Optimized pulse sequences for suppressing unwanted transitions in quantum systems

We investigate the nature of the pulse sequence so that unwanted transitions in quantum systems can be inhibited optimally. For this purpose we show that the sequence of pulses proposed by Uhrig [Phys. Rev. Lett. \textbf{98}, 100504 (2007)] in the context of inhibition of environmental dephasing effects is optimal. We derive exact results for inhibiting the transitions and confirm the results numerically. We posit a very significant improvement by usage of the Uhrig sequence over an equidistant sequence in decoupling a quantum system from unwanted transitions. The physics of inhibition is the destructive interference between transition amplitudes before and after each pulse.Comment: 5 figure

A rate equation approach to cavity mediated laser cooling

The cooling rate for cavity mediated laser cooling scales as the Lamb-Dicke parameter eta squared. A proper analysis of the cooling process hence needs to take terms up to eta^2 in the system dynamics into account. In this paper, we present such an analysis for a standard scenario of cavity mediated laser cooling with eta << 1. Our results confirm that there are many similarities between ordinary and cavity mediated laser cooling. However, for a weakly confined particle inside a strongly coupled cavity, which is the most interesting case for the cooling of molecules, numerical results indicate that even more detailed calculations are needed to model the cooling process accurately.Comment: 15 pages, 10 figures, minor corrections, PRA (in press

Loss-Induced Limits to Phase Measurement Precision with Maximally Entangled States

The presence of loss limits the precision of an approach to phase measurement using maximally entangled states, also referred to as NOON states. A calculation using a simple beam-splitter model of loss shows that, for all nonzero values L of the loss, phase measurement precision degrades with increasing number N of entangled photons for N sufficiently large. For L above a critical value of approximately 0.785, phase measurement precision degrades with increasing N for all values of N. For L near zero, phase measurement precision improves with increasing N down to a limiting precision of approximately 1.018 L radians, attained at N approximately equal to 2.218/L, and degrades as N increases beyond this value. Phase measurement precision with multiple measurements and a fixed total number of photons N_T is also examined. For L above a critical value of approximately 0.586, the ratio of phase measurement precision attainable with NOON states to that attainable by conventional methods using unentangled coherent states degrades with increasing N, the number of entangled photons employed in a single measurement, for all values of N. For L near zero this ratio is optimized by using approximately N=1.279/L entangled photons in each measurement, yielding a precision of approximately 1.340 sqrt(L/N_T) radians.Comment: Additional references include

Vacuum state truncation via the quantum Zeno effect

In the context of quantum state engineering we analyze the effect of observation on nonlinear optical $n$-photon Fock state generation. We show that it is possible to truncate the vacuum component from an arbitrary photon number superposition without modifying its remaining parts. In the course of the full dynamical analysis of the effect of observation, it is also found that the Zeno and the anti-Zeno effects repeat periodically. We discuss the close relationship between vacuum state truncation and so-called "interaction-free" measurement.Comment: 4 pages, 2 figures, LaTeX; TeX errors fixe

Concentration and purification of entanglement for qubit systems with ancillary cavity fields

We propose schemes for entanglement concentration and purification for qubit systems encoded in flying atomic pairs. We use a cavity-quantum electrodynamics setting as the paradigmatic scenario within which our proposals can be implemented. Maximally entangled pure states of qubits can be produced as a result of our protocols. In particular, the concentration protocol yields Bell states with the largest achievable theoretical probability while the purification scheme produces arbitrarily pure Bell states. The requirements for the implementation of these protocols are modest, within the state of the art, and we address all necessary steps in two specific set-ups based on experimentally mature microwave technology.Comment: 10 pages, 6 figure

Beam splitting and Hong-Ou-Mandel interference for stored light

Storing and release of a quantum light pulse in a medium of atoms in the tripod configuration are studied. Two complementary sets of control fields are defined, which lead to independent and complete photon release at two stages. The system constitutes a new kind of a flexible beam splitter in which the input and output ports concern photons of the same direction but well separated in time. A new version of Hong-Ou-Mandel interference is discussed.Comment: 8 pages, 3 figure

Generalized Toffoli gates using qudit catalysis

We present quantum networks for a n-qubit controlled gate C^{n-1}(U) which use a higher dimensional (qudit) ancilla as a catalyser. In its simplest form the network has only n two-particle gates (qubit-qudit) -- this is the minimum number of two-body interactions needed to couple all n+1 subsystems (n qubits plus one ancilla). This class of controlled gates includes the generalised Toffoli gate C^{n-1}(X) on n qubits, which plays an important role in several quantum algorithms and error correction. A particular example implementing this model is given by the dispersive limit of a generalised Jaynes-Cummings Hamiltonian of an effective spin-s interacting with a cavity mode.Comment: 5 pages, 3 fig

Generating entanglement of photon-number states with coherent light via cross-Kerr nonlinearity

We propose a scheme for generating entangled states of light fields. This scheme only requires the cross-Kerr nonlinear interaction between coherent light-beams, followed by a homodyne detection. Therefore, this scheme is within the reach of current technology. We study in detail the generation of the entangled states between two modes, and that among three modes. In addition to the Bell states between two modes and the W states among three modes, we find plentiful new kinds of entangled states. Finally, the scheme can be extend to generate the entangled states among more than three modes.Comment: 2 figure

Quantum Cryptography Approaching the Classical Limit

We consider the security of continuous-variable quantum cryptography as we approach the classical-limit, i.e., when the unknown preparation noise at the sender's station becomes significantly noisy or thermal (even by as much as 10,000 times the variance of the vacuum mode). We show that, provided the channel transmission losses do not exceed 50%, the security of quantum cryptography is not dependent on the channel transmission, and is therefore, incredibly robust against significant amounts of excess preparation noise. We extend these results to consider for the first time quantum cryptography at wavelengths considerably longer than optical and find that regions of security still exist all the way down to the microwave.Comment: Letter (4 pages) followed by appendix (4 pages). Updated from published version with some minor correction

Highly-functionalised difluorinated cyclohexane polyols via the Diels–Alder reaction : regiochemical control via the phenylsulfonyl group

A difluorinated dienophile underwent cycloaddition reactions with a range of furans to afford cycloadducts whichcould be processed regio- and stereoselectively via episulfonium ions, generated by the reaction between their alkenyl groups and phenylsulfenyl chloride. The oxabicyclic products were oxidised to the phenylsulfonyl level and ring opened via E1CB or reductive desulfonative pathways to afford, ultimately, difluorinated cyclohexene or cyclohexane polyols