210 research outputs found
Static Critical Behavior of the Spin-Freezing Transition in the Geometrically Frustrated Pyrochlore Antiferromagnet Y2Mo2O7
Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a
spin-freezing transition and magnetic irreversibilities below a temperature Tf
similar to what is observed nonlinear magnetization measurements on Y2Mo2O7
that provide strong evidence that there is an underlying thermodynamic phase
transition at Tf, which is characterized by critical exponents \gamma \approx
2.8 and \beta \approx 0.8. These values are typical of those found in random
spin glasses, despite the fact that the level of random disorder in Y2Mo2O7 is
immeasurably small.Comment: Latex file, calls for 4 encapsulated postscript figures (included).
Submitted to Phys. Rev. Letters
Aging and memory properties of topologically frustrated magnets
The model 2d kagome system (H3O)Fe3(SO4)2(OH)6 and the 3d pyrochlore Y2Mo2O7
are two well characterized examples of low-disordered frustrated
antiferromagnets which rather then condensing into spin liquid have been found
to undergo a freezing transition with spin glass-like properties. We explore
more deeply the comparison of their properties with those of spin glasses, by
the study of characteristic rejuvenation and memory effects in the
non-stationary susceptibility. While the pyrochlore shows clear evidence for
these non-trivial effects, implying temperature selective aging, that is
characteristic of a wide hierarchical distribution of equilibration processes,
the kagome system does n not show clearly these effects. Rather, it seems to
evolve towards the same final state independently of temperature.Comment: submitted for the proceedings of the 46th MMM conference (Seattle,
2001
The magnetic response at the metal–insulator transition in La1−xSrxTiO3 (abstract)
We report on recent inelastic neutron scattering measurements of the magnetic response close to the metal–insulator transition in La1−xSrxTiO3. Specific heat and susceptibility data from Tokura et al. give evidence for a divergent effective mass at the critical concentration xc=0.05 in agreement with recent mean‐field theories of the transition. The mass enhancement is believed to arise from the formation of a d‐electron resonance at the Fermi energy close to the transition. The aim of this investigation is to look for evidence of this resonance in the dynamic magnetic susceptibility. We studied samples with x=0, 0.05, and 0.2 using incident energies between 25 and 200 meV. After correction for the phonon scattering, we observe a broad response above a threshold of 20–30 meV extending to over 100 meV. In addition, the Mott insulating antiferromagnet (x=0) has a peak at 40 meV, consistent with the estimated activation energy derived from resistivity measurements. This feature becomes washed out with temperature and doping. Possible origins for this peak are discussed. © 1996 American Institute of Physics.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/70552/2/JAPIAU-79-8-6432-1.pd
Manifestation of geometric frustration on magnetic and thermodynamic properties of pyrochlores (X=Ti, Zr)
We present here magnetization, specific heat and Raman studies on
single-crystalline specimens of the first pyrochlore member of
the rare-earth titanate series. Its analogous compound in the
rare-earth zirconate series is also investigated in the polycrystalline form.
The Sm spins in remain unordered down to at least T = 0.5 K. The
absence of magnetic ordering is attributed to very small values of exchange
() and dipolar interaction ()
between the spins in this pyrochlore. In contrast, the pyrochlore
is characterized by a relatively large value of Sm-Sm spin
exchange (); however, long-range ordering of the
spins is not established at least down to T = 0.67 K, due to
frustration of the spins on the pyrochlore lattice. The ground state
of ions in both pyrochlores is a well-isolated Kramer's doublet. The
higher-lying crystal field excitations are observed in the low-frequency region
of the Raman spectra of the two compounds recorded at T = 10 K. At higher
temperatures, the magnetic susceptibility of shows a broad
maximum at T = 140 K while that of changes monotonically. Whereas
is a promising candidate for investigating spin-fluctuations on a
frustrated lattice as indicated by our data, the properties of
seem to conform to a conventional scenario where geometrical frustration of the
spin exclude their long-range ordering.Comment: 24 pages, 6 figures, Accepted for publication in Phys. Rev.
Magnetic Ordering in the Spin-Ice Candidate HoRuO
Neutron scattering measurements on the spin-ice candidate material
HoRuO have revealed two magnetic transitions at T 95 K and T
1.4 K to long-range ordered states involving the Ru and Ho sublattices,
respectively. Between these transitions, the Ho moments form
short-ranged ordered spin clusters. The internal field provided by the ordered
S=1 Ru moments disrupts the fragile spin-ice state and drives the
Ho moments to order. We have directly measured a slight shift in the
Ho crystal field levels at 95 K from the Ru ordering.Comment: 4 pages, 5 figures, submitted to Phys. Rev. Letter
Transition to Long Range Magnetic Order in the Highly Frustrated Insulating Pyrochlore Antiferromagnet Gd_2Ti_2O_7
Experimental evidence from measurements of the a.c. and d.c. susceptibility,
and heat capacity data show that the pyrochlore structure oxide, Gd_2Ti_2O_7,
exhibits short range order that starts developing at 30K, as well as long range
magnetic order at K. The Curie-Weiss temperature, =
-9.6K, is largely due to exchange interactions. Deviations from the Curie-Weiss
law occur below 10K while magnetic heat capacity contributions are found
at temperatures above 20K. A sharp maximum in the heat capacity at K
signals a transition to a long range ordered state, with the magnetic specific
accounting for only 50% of the magnetic entropy. The heat capacity above
the phase transition can be modeled by assuming that a distribution of random
fields acts on the ground state for Gd. There is no
frequency dependence to the a.c. susceptibility in either the short range or
long range ordered regimes, hence suggesting the absence of any spin-glassy
behavior. Mean field theoretical calculations show that no long range ordered
ground state exists for the conditions of nearest-neighbor antiferromagnetic
exchange and long range dipolar couplings. At the mean-field level, long range
order at various commensurate or incommensurate wave vectors is found only upon
inclusion of exchange interactions beyond nearest-neighbor exchange and dipolar
coupling. The properties of Gd$_2Ti_2O_7 are compared with other geometrically
frustrated antiferromagnets such as the Gd_3Ga_5O_{12} gadolinium gallium
garnet, RE_2Ti_2O_7 pyrochlores where RE = Tb, Ho and Tm, and Heisenberg-type
pyrochlore such as Y_2Mo_2O_7, Tb_2Mo_2O_7, and spinels such as ZnFe_2O_4Comment: Letter, 6 POSTSCRIPT figures included. (NOTE: Figure 5 is not
included --) To appear in Physical Review B. Contact:
[email protected]
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