Plasma Dynamics Characterization for Improvement of Resonantly Enhanced Harmonics Generation in Indium and Tin Laser-Produced Plasmas

R.A.G. is grateful to H. Kuroda for providing the access to the laser facility. As a Center of Excellence, the Institute of Solid State Physics at the University of Latvia received funding from the European Union’s Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement no. 739508, project CAMART².In this study, we characterize the properties of indium and tin laser-induced plasmas responsible for efficient high-order harmonics generation of the ultrashort pulses propagating through these media. The optimally formed plasma was determined using the analysis of the time-resolved variations in the spectral and morphological features of spreading indium and tin plasma components under different regimes of laser ablation. We report the measurements of plasma velocities under different regimes of ablation and correlate them with the optimal delay between the heating and probe laser pulses for the generation of harmonics with the highest yield. Electron temperatures and densities are determined using the integrated and time-resolved spectral measurements of plasmas. The resonance-enhanced harmonics are compared with other harmonics from the point of view of the modulation of plasma characteristics. The harmonics of 800 and 1200–2200 nm lasers and their second-harmonic fields were analyzed at optimal conditions of Sn and In plasma formation. The novelty of this work is the implementation of the diagnostics of the dynamics of plasma characteristics for the determination of the optimal plasma formation for harmonics generation. Such an approach allows for the demonstration of the maximal harmonic yield from the studied plasma and the definition of the various resonance-induced harmonic generation conditions. © 2022 by the authors.European Regional Development Fund (1.1.1.5/19/A/003); Institute of Solid-State Physics, University of Latvia has received funding from the European Union's Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-Teaming Phase 2 under grant agreement No. 739508, project CAMART2

Variation of Nonlinear Refraction and Three-Photon Absorption of Indium–Tin Oxide Quantum Dot Thin Films and Solutions in Near Infrared Range

Authors acknowledge the support of J. Grube and A. Sarakovskis in providing the laser facility for these studies. Institute of Solid State Physics, University of Latvia as the Center of Excellence has received funding from the European Union’s Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2.We characterize the nonlinear optical properties of indium–tin oxide (ITO) quantum dots (QDs) in the IR range using the Z-scan method. We present results of three-photon absorption (3PA), third harmonic generation (3HG), and Kerr-effect-induced nonlinear refraction in ITO QDs. Z-scan measurements were carried out for the QDs solution, while 3HG was demonstrated using QD thin films. The Kerr-induced nonlinear refractive index was analyzed along the 800–950 nm range showing an increase in this parameter from −6.7 × 10−18 to −1.5 × 10−17 m2 W−1. At longer wavelengths (1000–1100 nm), the higher-order effects started to contribute to a nonlinear refractive index. The 3PA coefficient at 950 nm was measured to be 1.42 × 10−25 m3/W2. We discuss the peculiarities in the wavelength-dependent variation of the coefficient of nonlinear absorption responsible for 3PA in the range of 800–1150 nm. Third harmonic generation was analyzed in the 1200–1550 nm spectral range. The absolute value of 3HG conversion efficiency in the 150 nm thick film at the wavelength of laser radiation (1350 nm) was estimated to be ~10–5. --//-- This is an open access article Bundulis, A.; Berzina, A.; Kim, V.V.; Polyakov, B.; Novikovs, A.; Ganeev, R.A. Variation of Nonlinear Refraction and Three-Photon Absorption of Indium–Tin Oxide Quantum Dot Thin Films and Solutions in Near Infrared Range. Nanomaterials 2023, 13, 2320. https://doi.org/10.3390/nano13162320 published under the CC BY 4.0 licence.Institute of Solid State Physics, University of Latvia as the Center of Excellence has received funding from the European Union’s Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2

High-order harmonics generation in Cd and Pd laser-induced plasmas

R.A.G. is grateful to H. Kuroda for providing access to the laser facility. Institute of Solid State Physics, University of Latvia as the Center of Excellence has received funding from the European Union's Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2.We demonstrate the generation of high-order harmonics of laser pulses in palladium and cadmium plasmas. We adjusted the wavelength of driving pulses to investigate the resonance enhancement in different ranges of extreme ultraviolet region. The summation of incommensurate waves during the two-color pump of Pd and Cd plasmas allowed the generation of a broader range of harmonics. The theoretical aspects of the two-color pump of the laser-induced plasma are discussed. © 2023 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement --//-- This is an open access article Rashid A. Ganeev, Vyacheslav V. Kim, Jelena Butikova, Aigars Atvars, Jurgis Grube, Anatolijs Sarakovskis, and Arnolds Ubelis, "High-order harmonics generation in Cd and Pd laser-induced plasmas," Opt. Express 31, 26626-26642 (2023), https://doi.org/10.1364/OE.493754 published under the CC BY 4.0 licence.European Regional Development Fund (1.1.1.5/19/A/003); World Bank Project (REP-04032022-206).Institute of Solid State Physics, University of Latvia as the Center of Excellence has received funding from the European Union's Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2

Nonlinear absorption and refraction of picosecond and femtosecond pulses in HgTe quantum dot films

We report measurements of the saturated intensities, saturable absorption, and nonlinear refraction in 70-nm thick films containing 4 nm HgTe quantum dots. We demonstrate strong nonlinear refraction and saturable absorption in the thin films using tunable picosecond and femtosecond pulses. Studies were carried out using tunable laser pulses in the range of 400–1100 nm. A significant variation of the nonlinear refraction along this spectral range was demonstrated. The maximal values of the nonlinear absorption coefficients and nonlinear refractive indices determined within the studied wavelength range were −2.4 × 10−5 cm2 W−1 (in the case of 28 ps, 700 nm probe pulses) and −3 × 10−9 cm2 W−1 (in the case of 28 ps, 400 nm probe pulses), respectively. Our studies show that HgTe quantum dots can be used in different fields e.g., as efficient emitters of high-order harmonics of ultrashort laser pulses or as laser mode-lockers. © 2021 by the authors. Licensee MDPI, Basel, Switzerland. Published under the CC BY 4.0 license.European Regional Development Fund (1.1.1.5/19/A/003), Latvian Council of Sciences (lzp-2020/2-0238). Institute of Solid State Physics, University of Latvia as the Center of Excellence acknowledges funding from the European Union's Horizon 2020 Framework Programme H2020-WIDESPREAD-01-2016-2017-TeamingPhase2 under grant agreement No. 739508, project CAMART2

Laser-surface interactions

This book is about the interaction of laser radiation with various surfaces at variable parameters of radiation. As a basic principle of classification we chose the energetic or intensity level of interaction of laser radiation with the surfaces. These two characteristics of laser radiation are the most important parameters defining entire spectrum of the processes occurring on the surfaces during interaction with electromagnetic waves. This is a first book containing a whole spectrum of the laser-surface interactions distinguished by the ranges of used laser intensity. It combines the surface response starting from extremely weak laser intensities (~1 W cm-2) up to the relativistic intensities (~1020 W cm-2 and higher). The book provides the basic information about lasers and acquaints the reader with both common applications of laser-surface interactions (laser-related printers, scanners, barcode readers, discs, material processing, military, holography, medicine, etc) and unusual uses of the processes on the surfaces under the action of lasers (art conservation, rangefinders and velocimeters, space and earth explorations, surface engineering and ablation, and others). The scientific applications of laser-surfaces interactions (surface optical nonlinearities, surface enhanced Raman spectroscopy, surface nanostructuring, nanoripples and clusters formation, X-ray lasers and harmonic generation from the surfaces) are discussed from the point of view of the close relations between the properties of surface and matter, which is a cornerstone of most of studies of materials. The novelty of the approach developed in Laser - Surface Interactions is related with the interconnection of scientific studies with numerous applications of the laser-surface interactions separated in different chapters by the ranges of laser intensities. We present most recent achievements in this field. The book provides valuable information for different ranges of reader's preparedness to the laser-related topics (from unprepared readers, to students, engineers and researchers, professionals and academics)

Laser-Induced Molecular Plasma: A Medium for High-Order Harmonics Generation of Ultrashort Pulses

I present a study of laser-induced plasmas (LIPs) produced on the surfaces of molecular targets to create optimal conditions for high-order harmonics generation during the propagation of femtosecond pulses through the LIP. The resonance enhancement of a harmonic, two-color pump of plasma, quasi-phase-matching and nanoparticle-induced growth of the harmonic yield are analyzed, which allows for the formation of sources of coherent extreme ultraviolet radiation based on molecular plasma formation

High-order harmonics enhancement in laser-induced plasma

Abstract The methods of enhancement of the strong high-order harmonics of femtosecond pulses in laser-induced plasma are demonstrated. It comprises the application of the four techniques allowing the enhancement of harmonics in different spectral ranges. Among them are the selection of targets for ablation to create the conditions for resonance enhancement of single harmonic, formation of the quasi-phase-matching of a spectrally tunable group of harmonics, application of the two-color pump of plasma, and the formation of nanoparticles-contained plasmas. The number of generated coherent XUV photons increased in the region of single resonantly enhanced harmonic (62 nm) and the shorter-wavelength region (30–50 nm). The above techniques of harmonics enhancement allowed a significant (up to 50 times) growth in a whole harmonic yield in the case of indium plasma. We discuss the reasons preventing the joint implementation of the four methods of harmonics enhancement in the same spectral region

Plasma harmonics

Preface; Why plasma harmonics? A very brief introduction Early stage of plasma harmonic studies - hopes and frustrations New developments in plasma harmonics studies: first successes Improvements of plasma harmonics; Theoretical basics of plasma harmonics; Basics of HHG Harmonic generation in fullerenes using few-cycle pulsesVarious approaches for description of observed peculiarities of resonant enhancement of a single harmonic in laser plasmaTwo-colour pump resonance-induced enhancement of odd and even harmonics from a tin plasmaCalculations of single harmonic generation from Mn plasma;Low-