Novel substrates for Helium adsorption: Graphane and Graphene-Fluoride

The discovery of fullerenes has stimulated extensive exploration of the resulting behavior of adsorbed films. Our study addresses the planar substrates graphene-fluoride (GF) and graphane (GH) in comparison to graphene. We present initial results concerning the potential energy, energy bands and low density behavior of 4He and 3He films on such different surfaces. For example, while graphene presents an adsorption potential that is qualitatively similar to that on graphite, GF and GH yield potentials with different symmetry, a number of adsorption sites double that on graphene/graphite and a larger corrugation for the adatom. In the case of GF, the lowest energy band width is similar to that on graphite but the He atom has a significantly larger effective mass and the adsorption energy is about three time that on graphite. Implications concerning the monolayer phase diagram of 4He are explored with the exact path integral ground state method. A commensurate ordered state similar to the sqrt{3} x sqrt{3} R30^o state on graphite is found the be unstable both on GF and on GH. The ground states of submonolayer 4He on both GF and GH are superfluids with a Bose Einstein condensate fraction of about 10%.Comment: 6 pages, 3 figures, LT26 proceedings, accepted for publication in Journal of Physics: Conference Serie

Bose-Einstein Condensation at a Helium Surface

Path Integral Monte Carlo was used to calculate the Bose-Einstein condensate fraction at the surface of a helium film at $T=0.77 K$, as a function of density. Moving from the center of the slab to the surface, the condensate fraction was found to initially increase with decreasing density to a maximum value of 0.9 before decreasing. Long wavelength density correlations were observed in the static structure factor at the surface of the slab. Finally, a surface dispersion relation was calculated from imaginary-time density-density correlations.Comment: 8 pages, 5 figure

Analysis of the IBEX-Lo interstellar hydrogen fluxes collected in 2009–2018 as a tool for sensing of the solar radiation pressure and the hydrogen ionization rate

The Interstellar Boundary Explorer (IBEX) has been measuring interstellar hydrogen fluxes at 1 au since 2009. In this paper,we analysed all available data obtained with the IBEX-Lo instrument at energies 11–41 eV using our numerical kinetic modelof the interstellar hydrogen distribution in the heliosphere. We performed a fitting of the data to find independently the modelparameters: the ratio of the solar radiation pressure to the solar gravitation (μ0), ionization rate of hydrogen atoms at 1 au(β0), parameters of the secondary interstellar atoms at 70 au from the Sun, which provide the best agreement with the data byminimization of metricχ2. We also analysed temporal variations of the ratio of the fluxes measured in a fixed direction at energybin 1 and energy bin 2. It is found that in 2009–2011 and 2017–2016 the ratio provided by the model is smaller than in the IBEX-Lo data, while in 2012–2015, oppositely, the model ratio is larger compared to the data. This might be caused by the incorrectseparation of the measured fluxes between energy channels in the data, or by some additional physical factors that are omitted inthe model. Understanding this issue may be important for the preparation of future Interstellar Mapping and Acceleration Probemission. At this stage, we relied on the sum of the fluxes measured in energy bins 1 and 2 for comparison to model predictions

Study of solid 4He in two dimensions. The issue of zero-point defects and study of confined crystal

Defects are believed to play a fundamental role in the supersolid state of 4He. We report on studies by exact Quantum Monte Carlo (QMC) simulations at zero temperature of the properties of solid 4He in presence of many vacancies, up to 30 in two dimensions (2D). In all studied cases the crystalline order is stable at least as long as the concentration of vacancies is below 2.5%. In the 2D system for a small number, n_v, of vacancies such defects can be identified in the crystalline lattice and are strongly correlated with an attractive interaction. On the contrary when n_v~10 vacancies in the relaxed system disappear and in their place one finds dislocations and a revival of the Bose-Einstein condensation. Thus, should zero-point motion defects be present in solid 4He, such defects would be dislocations and not vacancies, at least in 2D. In order to avoid using periodic boundary conditions we have studied the exact ground state of solid 4He confined in a circular region by an external potential. We find that defects tend to be localized in an interfacial region of width of about 15 A. Our computation allows to put as upper bound limit to zero--point defects the concentration 0.003 in the 2D system close to melting density.Comment: 17 pages, accepted for publication in J. Low Temp. Phys., Special Issue on Supersolid

Toward accurate CO_2 and CH_4 observations from GOSAT

The column-average dry air mole fractions of atmospheric carbon dioxide and methane (X_(CO_2) and X_(CH_4)) are inferred from observations of backscattered sunlight conducted by the Greenhouse gases Observing SATellite (GOSAT). Comparing the first year of GOSAT retrievals over land with colocated ground-based observations of the Total Carbon Column Observing Network (TCCON), we find an average difference (bias) of −0.05% and −0.30% for X_(CO_2) and X_(CH_4) with a station-to-station variability (standard deviation of the bias) of 0.37% and 0.26% among the 6 considered TCCON sites. The root-mean square deviation of the bias-corrected satellite retrievals from colocated TCCON observations amounts to 2.8 ppm for X_(CO_2) and 0.015 ppm for X_(CH_4). Without any data averaging, the GOSAT records reproduce general source/sink patterns such as the seasonal cycle of X_(CO_2) suggesting the use of the satellite retrievals for constraining surface fluxes

The downwind hemisphere of the heliosphere: Eight years of IBEX-Lo observations

We present a comprehensive study of energetic neutral atoms (ENAs) of 10 eV to 2.5 keV from the downwind hemisphere of the heliosphere. These ENAs are believed to originate mostly from pickup protons and solar wind protons in the inner heliosheath. This study includes all low-energy observations made with the Interstellar Boundary Explorer over the first 8 years. Since the protons around 0.1 keV dominate the plasma pressure in the inner heliosheath in downwind direction, these ENA observations offer the unique opportunity to constrain the plasma properties and dimensions of the heliosheath where no in-situ observations are available. We first derive energy spectra of ENA intensities averaged over time for 49 macropixels covering the entire downwind hemisphere. The results confirm previous studies regarding integral intensities and the roll-over around 0.1 keV energy. With the expanded dataset we now find that ENA intensities at 0.2 and 0.1 keV seem to anti-correlate with solar activity. We then derive the product of total plasma pressure and emission thickness of protons in the heliosheath to estimate lower limits on the thickness of the inner heliosheath. The temporally averaged ENA intensities support a rather spherical shape of the termination shock and a heliosheath thickness between 150 and 210 au for most regions of the downwind hemisphere. Around the nominal downwind direction of 76{\deg} ecliptic longitude, the heliosheath is at least 280 au thick. There, the neutral hydrogen density seems to be depleted compared to upwind directions by roughly a factor of 2.Comment: Preprint of article in The Astrophysical Journa

Protostellar Collapse with Various Metallicities

The thermal and chemical evolution of gravitationally collapsing protostellar clouds is investigated, focusing attention on their dependence on metallicity. Calculations are carried out for a range of metallicities spanning the local interstellar value to zero. During the time when clouds are transparent to continuous radiation, the temperatures are higher for those with lower metallicity, reflecting lower radiative ability. However, once the clouds become opaque, in the course of the adiabatic contraction of the transient cores, their evolutionary trajectories in the density-temperature plane converge to a unique curve that is determined by only physical constants. The trajectories coincide with each other thereafter. Consequently, the size of the stellar core at the formation is the same regardless of the gas composition of the parent cloud.Comment: 30 pages. The Astrophysical Journal, 533, in pres

The Minimum Stellar Mass in Early Galaxies

The conditions for the fragmentation of the baryonic component during merging of dark matter halos in the early Universe are studied. We assume that the baryonic component undergoes a shock compression. The characteristic masses of protostellar molecular clouds and the minimum masses of protostars formed in these clouds decrease with increasing halo mass. This may indicate that the initial stellar mass function in more massive galaxies was shifted towards lower masses during the initial stages of their formation. This would result in an increase of the number of stars per unit halo mass, i.e., the efficiency of star formation.Comment: 18 pages, 7 figure

Solid 4He and the Supersolid Phase: from Theoretical Speculation to the Discovery of a New State of Matter? A Review of the Past and Present Status of Research

The possibility of a supersolid state of matter, i.e., a crystalline solid exhibiting superfluid properties, first appeared in theoretical studies about forty years ago. After a long period of little interest due to the lack of experimental evidence, it has attracted strong experimental and theoretical attention in the last few years since Kim and Chan (Penn State, USA) reported evidence for nonclassical rotational inertia effects, a typical signature of superfluidity, in samples of solid 4He. Since this "first observation", other experimental groups have observed such effects in the response to the rotation of samples of crystalline helium, and it has become clear that the response of the solid is extremely sensitive to growth conditions, annealing processes, and 3He impurities. A peak in the specific heat in the same range of temperatures has been reported as well as anomalies in the elastic behaviour of solid 4He with a strong resemblance to the phenomena revealed by torsional oscillator experiments. Very recently, the observation of unusual mass transport in hcp solid 4He has also been reported, suggesting superflow. From the theoretical point of view, powerful simulation methods have been used to study solid 4He, but the interpretation of the data is still rather difficult; dealing with the question of supersolidity means that one has to face not only the problem of the coexistence of quantum coherence phenomena and crystalline order, exploring the realm of spontaneous symmetry breaking and quantum field theory, but also the problem of the role of disorder, i.e., how defects, such as vacancies, impurities, dislocations, and grain boundaries, participate in the phase transition mechanism.Comment: Published on J. Phys. Soc. Jpn., Vol.77, No.11, p.11101

The impact of spectral resolution on satellite retrieval accuracy of CO_2 and CH_4

The Fourier-transform spectrometer on board the Japanese GOSAT (Greenhouse gases Observing SATellite) satellite offers an excellent opportunity to study the impact of instrument resolution on retrieval accuracy of CO_2 and CH_4. This is relevant to further improve retrieval accuracy and to optimize the cost–benefit ratio of future satellite missions for the remote sensing of greenhouse gases. To address this question, we degrade GOSAT measurements with a spectral resolution of ≈ 0.24 cm^(−1) step by step to a resolution of 1.5 cm^(−1). We examine the results by comparing relative differences at various resolutions, by referring the results to reference values from the Total Carbon Column Observing Network (TCCON), and by calculating and inverting synthetic spectra for which the true CO_2 and CH_4 columns are known. The main impacts of degrading the spectral resolution are reproduced for all approaches based on GOSAT measurements; pure forward model errors identified with simulated measurements are much smaller. For GOSAT spectra, the most notable effect on CO_2 retrieval accuracy is the increase of the standard deviation of retrieval errors from 0.7 to 1.0% when the spectral resolution is reduced by a factor of six. The retrieval biases against atmospheric water abundance and air mass become stronger with decreasing resolution. The error scatter increase for CH_4 columns is less pronounced. The selective degradation of single spectral windows demonstrates that the retrieval accuracy of CO_2 and CH_4 is dominated by the spectral range where the absorption lines of the target molecule are located. For both GOSAT and synthetic measurements, retrieval accuracy decreases with lower spectral resolution for a given signal-to-noise ratio, suggesting increasing interference errors