19 research outputs found
SDW and FISDW transition of (TMTSF)ClO at high magnetic fields
The magnetic field dependence of the SDW transition in (TMTSF)ClO for
various anion cooling rates has been measured, with the field up to 27T
parallel to the lowest conductivity direction . For quenched
(TMTSF)ClO, the SDW transition temperature increases
from 4.5K in zero field up to 8.4K at 27T. A quadratic behavior is observed
below 18T, followed by a saturation behavior. These results are consistent with
the prediction of the mean-field theory. From these behaviors,
is estimated as =13.5K for the perfect nesting case. This
indicates that the SDW phase in quenched (TMTSF)ClO, where is less than 6K, is strongly suppressed by the two-dimensionality of
the system. In the intermediate cooled state in which the SDW phase does not
appear in zero field, the transition temperature for the field-induced SDW
shows a quadratic behavior above 12T and there is no saturation behavior even
at 27T, in contrast to the FISDW phase in the relaxed state. This behavior can
probably be attributed to the difference of the dimerized gap due to anion
ordering.Comment: 4pages,5figures(EPS), accepted for publication in PR
Spin-density-wave transition of (TMTSF)PF at high magnetic fields
The transverse magnetoresistance of the Bechgaard salt (TMTSF)PF has
been measured for various pressures, with the field up to 24 T parallel to the
lowest conductivity direction c. A quadratic behavior is observed in
the magnetic field dependence of the spin-density-wave (SDW) transition
temperature . With increasing pressure,
decreases and the coefficient of the quadratic term increases. These results
are consistent with the prediction of the mean-field theory based on the
nesting of the quasi one-dimensional Fermi surface. Using a mean field theory,
for the perfect nesting case is estimated as about 16 K. This
means that even at ambient pressure where is 12 K, the SDW
phase of (TMTSF)PF is substantially suppressed by the
two-dimensionality of the system.Comment: 11pages,6figures(EPS), accepted for publication in PR
Periodic orbit resonances in layered metals in tilted magnetic fields
The frequency dependence of the interlayer conductivity of a layered Fermi
liquid in a magnetic field which is tilted away from the normal to the layers
is considered. For both quasi-one- and quasi-two-dimensional systems resonances
occur when the frequency is a harmonic of the frequency at which the magnetic
field causes the electrons to oscillate on the Fermi surface within the layers.
The intensity of the different harmonic resonances varies significantly with
the direction of the field. The resonances occur for both coherent and weakly
incoherent interlayer transport and so their observation does not imply the
existence of a three-dimensional Fermi surface.Comment: 4 pages, RevTeX + epsf, 2 figures. Discussion of other work revised.
To appear in Phys. Rev. B, Rapid Commun., October 1
Determination of the Fermi Velocity by Angle-dependent Periodic Orbit Resonance Measurements in the Organic Conductor alpha-(BEDT-TTF)2KHg(SCN)4
We report detailed angle-dependent studies of the microwave (f=50 to 90 GHz)
interlayer magneto-electrodynamics of a single crystal sample of the organic
charge-density-wave (CDW) conductor alpha-(BEDT-TTF)2KHg(SCN)4. Recently
developed instrumentation enables both magnetic field (B) sweeps for a fixed
sample orientation and, for the first time, angle sweeps at fixed f/B. We
observe series' of resonant absorptions which we attribute to periodic orbit
resonances (POR) - a phenomenon closely related to cyclotron resonance. The
angle dependence of the POR indicate that they are associated with the low
temperature quasi-one-dimensional (Q1D) Fermi surface (FS) of the title
compound; indeed, all of the resonance peaks collapse beautifully onto a single
set of f/B versus angle curves, generated using a semiclassical
magneto-transport theory for a single Q1D FS. We show that Q1D POR measurements
provide one of the most direct methods for determining the Fermi velocity,
without any detailed assumptions concerning the bandstructure; our analysis
yields an average value of v_F=6.5x10^4 m/s. Quantitative analysis of the POR
harmonic content indicates that the Q1D FS is strongly corrugated. This is
consistent with the assumption that the low-temperature FS derives from a
reconstruction of the high temperature quasi-two-dimensional FS, caused by the
CDW instability. Detailed analysis of the angle dependence of the POR yields
parameters associated with the CDW superstructure which are consistent with
published results. Finally, we address the issue as to whether or not the
interlayer electrodynamics are coherent in the title compound.Comment: 28 pages, including 6 figures. Submitted to PR
Orbital quantization in the high magnetic field state of a charge-density-wave system
A superposition of the Pauli and orbital coupling of a high magnetic field to
charge carriers in a charge-density-wave (CDW) system is proposed to give rise
to transitions between subphases with quantized values of the CDW wavevector.
By contrast to the purely orbital field-induced density-wave effects which
require a strongly imperfect nesting of the Fermi surface, the new transitions
can occur even if the Fermi surface is well nested at zero field. We suggest
that such transitions are observed in the organic metal
-(BEDT-TTF)KHg(SCN) under a strongly tilted magnetic field.Comment: 14 pages including 4 figure
Coherent vs incoherent interlayer transport in layered metals
The magnetic-field, temperature, and angular dependence of the interlayer
magnetoresistance of two different quasi-two-dimensional (2D) organic
superconductors is reported. For -(BEDT-TTF)I we find a
well-resolved peak in the angle-dependent magnetoresistance at (field parallel to the layers). This clear-cut proof for the coherent
nature of the interlayer transport is absent for
''-(BEDT-TTF)SFCHCFSO. This and the non-metallic
behavior of the magnetoresistance suggest an incoherent quasiparticle motion
for the latter 2D metal.Comment: 4 pages, 4 figures. Phys. Rev. B, in pres
Coexistence or Separation of the Superconducting, Antiferromagnetic, and Paramagnetic Phases in Quasi One-Dimensional (TMTSF)2PF6 ?
We report on experimental studies of the character of phase transitions in
the quasi-1D organic compound (TMTSF)2PF6 in the close vicinity of the borders
between the paramagnetic metal PM, antiferromagnetic insulator AF, and
superconducting SC states. In order to drive the system through the phase
border P_0(T_0), the sample was maintained at fixed temperature T and pressure
P, whereas the critical pressure P_0 was tuned by applying the magnetic field
B. In this approach, the magnetic field was used (i) for tuning (P-P_0), and
(ii) for identifying the phase composition (due to qualitatively different
magnetoresistance behavior in different phases). Experimentally, we measured
R(B) and its temperature dependence R(B,T) in the pressure range (0 - 1)GPa.
Our studies focus on the features of the magnetoresistance at the phase
transition between the PM and AF phases, in the close vicinity to the
superconducting transition at T~1K. We found pronounced history effects arising
when the AF/PM phase border is crossed by sweeping the magnetic field: the
resistance depends on a trajectory which the system arrives at a given point of
the P-B-T phase space. In the transition from the PM to AF phase, the features
of the PM phase extends well into the AF phase. At the opposite transition from
the AF to PM phase, the features of the AF phase are observed in the PM phase.
These results evidence for a macroscopically inhomogeneous state, which
contains macroscopic inclusions of the minority phase. When the system is
driven away from the transition, the homogeneous state is restored; upon a
return motion to the phase boundary, no signatures of the minority phase are
observed up to the very phase boundary.Comment: 10 figures, 23 page
Larkin-Ovchinnikov-Fulde-Ferrell state in quasi-one-dimensional superconductors
The properties of a quasi-one-dimensional (quasi-1D) superconductor with {\it
an open Fermi surface} are expected to be unusual in a magnetic field. On the
one hand, the quasi-1D structure of the Fermi surface strongly favors the
formation of a non-uniform state (Larkin-Ovchinnikov-Fulde-Ferrell (LOFF)
state) in the presence of a magnetic field acting on the electron spins. On the
other hand, a magnetic field acting on an open Fermi surface induces a
dimensional crossover by confining the electronic wave-functions wave-functions
along the chains of highest conductivity, which results in a divergence of the
orbital critical field and in a stabilization at low temperature of a cascade
of superconducting phases separated by first order transistions. In this paper,
we study the phase diagram as a function of the anisotropy. We discuss in
details the experimental situation in the quasi-1D organic conductors of the
Bechgaard salts family and argue that they appear as good candidates for the
observation of the LOFF state, provided that their anisotropy is large enough.
Recent experiments on the organic quasi-1D superconductor (TMTSF)ClO
are in agreement with the results obtained in this paper and could be
interpreted as a signature of a high-field superconducting phase. We also point
out the possibility to observe a LOFF state in some quasi-2D organic
superconductors.Comment: 24 pages+17 figures (upon request), RevTex, ORSAY-LPS-24109
Magnetic field-dependent interplay between incoherent and Fermi liquid transport mechanisms in low-dimensional tau phase organic conductors
We present an electrical transport study of the 2-dimensional (2D) organic
conductor tau-(P-(S,S)-DMEDT-TTF)_2(AuBr)_2(AuBr_2)_y (y = 0.75) at low
temperatures and high magnetic fields. The inter-plane resistivity rho_zz
increases with decreasing temperature, with the exception of a slight anomaly
at 12 K. Under a magnetic field B, both rho_zz and the in-plane resistivity
plane rho_xx show a pronounced negative and hysteretic magnetoresistance with
Shubnikov de Haas (SdH)oscillations being observed in some (high
quality)samples above 15 T. Contrary to the predicted single, star-shaped,
closed orbit Fermi surface from band structure calculations (with an expected
approximate area of 12.5% of A_FBZ), two fundamental frequencies F_l and F_h
are detected in the SdH signal. These orbits correspond to 2.4% and 6.8% of the
area of the first Brillouin zone(A_FBZ), with effective masses F_l = 4.0 +/-
0.5 and F_h = 7.3 +/- 0.1. The angular dependence, in tilted magnetic fields of
F_l and F_h, reveals the 2D character of the FS and Angular dependent
magnetoresistance (AMRO) further suggests a FS which is strictly 2-D where the
inter-plane hopping t_c is virtually absent or incoherent. The Hall constant
R_xy is field independent, and the Hall mobility increases by a factor of 3
under moderate magnetic fields. Our observations suggest a unique physical
situation where a stable 2D Fermi liquid state in the molecular layers are
incoherently coupled along the least conducting direction. The magnetic field
not only reduces the inelastic scattering between the 2D metallic layers, but
it also reveals the incoherent nature of interplane transport in the AMRO
spectrum. The apparent ferromagnetism of the hysteretic magnetoresistance
remains an unsolved problem.Comment: 33 pages, 11 figure
Organic Superconductors: when correlations and magnetism walk in
This survey provides a brief account for the start of organic
superconductivity motivated by the quest for high Tc superconductors and its
development since the eighties'. Besides superconductivity found in 1D organics
in 1980, progresses in this field of research have contributed to better
understand the physics of low dimensional conductors highlighted by the wealth
of new remarkable properties. Correlations conspire to govern the low
temperature properties of the metallic phase. The contribution of
antiferromagnetic fluctuations to the interchain Cooper pairing proposed by the
theory is borne out by experimental investigations and supports
supercondutivity emerging from a non Fermi liquid background. Quasi one
dimensional organic superconductors can therefore be considered as simple
prototype systems for the more complex high Tc materials.Comment: 41 pages, 21 figures to be published in Journal of Superconductivity
and Novel Magnetis