Transition from a Tomonaga-Luttinger liquid to a Fermi liquid in potassium intercalated bundles of single wall carbon nanotubes

We report on the first direct observation of a transition from a Tomonaga-Luttinger liquid to a Fermi liquid behavior in potassium intercalated mats of single wall carbon nanotubes (SWCNT). Using high resolution photoemission spectroscopy an analysis of the spectral shape near the Fermi level reveals a Tomonaga-Luttinger liquid power law scaling in the density of states for the pristine sample and for low dopant concentration. As soon as the doping is high enough to fill bands of the semiconducting tubes a distinct transition to a bundle of only metallic SWCNT with a scaling behavior of a normal Fermi liquid occurs. This can be explained by a strong screening of the Coulomb interaction between charge carriers and/or an increased hopping matrix element between the tubes.Comment: 5 pages, 4 figure

Extremely Small Energy Gap in the Quasi-One-Dimensional Conducting Chain Compound SrNbO3.41_{3.41}

Resistivity, optical, and angle-resolved photoemission experiments reveal unusual one-dimensional electronic properties of highly anisotropic SrNbO$_{3.41}$. Along the conducting chain direction we find an extremely small energy gap of only a few meV at the Fermi level. A discussion in terms of typical 1D instabilities (Peierls, Mott-Hubbard) shows that neither seems to provide a satisfactory explanation for the unique properties of SrNbO$_{3.41}$.Comment: 4 pages, 3 figure

Ag-coverage-dependent symmetry of the electronic states of the Pt(111)-Ag-Bi interface: The ARPES view of a structural transition

We studied by angle-resolved photoelectron spectroscopy the strain-related structural transition from a pseudomorphic monolayer (ML) to a striped incommensurate phase in an Ag thin film grown on Pt(111). We exploited the surfactant properties of Bi to grow ordered Pt(111)-xMLAg-Bi trilayers with 0 < x < 5 ML, and monitored the dispersion of the Bi-derived interface states to probe the structure of the underlying Ag film. We find that their symmetry changes from threefold to sixfold and back to threefold in the Ag coverage range studied. Together with previous scanning tunneling microscopy and photoelectron diffraction data, these results provide a consistent microscopic description of the coverage-dependent structural transition.Comment: 10 pages, 9 figure

Tunable Polaronic Conduction in Anatase TiO2

Oxygen vacancies created in anatase TiO2 by UV photons (80–130 eV) provide an effective electron-doping mechanism and induce a hitherto unobserved dispersive metallic state. Angle resolved photoemission reveals that the quasiparticles are large polarons. These results indicate that anatase can be tuned from an insulator to a polaron gas to a weakly correlated metal as a function of doping and clarify the nature of conductivity in this material.open1192sciescopu

Evolution of the quasiparticle spectral function in cuprates

We analyzed photoemssion data for several doping levels of the Bi_2Sr_2CaCu_2O_{8+x} compounds, ranging from overdoped to underdoped. We show that the high frequency part of the spectra near (0,\pi) can be described by Fermi liquid theory in the overdoped regime, but exhibits a non-Fermi liquid behavior in the underdoped regime. We further demonstrate that this novel behavior fits reasonably well to a 1/\sqrt{\omega} behavior suggested for systems with strong spin fluctuations.Comment: 5 pages, 2 figures (EPS), RevTeX, submitted to Phys Rev B R

Nodal Landau Fermi-Liquid Quasiparticles in Overdoped La1.77_{1.77}Sr0.23_{0.23}CuO4_4

Nodal angle resolved photoemission spectra taken on overdoped La$_{1.77}$Sr$_{0.23}$CuO$_4$ are presented and analyzed. It is proven that the low-energy excitations are true Landau Fermi-liquid quasiparticles. We show that momentum and energy distribution curves can be analyzed self-consistently without quantitative knowledge of the bare band dispersion. Finally, by imposing Kramers-Kronig consistency on the self-energy $\Sigma$, insight into the quasiparticle residue is gained. We conclude by comparing our results to quasiparticle properties extracted from thermodynamic, magneto-resistance, and high-field quantum oscillation experiments on overdoped Tl$_2$Ba$_2$CuO$_{6+\delta}$.Comment: Accepted for publication in Phys. Rev.

Electronic Instability in a Zero-Gap Semiconductor: The Charge-DensityWave in (TaSe4)(2)I

We report a comprehensive study of the paradigmatic quasi-1D compound (TaSe4)(2)I performed by means of angle-resolved photoemission spectroscopy (ARPES) and first-principles electronic structure calculations. We find it to be a zero-gap semiconductor in the nondistorted structure, with non-negligible interchain coupling. Theory and experiment support a Peierls-like scenario for the charge-density wave formation below T-CDW = 263 K, where the incommensurability is a direct consequence of the finite interchain coupling. The formation of small polarons, strongly suggested by the ARPES data, explains the puzzling semiconductor-to-semiconductor transition observed in transport at T-CDW.open114sciescopu

Silicon surface with giant spin-splitting

We demonstrate the induction of a giant Rashba-type spin-splitting on a semiconducting substrate by means of a Bi trimer adlayer on a Si(111) wafer. The in-plane inversion symmetry is broken so that the in-plane potential gradient induces a giant spin-splitting with a Rashba energy of about 140 meV, which is more than an order of magnitude larger than what has previously been reported for any semiconductor heterostructure. The separation of the electronic states is larger than their lifetime broadening, which has been directly observed with angular resolved photoemission spectroscopy. The experimental results are confirmed by relativistic first-principles calculations. We envision important implications for basic phenomena as well as for the semiconductor based technology

Spectroscopic signatures of a bandwidth-controlled Mott transition at the surface of 1T-TaSe2_2

High-resolution angle-resolved photoemission (ARPES) data show that a metal-insulator Mott transition occurs at the surface of the quasi-two dimensional compound TaSe$_2$. The transition is driven by the narrowing of the Ta $5d$ band induced by a temperature-dependent modulation of the atomic positions. A dynamical mean-field theory calculation of the spectral function of the half-filled Hubbard model captures the main qualitative feature of the data, namely the rapid transfer of spectral weight from the observed quasiparticle peak at the Fermi surface to the Hubbard bands, as the correlation gap opens up.Comment: 4 pages, 4 figures; one modified figure, added referenc

Local spectral properties of Luttinger liquids: scaling versus nonuniversal energy scales

Motivated by recent scanning tunneling and photoemission spectroscopy measurements on self-organized gold chains on a germanium surface we reinvestigate the local single-particle spectral properties of Luttinger liquids. In the first part we use the bosonization approach to exactly compute the local spectral function of a simplified field theoretical low-energy model and take a closer look at scaling properties as a function of the ratio of energy and temperature. Translational invariant Luttinger liquids as well as those with an open boundary (cut chain geometry) are considered. We explicitly show that the scaling functions of both setups have the same analytic form. The scaling behavior suggests a variety of consistency checks which can be performed on measured data to experimentally verify Luttinger liquid behavior. In a second part we approximately compute the local spectral function of a microscopic lattice model---the extended Hubbard model---close to an open boundary using the functional renormalization group. We show that as a function of energy and temperature it follows the field theoretical prediction in the low-energy regime and point out the importance of nonuniversal energy scales inherent to any microscopic model. The spatial dependence of this spectral function is characterized by oscillatory behavior and an envelope function which follows a power law both in accordance with the field theoretical continuum model. Interestingly, for the lattice model we find a phase shift which is proportional to the two-particle interaction and not accounted for in the standard bosonization approach to Luttinger liquids with an open boundary. We briefly comment on the effects of several one-dimensional branches cutting the Fermi energy and Rashba spin-orbit interaction.Comment: 19 pages, 5 figures, version as accepted for publication in J. Phys.:Condensed Matte