified threonine and serine residues in KaiC at three residues (T426, S431, and T432) as potential sites at which KaiC is phosphorylated; mutation of any of these three sites to alanine abolishes rhythmicity, revealing an essential clock role for each residue separately and for KaiC phosphorylation in general. Mass spectrometry studies confirmed that the S431 and T432 residues are key phosphorylation sites, however, the role of the threonine residue at position 426 was not clear from the mass spectrometry measurements.Mutational approaches and biochemical analyses of KaiC support a key role for T426 in control of the KaiC phosphorylation status in vivo and in vitro and demonstrates that alternative amino acids at residue 426 dramatically affect KaiC's properties in vivo and in vitro, especially genetic dominance/recessive relationships, KaiC dephosphorylation, and the formation of complexes of KaiC with KaiA and KaiB. These mutations alter key circadian properties, including period, amplitude, robustness, and temperature compensation. Crystallographic analyses indicate that the T426 site is phosphorylatible under some conditions, and in vitro phosphorylation assays of KaiC demonstrate labile phosphorylation of KaiC when the primary S431 and T432 sites are blocked.T426 is a crucial site that regulates KaiC phosphorylation status in vivo and in vitro and these studies underscore the importance of KaiC phosphorylation status in the essential cyanobacterial circadian functions. The regulatory roles of these phosphorylation sites--including T426--within KaiC enhance our understanding of the molecular mechanism underlying circadian rhythm generation in cyanobacteria