Stabilization of A-type layered antiferromagnetic phase in LaMnO_3 by cooperative Jahn-Teller deformations

It is shown that the layered antiferromagnetic order in stoechiometric LaMnO_3 cannot be understood purely from electronic interactions. On the contrary, it mainly results from strong cooperative Jahn-Teller deformations. Those involve a compression of the Mn-O octahedron along the c-axis (mode Q_3 < 0), while alternate Jahn-Teller deformations occur in the ab-plane (mode Q_2). These deformations stabilize a certain type of orbital ordering. The resulting superexchange couplings are calculated by exact diagonalization, taking into account both e_g and t_{2g} orbitals. The main result is that antiferromagnetic (ferromagnetic) coupling along the c-direction (ab-planes) can be understood only if the Jahn-Teller energy is much larger than the superexchange couplings, which is consistent with experiments. This mechanism contrasts with that based on weak Jahn-Teller coupling which instead predicts elongation along the c-axis (Q_3 > 0). The crucial role of the deformation anisotropy Q_2/Q_3 is also emphasized.Comment: 8 pages, 6 figure

Jahn-Teller, Charge and Magnetic Ordering in half-doped Manganese Oxides

The phase diagram of half-doped manganite systems of formula A_{0.5}A'_{0.5}MnO_3 is investigated within a single-orbital model incorporating magnetic double-exchange and superexchange, together with intersite Coulomb and electron-lattice interactions. Strong Jahn-Teller and breathing mode deformations compete together and result in shear lattice deformations. The latters stabilize the charge-ordered CE-type phase, which undergo first-order transitions with temperature or magnetic field to either Ferromagnetic metallic or Paramagnetic insulating phases. An essential feature is the self-consistent screening of Coulomb and electron-phonon interactions in the ferromagnetic phase.Comment: 10 pages, six figures (eps files) +two class file

A large-N analysis of the local quantum critical point and the spin-liquid phase

We study analytically the Kondo lattice model with an additional nearest-neighbor antiferromagnetic interaction in the framework of large-N theory. We find that there is a local quantum critical point between two phases, a normal Fermi-liquid and a spin-liquid in which the spins are decoupled from the conduction electrons. The local spin susceptibility displays a power-law divergence throughout the spin liquid phase. We check the reliability of the large-N results by solving by quantum Monte Carlo simulation the N=2 spin-liquid problem with no conduction electrons and find qualitative agreement. We show that the spin-liquid phase is unstable at low temperatures, suggestive of a first-order transition to an ordered phase.Comment: 4 pages and 1 figur

Joint superexchange--Jahn-Teller mechanism for A-type antiferromagnetism in LaMnO3LaMnO_3

We propose a mechanism for A-type antiferromagnetism in orthorombic LaMnO_3, compatible with the large Jahn-Teller splitting inferred from structural data. Orbital ordering resulting from Jahn-Teller distortions effectively leads to A-type ordering (antiferromagnetic in the c axis and ferromagnetic in the ab plane) provided the in-plane distorsion Q_2 is large enough, a condition generally fulfilled in existing data.Comment: 4 pages Late

Phase separation and long wave-length charge instabilities in spin-orbit coupled systems

We investigate a two-dimensional electron model with Rashba spin-orbit interaction where the coupling constant $g=g(n)$ depends on the electronic density. It is shown that this dependence may drive the system unstable towards a long-wave length charge density wave (CDW) where the associated second order instability occurs in close vicinity to global phase separation. For very low electron densities the CDW instability is nesting-induced and the modulation follows the Fermi momentum $k_F$. At higher density the instability criterion becomes independent of $k_F$ and the system may become unstable in a broad momentum range. Finally, upon filling the upper spin-orbit split band, finite momentum instabilities disappear in favor of phase separation alone. We discuss our results with regard to the inhomogeneous phases observed at the LaAlO$_3$/SrTiO$_3$ or LaTiO$_3$/SrTiO$_3$ interfaces.Comment: 6 pages, 6 figure

Phase diagrams of voltage-gated oxide interfaces with strong Rashba coupling

We propose a model for the two-dimensional electron gas formed at the interface of oxide heterostructures that includes a Rashba spin-orbit coupling proportional to an electric field oriented perpendicularly to the interface. Taking into account the electron density dependence of this electric field confining the electron gas at the interface, we report the occurrence of a phase separation instability (signaled by a negative compressibility) for realistic values of the spin-orbit coupling and of the electronic band-structure parameters at zero temperature. We extend the analysis to finite temperatures and in the presence of an in-plane magnetic field, thereby obtaining two phase diagrams which exhibit a phase separation dome. By varying the gating potential the phase separation dome may shrink and vanish at zero temperature into a quantum critical point where the charge fluctuates dynamically. Similarly the phase separation may be spoiled by a planar magnetic field even at zero temperature leading to a line of quantum critical points.Comment: 17 pages, 17 figure