300 research outputs found
Anomalous Nernst Effect in Nonmagnetic Nodal Line Semimetal PbTaSe
PbTaSe is a unique topological material, in which the number of nodal
lines is expected to change at the structural transition between the lower
temperature/pressure "L" phase and the higher temperature/pressure "H" phase.
We report the anomalous Nernst effect attributed to the Berry curvature of
nodal lines and its change with the structural transition. In the L phase, the
Nernst coefficient () shows the step-like magnetic field dependence
reminiscent of the anomalous Nernst effect of nonmagnetic Dirac/Weyl
semimetals. By applying hydrostatic pressure, we discovered that the amplitude
of the anomalous component significantly decreases at the transition to the H
phase, which might correspond to the partial annihilation of nodal line
structures.Comment: 29 page, 14 figure
Novel Charge Order and Superconductivity in Two-Dimensional Frustrated Lattice at Quarter Filling
Motivated by the various physical properties observed in
-(BEDT-TTF)X, we study the ground state of extended Hubbard model
on two-dimensional anisotropic triangular lattice at 1/4-filling with
variational Monte Carlo method. It is shown that the nearest-neighbor Coulomb
interaction enhances the charge fluctuation and it induces the anomalous state
such as charge-ordered metallic state and the triplet next-nearest-neighbor
-wave superconductivity. We discuss the relation to the real materials and
propose the unified view of the family of -(BEDT-TTF)X.Comment: 4 pages, 5 figure
Unconventional charge density wave in the organic conductor alpha-(BEDT-TTF)_2KHg(SCN)_4
The low temperature phase (LTP) of alpha-(BEDT-TTF)_2KHg(SCN)_4 salt is known
for its surprising angular dependent magnetoresistance (ADMR), which has been
studied intensively in the last decade. However, the nature of the LTP has not
been understood until now. Here we analyse theoretically ADMR in unconventional
(or nodal) charge density wave (UCDW). In magnetic field the quasiparticle
spectrum in UCDW is quantized, which gives rise to spectacular ADMR. The
present model accounts for many striking features of ADMR data in
alpha-(BEDT-TTF)_2KHg(SCN)_4.Comment: 5 pages, 6 figure
The Origin of the Charge Ordering and Its Relevance to Superconductivity in -(BEDT-TTF)X: The Effect of the Fermi Surface Nesting and the Distant Electron-Electron Interactions
The origin of the charge ordering in organic compounds -(BEDT-TTF) ((SCN), Tl,Rb,Co, Cs,Zn) is studied using an extended
Hubbard model. Calculating the charge susceptibility within random phase
approximation (RPA), we find that the charge
ordering observed at relatively high temperatures can be considered as a
consequence of a cooperation between the Fermi surface nesting, controlled by
the hopping integral in the direction, and the electron-electron
interactions, where the distant (next nearest neighbor) interactions that have
not been taken into account in most of the previous studies play an important
role.Mean field analysis at T=0 also supports the RPA results, and further
shows that in the charge ordered state, some portions of the Fermi
surface remain ungapped and are nested with a nesting vector close to the
modulation wave vector of the horizontal stripe ordering observed at low
temperatures in (SCN). We further study the possibility of
superconductivity by taking into account the distant off-site repulsions and
the band structure corresponding to I, in which superconductivity is
experimentally observed. We find that there is a close competition between
-wave-like singlet pairing and -wave-like triplet pairing due
to a cooperation between the charge and the spin fluctuations. The present
analysis provides a possible unified understanding of the experimental phase
diagram of the -(BEDT-TTF) family, ranging from a charge ordered
insulator to a superconductor.Comment: 13 pages, 18 figures (Figs.5,6,7,14,15,18 compressed using jpeg2ps
Finite-Temperature Properties across the Charge Ordering Transition -- Combined Bosonization, Renormalization Group, and Numerical Methods
We theoretically describe the charge ordering (CO) metal-insulator transition
based on a quasi-one-dimensional extended Hubbard model, and investigate the
finite temperature () properties across the transition temperature, . In order to calculate dependence of physical quantities such as the
spin susceptibility and the electrical resistivity, both above and below
, a theoretical scheme is developed which combines analytical
methods with numerical calculations. We take advantage of the renormalization
group equations derived from the effective bosonized Hamiltonian, where Lanczos
exact diagonalization data are chosen as initial parameters, while the CO order
parameter at finite- is determined by quantum Monte Carlo simulations. The
results show that the spin susceptibility does not show a steep singularity at
, and it slightly increases compared to the case without CO because
of the suppression of the spin velocity. In contrast, the resistivity exhibits
a sudden increase at , below which a characteristic dependence
is observed. We also compare our results with experiments on molecular
conductors as well as transition metal oxides showing CO.Comment: 9 pages, 8 figure
Electronic correlation in the infrared optical properties of the quasi two dimensional -type BEDT-TTF dimer system
The polarized optical reflectance spectra of the quasi two dimensional
organic correlated electron system -(BEDT-TTF)Cu[N(CN)],
Br and Cl are measured in the infrared region. The former shows the
superconductivity at 11.6 K and the latter does the
antiferromagnetic insulator transition at 28 K. Both the
specific molecular vibration mode of the BEDT-TTF molecule and
the optical conductivity hump in the mid-infrared region change correlatively
at 38 K of -(BEDT-TTF)Cu[N(CN)]Br, although
no indication of but the insulating behaviour below 50-60 K are found in -(BEDT-TTF)Cu[N(CN)]Cl. The
results suggest that the electron-molecular vibration coupling on the
mode becomes weak due to the enhancement of the itinerant
nature of the carriers on the dimer of the BEDT-TTF molecules below ,
while it does strong below because of the localized carriers on
the dimer. These changes are in agreement with the reduction and the
enhancement of the mid-infrared conductivity hump below and , respectively, which originates from the transitions between the upper
and lower Mott-Hubbard bands. The present observations demonstrate that two
different metallic states of -(BEDT-TTF)Cu[N(CN)]Br are
regarded as {\it a correlated good metal} below including the
superconducting state and {\it a half filling bad metal} above . In
contrast the insulating state of -(BEDT-TTF)Cu[N(CN)]Cl
below is the Mott insulator.Comment: 8 pages, 7 figure
Fermiology and superconductivity studies on the non-tetrachalcogenafulvalene structured organic superconductor beta-(BDA-TTP)_2SbF_6
The quantum oscillatory effect and superconductivity in a
non-tetrachalcogenafulvalene (TCF) structure based organic superconductor
beta-(BDA-TTP)_2SbF_6 are studied. Here the Shubnikov-de Haas effect (SdH) and
angular dependent magnetoresistance oscillations (AMRO) are observed. The
oscillation frequency associated with a cylindrical Fermi surface is found to
be about 4050 tesla, which is also verified by the tunnel diode oscillator
(TDO) measurement. The upper critical field Hc2 measurement in a tilted
magnetic field and the TDO measurement in the mixed state reveal a highly
anisotropic superconducting nature in this material. We compared physical
properties of beta-(BDA-TTP)_2SbF_6 with typical TCF structure based quasi
two-dimensional organic conductors. A notable feature of beta-(BDA-TTP)_2SbF_6
superconductor is a large value of effective cyclotron mass m_c^*=12.4+/1.1
m_e, which is the largest yet found in an organic superconductor. A possible
origin of the enhanced effective mass and its relation to the superconductivity
are briefly discussed.Comment: 8 pages, 10 figure
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