128 research outputs found
NMR Detection of Temperature-Dependent Magnetic Inhomogeneities in URu2Si2
We present 29Si-NMR relaxation and spectral data in URu2Si2. Our echo-decay
experiments detect slowly fluctuating magnetic field gradients. In addition, we
find that the echo-decay shape (time dependence) varies with temperature T and
its rate behaves critically near the Neel temperature TN, indicating a
correlation between the gradient fluctuations and the transition to
small-moment order. T-dependent broadening contributions become visible below
100 Kelvin and saturate somewhat above TN, remaining saturated at lower
temperatures. Together, the line width and shift suggest partial lattice
distortions below TN. We propose an intrinsic minority phase below
and compare our results with one of the current theoretical models.Comment: 2 pages RevTeX, 1 figure, SCES 99-Japan, to appear in Physica
Direct evidence for critical exchange coupling via Allayers in the heavy fermion compound CePd2Al3
The long-range planar-type antiferromagnetic ordering in the heavy-fermion compound CePd2Al3 is shown to critically depend on the exact occupation and distribution of aluminum atoms over their available lattice sites. A poly-crystalline sample (TN=2.7 K) is systematically compared with a nonordering single crystal, by means of susceptibility, specific heat, and site-specific Al-NQR/NMR experiments. Implications for other Al-containing heavy-fermion systems are discussed
Susceptibility inhomogeneity and non-Fermi liquid behavior in UCu_{5-x}Pt_x
Transverse-field muSR shifts and relaxation rates have been measured in the
non-Fermi liquid (NFL) alloy system UCu_{5-x}Pt_x, x = 1.0, 1.5, and 2.5. At
low temperatures the fractional spread in Knight shifts delta K/K approx
deltachi/chi is gtrsim 2 for x = 1, but is only half this value for x = 1.5 and
2.5. In a disorder-driven scenario where the NFL behavior is due to a broadly
distributed (Kondo or Griffiths-phase cluster) characteristic energy E, our
results indicate that delta E/E_{rm av} approx (delta K/K)_{T=0} is similar for
UCu_{5-x}Pd_x (x = 1 and 1.5) and UCu_4Pt, but is reduced for UCu_{5-x}Pt_x, x
= 1.5 and 2.5. This reduction is due to a marked increase of E with increasing
x; the spread delta E is found to be roughly independent of x. Our results
correlate with the observed suppression of other NFL anomalies for x > 1 in
UCu_{5-x}Pt_x but not in UCu_{5-x}Pd_x, and are further evidence for the
importance of disorder in the NFL behavior of both these alloy systems.Comment: 4 pages, 2 figures, submitted to 10th International Conference on
Muon Spin Rotation, Relaxation, and Resonance, Oxford, UK, August 200
Glassy Spin Dynamics in Non-Fermi-Liquid UCu_{5-x}Pd_x, x = 1.0 and 1.5
Local f-electron spin dynamics in the non-Fermi-liquid heavy-fermion alloys
UCu_{5-x}Pd_x, x = 1.0 and 1.5, have been studied using muon spin-lattice
relaxation. The sample-averaged asymmetry function Gbar(t) indicates strongly
inhomogeneous spin fluctuations, and exhibits the scaling Gbar(t,H) =
Gbar(t/H^\gamma) expected from glassy dynamics. At 0.05 K \gamma(x=1.0) = 0.35
\pm 0.1, but \gamma(x=1.5) = 0.7 \pm 0.1. This is in contrast to inelastic
neutron scattering results, which yield \gamma = 0.33 for both concentrations.
There is no sign of static magnetism \gtrsim 10^{-3} \mu_B/U ion in either
material above 0.05 K. Our results strongy suggest that both alloys are quantum
spin glasses.Comment: 4 pages, 4 figures, to be published in Physical Review Letter
Spin dynamics in a structurally ordered non-Fermi liquid compound: YbRh_2Si_2
Muon spin relaxation (muSR) experiments have been carried out at low
temperatures in the non-Fermi-liquid heavy-fermion compound YbRh_2Si_2. The
longitudinal-field muSR relaxation function is exponential, indicative that the
dynamic spin fluctuations are homogeneous. The relaxation rate 1/T_1 varies
with applied field as H^{-y}, y = 1.0 \pm 0.1, which implies a scaling law of
the form \chi''(\omega) \propto \omega^{-y} f(\omega/T), \lim_{x\to0} f(x) = x
for the dynamic spin susceptibility.Comment: 5 pages, 2 figures. To be published in proceedings of musr2002
(Physica B
Magnetism and superconductivity in CeRh_{1-x}Ir_xIn_5 heavy fermion materials
We report on zero-field muon spin relaxation studies of cerium based
heavy-fermion materials CeRh_{1-x}Ir_xIn_5. In the superconducting x=0.75 and 1
compositions muon spin relaxation functions were found to be temperature
independent across T_c; no evidence for the presence of electronic magnetic
moments was observed. The x=0.5 material is antiferromagnetic below T_N=3.75 K
and superconducting below T_c=0.8 K. Muon spin realxation spectra show the
gradual onset of damped coherent oscillations characteristic of magnetic order
below T_N. At 1.65 K the total oscillating amplitude accounts for at least 85%
of the sample volume. No change in muon precession frequency or amplitude is
detected on cooling below T_c, indicating the microscopic coexistence of
magnetism and superconductivity in this material.Comment: 6 pages with 3 figures. Revision with corrected axis label (mK) in
Fig.
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