Characterization of aerosol hygroscopicity over the Northeast Pacific Ocean: Impacts on prediction of CCN and stratocumulus cloud droplet number concentrations

During the Marine Aerosol Cloud and Wildfire Study (MACAWS) in June and July of 2018, aerosol composition and cloud condensation nuclei (CCN) properties were measured over the N.E. Pacific to characterize the influence of aerosol hygroscopicity on predictions of ambient CCN and stratocumulus cloud droplet number concentrations (CDNC). Three vertical regions were characterized, corresponding to the marine boundary layer (MBL), an above‐cloud organic aerosol layer (AC‐OAL), and the free troposphere (FT) above the AC‐OAL. The aerosol hygroscopicity parameter (κ) was calculated from CCN measurements (κ_(CCN)) and bulk aerosol mass spectrometer (AMS) measurements (κ_(AMS)). Within the MBL, measured hygroscopicities varied between values typical of both continental environments (~0.2) and remote marine locations (~0.7). For most flights, CCN closure was achieved within 20% in the MBL. For five of the seven flights, assuming a constant aerosol size distribution produced similar or better CCN closure than assuming a constant “marine” hygroscopicity (κ = 0.72). An aerosol‐cloud parcel model was used to characterize the sensitivity of predicted stratocumulus CDNC to aerosol hygroscopicity, size distribution properties, and updraft velocity. Average CDNC sensitivity to accumulation mode aerosol hygroscopicity is 39% as large as the sensitivity to the geometric median diameter in this environment. Simulations suggest CDNC sensitivity to hygroscopicity is largest in marine stratocumulus with low updraft velocities (0.6 m s⁻¹), where hygroscopic properties of the Aitken mode dominate hygroscopicity sensitivity

Characterization of aerosol hygroscopicity over the Northeast Pacific Ocean: Impacts on prediction of CCN and stratocumulus cloud droplet number concentrations

During the Marine Aerosol Cloud and Wildfire Study (MACAWS) in June and July of 2018, aerosol composition and cloud condensation nuclei (CCN) properties were measured over the N.E. Pacific to characterize the influence of aerosol hygroscopicity on predictions of ambient CCN and stratocumulus cloud droplet number concentrations (CDNC). Three vertical regions were characterized, corresponding to the marine boundary layer (MBL), an above‐cloud organic aerosol layer (AC‐OAL), and the free troposphere (FT) above the AC‐OAL. The aerosol hygroscopicity parameter (κ) was calculated from CCN measurements (κ_(CCN)) and bulk aerosol mass spectrometer (AMS) measurements (κ_(AMS)). Within the MBL, measured hygroscopicities varied between values typical of both continental environments (~0.2) and remote marine locations (~0.7). For most flights, CCN closure was achieved within 20% in the MBL. For five of the seven flights, assuming a constant aerosol size distribution produced similar or better CCN closure than assuming a constant “marine” hygroscopicity (κ = 0.72). An aerosol‐cloud parcel model was used to characterize the sensitivity of predicted stratocumulus CDNC to aerosol hygroscopicity, size distribution properties, and updraft velocity. Average CDNC sensitivity to accumulation mode aerosol hygroscopicity is 39% as large as the sensitivity to the geometric median diameter in this environment. Simulations suggest CDNC sensitivity to hygroscopicity is largest in marine stratocumulus with low updraft velocities (0.6 m s⁻¹), where hygroscopic properties of the Aitken mode dominate hygroscopicity sensitivity

Inclusive Scattering of Polarized Electrons on Polarized 3He Effects of Final State Interaction and the Magnetic Form Factor of the Neutron

Effects of final state interaction on asymmetries in inclusive scattering of polarized electrons on polarized 3He are investigated using consistent 3He bound state wave function and 3N continuum scattering states. Significant effects are found, which influence the extraction of the magnetic neutron form factor from A_T'. The enhancement found experimentally for A_TL' near the 3N breakup threshold, which could not be explained in calculations carried through in plane wave impulse approximation up to now, occurs now also in theory if the full final state interaction is included.Comment: 29 pages, 5 figure

Inorganic Approach to Stabilizing Nanoscale Toroidicity in a Tetraicosanuclear Fe18_{18}Dy6_{6} Single Molecule Magnet

Cyclic coordination clusters (CCCs) are proving to provide an extra dimension in terms of exotic magnetic behavior as a result of their finite but cyclized chain structures. The Fe$_{18}$Dy$_{6}$ CCC is a Single Molecule Magnet with the highest nuclearity among Ln containing clusters. The three isostructural compounds [Fe$_{18}$Ln$_{6}$(μ-OH)$_{6}$(ampd)$_{12}$(Hampd)$_{12}$(PhCO$_{2}$)$_{24}$](NO$_{3}$)$_{6}$·38MeCN for Ln = Dy$^{III}$ (1), Lu$^{III}$ (2), or Y$^{III}$ (3), where H$_{2}^{-}$ampd = 2-amino-2-methyl-1,3-propanediol, are reported. These can be described in terms of the cyclization of six {Fe$_{3}$Ln(μOH)(ampd)$_{2}$(Hampd)$_{2}$(PhCO$_{2}$)$_{4}$}$^{+}$ units with six nitrate counterions to give the neutral cluster. The overall structure consists of two giant Dy$_{3}$ triangles sandwiching a strongly antiferromagnetically coupled Fe$_{18}$ ring, leading to a toroidal arrangement of the anisotropy axis of the Dy ions, making this the biggest toroidal arrangement on a molecular level known so far

Angle-resolved photoemission and first-principles electronic structure of single-crystalline α\alpha-uranium (001)

Continuing the photoemission study begun with the work of Opeil et al. [Phys. Rev. B \textbf{73}, 165109 (2006)], in this paper we report results of an angle-resolved photoemission spectroscopy (ARPES) study performed on a high-quality single-crystal $\alpha$-uranium at 173 K. The absence of surface-reconstruction effects is verified using X-ray Laue and low-energy electron diffraction (LEED) patterns. We compare the ARPES intensity map with first-principles band structure calculations using a generalized gradient approximation (GGA) and we find good correlations with the calculated dispersion of the electronic bands

Nucleon-Nucleon Phase Shifts and Pairing in Neutron Matter and Nuclear Matter

We consider 1S0 pairing in infinite neutron matter and nuclear matter and show that in the lowest order approximation, where the pairing interaction is taken to be the bare nucleon-nucleon (NN) interaction in the 1S0 channel, the pairing interaction and the energy gap can be determined directly from the 1S0 phase shifts. This is due to the almost separable character of the NN interaction in this partial wave. Since the most recent NN interactions are charge-dependent, we have to solve coupled gap equations for proton-proton, neutron-neutron, and neutron-proton pairing in nuclear matter. The results, however, are found to be close to those obtained with charge-independent potentials.Comment: 5 pages, 3 figures, RevTe

Hybrid stars with the color dielectric and the MIT bag models

We study the hadron-quark phase transition in the interior of neutron stars (NS). For the hadronic sector, we use a microscopic equation of state (EOS) involving nucleons and hyperons derived within the Brueckner-Bethe-Goldstone many-body theory, with realistic two-body and three-body forces. For the description of quark matter, we employ both the MIT bag model with a density dependent bag constant, and the color dielectric model. We calculate the structure of NS interiors with the EOS comprising both phases, and we find that the NS maximum masses are never larger than 1.7 solar masses, no matter the model chosen for describing the pure quark phase.Comment: 11 pages, 5 figures, submitted to Phys. Rev.

Anderson-localization versus delocalization of interacting fermions in one dimension

Using the density matrix renormalization group algorithm, we investigate the lattice model for spinless fermions in one dimension in the presence of a strong interaction and disorder. The phase sensitivity of the ground state energy is determined with high accuracy for systems up to a size of 60 lattice constants. This quantity is found to be log-normally distributed. The fluctuations grow algebraically with system size with a universal exponent of ~2/3 in the localized region of the phase diagram. Surprizingly, we find, for an attractive interaction, a delocalized phase of finite extension. The boundary of this delocalized phase is determined.Comment: 5 pages, 6 figures, revte

Phases of asymmetric nuclear matter with broken space symmetries

Isoscalar Cooper pairing in isospin asymmetric nuclear matter occurs between states populating two distinct Fermi surfaces, each for neutrons and protons. The transition from a BCS-like to the normal (unpaired) state, as the isospin asymmetry is increased, is intervened by superconducting phases which spontaneously break translational and rotational symmetries. One possibility is the formation of a condensate with a periodic crystallinelike structure where Cooper pairs carry net momentum (the nuclear Larkin-Ovchinnikov-Fulde-Ferrell-phase). Alternatively, perturbations of the Fermi surfaces away from spherical symmetry allow for minima in the condensate free energy which correspond to a states with quadrupole deformations of Fermi surfaces and zero momentum of the Cooper pairs. In a combined treatment of these phases we show that, although the Cooper pairing with finite momentum might arise as a local minimum, the lowest energy state features are deformed Fermi surfaces and Cooper pairs with vanishing total momentum.Comment: 22 pages, 6 figures, RevTex; v2: matches published version; v3: changes in the frontmatter, content unchange