13,573 research outputs found
Geometric-Phase-Effect Tunnel-Splitting Oscillations in Single-Molecule Magnets with Fourth-Order Anisotropy Induced by Orthorhombic Distortion
We analyze the interference between tunneling paths that occurs for a spin
system with both fourth-order and second-order transverse anisotropy. Using an
instanton approach, we find that as the strength of the second-order transverse
anisotropy is increased, the tunnel splitting is modulated, with zeros
occurring periodically. This effect results from the interference of four
tunneling paths connecting easy-axis spin orientations and occurs in the
absence of any magnetic field.Comment: 6 pages, 5 eps figures. Version published in EPL. Expanded from v1:
Appendix added, references added, 1 figure added, others modified
cosmeticall
Oscillatory Tunnel Splittings in Spin Systems: A Discrete Wentzel-Kramers-Brillouin Approach
Certain spin Hamiltonians that give rise to tunnel splittings that are viewed
in terms of interfering instanton trajectories, are restudied using a discrete
WKB method, that is more elementary, and also yields wavefunctions and
preexponential factors for the splittings. A novel turning point inside the
classically forbidden region is analysed, and a general formula is obtained for
the splittings. The result is appled to the \Fe8 system. A previous result for
the oscillation of the ground state splitting with external magnetic field is
extended to higher levels.Comment: RevTex, one ps figur
Large transverse field tunnel splittings in the Fe_8 spin Hamiltonian
The spin Hamiltonian that describes the molecular magnet Fe has biaxial
symmetry with mutually perpendicular easy, medium, and hard magnetic axes.
Previous calculations of the ground state tunnel splittings in the presence of
a magnetic field along the hard axis are extended, and the meaning of the
previously discovered oscillation of this splitting is further clarified
Spin Tunneling in Magnetic Molecules: Quasisingular Perturbations and Discontinuous SU(2) Instantons
Spin coherent state path integrals with discontinuous semiclassical paths are
investigated with special reference to a realistic model for the magnetic
degrees of freedom in the Fe8 molecular solid. It is shown that such paths are
essential to a proper understanding of the phenomenon of quenched spin
tunneling in these molecules. In the Fe8 problem, such paths are shown to arise
as soon as a fourth order anisotropy term in the energy is turned on, making
this term a singular perturbation from the semiclassical point of view. The
instanton approximation is shown to quantitatively explain the magnetic field
dependence of the tunnel splitting, as well as agree with general rules for the
number of quenching points allowed for a given value of spin. An accurate
approximate formula for the spacing between quenching points is derived
Quantum Thermoactivation of Nanoscale Magnets
The integral relaxation time describing the thermoactivated escape of a
uniaxial quantum spin system interacting with a boson bath is calculated
analytically in the whole temperature range. For temperatures T much less than
the barrier height \Delta U, the level quantization near the top of the barrier
and the strong frequency dependence of the one-boson transition probability can
lead to the regularly spaced deep minima of the thermoactivation rate as a
function of the magnetic field applied along the z axis.Comment: 4 pages, no figures, rejected from Phys. Rev. Let
Quenched Spin Tunneling and Diabolical Points in Magnetic Molecules: II. Asymmetric Configurations
The perfect quenching of spin tunneling first predicted for a model with
biaxial symmetry, and recently observed in the magnetic molecule Fe_8, is
further studied using the discrete phase integral (or
Wentzel-Kramers-Brillouin) method. The analysis of the previous paper is
extended to the case where the magnetic field has both hard and easy
components, so that the Hamiltonian has no obvious symmetry. Herring's formula
is now inapplicable, so the problem is solved by finding the wavefunction and
using connection formulas at every turning point. A general formula for the
energy surface in the vicinity of the diabolo is obtained in this way. This
formula gives the tunneling apmplitude between two wells unrelated by symmetry
in terms of a small number of action integrals, and appears to be generally
valid, even for problems where the recursion contains more than five terms.
Explicit results are obtained for the diabolical points in the model for Fe_8.
These results exactly parallel the experimental observations. It is found that
the leading semiclassical results for the diabolical points appear to be exact,
and the points themselves lie on a perfect centered rectangular lattice in the
magnetic field space. A variety of evidence in favor of this perfect lattice
hypothesis is presented.Comment: Revtex; 4 ps figures; follow up to cond-mat/000311
Crystallography of the NiHfSi Phase in a NiAl (0.5 Hf) Single-Crystal Alloy
Small additions of Hf to conventionally processed NiAl single crystals result in the precipitation of a high density of cuboidal G-phase along with a newly identified silicide phase. Both of these phases form in the presence of Si which is not an intentional alloying addition but is a contaminant resulting from contact with the ceramic shell molds during directional solidification of the single-crystal ingots. The morphology, crystal structure and Orientation Relationship (OR) of the silicide phase in a NiAl (0.5 at.%Hf) single-crystal alloy have been determined using transmission electron microscopy, electron microdiffraction and energy dispersive X-ray spectroscopy. Qualitative elemental analysis and indexing of the electron microdiffraction patterns from the new phase indicate that it is an orthorhombic NiHfSi phase with unit cell parameters, a = 0.639 nm, b = 0.389 nm and c = 0.72 nm, and space group Pnma. The NiHfSi phase forms as thin rectangular plates on NiAl/111/ planes with an OR that is given by NiHfSi(100))(parallel) NiAl(111) and NiHfSi zone axes(010) (parallel) NiAl zone axes (101). Twelve variants of the NiHfSi phase were observed in the alloy and the number of variants and rectangular morphology of NiHfSi plates are consistent with symmetry requirements. Quenching experiments indicate that nucleation of the NiHfSi phase in NiAI(Hf) alloys is aided by the formation of NiAl group of zone axes (111) vacancy loops that form on the NiAl /111/ planes
Quantum Lightning Never Strikes the Same State Twice
Public key quantum money can be seen as a version of the quantum no-cloning
theorem that holds even when the quantum states can be verified by the
adversary. In this work, investigate quantum lightning, a formalization of
"collision-free quantum money" defined by Lutomirski et al. [ICS'10], where
no-cloning holds even when the adversary herself generates the quantum state to
be cloned. We then study quantum money and quantum lightning, showing the
following results:
- We demonstrate the usefulness of quantum lightning by showing several
potential applications, such as generating random strings with a proof of
entropy, to completely decentralized cryptocurrency without a block-chain,
where transactions is instant and local.
- We give win-win results for quantum money/lightning, showing that either
signatures/hash functions/commitment schemes meet very strong recently proposed
notions of security, or they yield quantum money or lightning.
- We construct quantum lightning under the assumed multi-collision resistance
of random degree-2 systems of polynomials.
- We show that instantiating the quantum money scheme of Aaronson and
Christiano [STOC'12] with indistinguishability obfuscation that is secure
against quantum computers yields a secure quantum money schem
Inverse problem for the Landau-Zener effect
We consider the inverse Landau-Zener problem which consists in finding the
energy-sweep functions W(t)=E1(t)-E2(t) resulting in the required time
dependences of the level populations for a two-level system crossing the
resonance one or more times during the sweep. We find sweep functions of
particular forms that let manipulate the system in a required way, including
complete switching from the state 1 to the state 2 and preparing the system at
the exact ground and excited states at resonance.Comment: 7 EPL pages, 6 figure
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