144 research outputs found
Quasi-Particle Spectra, Charge-Density-Wave, Superconductivity and Electron-Phonon Coupling in 2H-NbSe2
High-resolution photoemission has been used to study the electronic structure
of the charge density wave (CDW) and superconducting (SC) dichalcogenide, 2H-
NbSe2. From the extracted self-energies, important components of the
quasiparticle (QP) interactions have been identified. In contrast to previously
studied TaSe2, the CDW transition does not affect the electronic properties
significantly. The electron-phonon coupling is identified as a dominant
contribution to the QP self-energy and is shown to be very anisotropic
(k-dependent) and much stronger than in TaSe2.Comment: 4 pages, 3 figures, minor changes, to appear in PR
High-Resolution Electron Time-of-Flight Apparatus for the Soft-X-Ray Region
A gas-phase time-of-flight (TOF) apparatus, capable of supporting as many as six electron-TOF analyzers viewing the same interaction region, has been developed to measure energy- and angle-resolved electrons with kinetic energies up to 5 keV. Each analyzer includes a newly designed lens system that can retard electrons to about 2% of their initial kinetic energy without significant loss of transmission; the analyzers can thus achieve a resolving power (E/ΔE) greater than 104 over a wide kinetic-energy range. Such high resolving power is comparable to the photon energy resolution of state-of-the-art synchrotron–radiation beamlines in the soft x-ray range, opening the TOF technique to numerous high-resolution applications. In addition, the angular placement of the analyzers, by design, permits detailed studies of nondipolar angular distribution effects in gas-phase photoemission
Strain dependence of bonding and hybridization across the metal-insulator transition of VO2
Soft x-ray spectroscopy is used to investigate the strain dependence of the
metal-insulator transition of VO2. Changes in the strength of the V 3d - O 2p
hybridization are observed across the transition, and are linked to the
structural distortion. Furthermore, although the V-V dimerization is
well-described by dynamical mean-field theory, the V-O hybridization is found
to have an unexpectedly strong dependence on strain that is not predicted by
band theory, emphasizing the relevance of the O ion to the physics of VO2
First Results from the High-Brightness X-Ray Spectroscopy Beamline 9.3.1 at ALS
Beamline 9.3.1 at the Advanced Light Source (ALS) is a windowless beamline, covering the 1–6 keV photon energy range. This beamline is designed to achieve the goal of high brightness at the sample for use in the x‐ray atomic and molecular spectroscopy (XAMS) science, surface and interface science, biology and x‐ray optical development programs at ALS. X‐ray absorption and time‐of‐flight photoemission measurements in 2–5 keV photon energy range along with the flux, resolution, spot size and stability of the beamline will be discussed. Prospects for future XAMS measurements will also be presented
The structural and magnetic properties of (In1-xFex)2O3 (0.0 <= x <= 0.25) system : prepared by gel combustion method
(In1-xFex)2O3 polycrystalline samples with x = (0.0, 0.05, 0.10, 0.15, 0.20
and 0.25) have been synthesized by a gel combustion method. Reitveld refinement
analysis of X raydiffraction data indicated the formation of single phase cubic
bixbyite structure without any parasitic phases. This observation is further
confirmed by high resolution transmission electron microscopy (HRTEM) imaging,
and indexing of the selected-area electron diffraction (SAED) patterns, X-ray
Absorption Spectroscopy (XAS) and Raman Spectroscopy. DC Magnetization studies
as a function of temperature and field indicatethat they are ferromagnetic with
Curie temperature (TC) well above room temperature.Comment: 9 pages 3 figure
Electric-octupole and pure-electric-quadrupole effects in soft-x-ray photoemission
Second-order [O(k^2), k=omega/c] nondipole effects in soft-x-ray
photoemission are demonstrated via an experimental and theoretical study of
angular distributions of neon valence photoelectrons in the 100--1200 eV
photon-energy range. A newly derived theoretical expression for nondipolar
angular distributions characterizes the second-order effects using four new
parameters with primary contributions from pure-quadrupole and octupole-dipole
interference terms. Independent-particle calculations of these parameters
account for a significant portion of the existing discrepancy between
experiment and theory for Ne 2p first-order nondipole parameters.Comment: 4 pages, 3 figure
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