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The polymeric conformational effect on capacitive deionization performance of graphene oxide/polypyrrole composite electrode
Exploitation of novel faradic materials is an alternative implementation for solving the problem of poor specific electrosorption capacity that conventional carbon materials are encountered in capacitive deionization. Particularly, composite electrode is just a suitable choice because of its potentially high ion-storage ability. Herein, a cyclic voltammetric treatment method with different low limit of potential window was used to manipulate the polymeric conformation and doping level of graphene oxide/polypyrrole (GO/PPy) composite electrode. Based on it, the effect of polymeric structure on the electrosorption performance was systematically studied. When the low limit of potential window is shifted negatively enough, the irreversible polymeric conformational shrinks of GO/PPy are promoted, which not only hinders the insertion process of ions, but also decreases the doping level of polymer due to the intensive interchain-action produced by more entangled polymeric chain. Thus, the number of intercalated ions should decrease, which is expressed by electrochemical impedance spectroscopy (EIS) results and is proportional to the electrosorption capacity of GO/PPy composite electrode in membrane capacitive deionization (MCDI) process. Our work suggests that the less packing density, higher doping level and more charge delocalization on PPy backbone in electrode are beneficial to enhance its capacitive deionization performance
Measurement of the c-axis optical reflectance of AFeAs (A=Ba, Sr) single crystals: Evidence of different mechanisms for the formation of two energy gaps
We present the c-axis optical reflectance measurement on single crystals of
BaFeAs and SrFeAs, the parent compounds of FeAs based
superconductors. Different from the ab-plane optical response where two
distinct energy gaps were observed in the SDW state, only the smaller energy
gap could be seen clearly for \textbf{E}c-axis. The very pronounced
energy gap structure seen at a higher energy scale for
\textbf{E}ab-plane is almost invisible. We propose a novel picture
for the band structure evolution across the SDW transition and suggest
different driving mechanisms for the formation of the two energy gaps.Comment: 4 page
Measurements of Heavy Flavor and Di-electron Production at STAR
Heavy quarks are produced early in the relativistic heavy ion collisions, and
provide an excellent probe into the hot and dense nuclear matter created at
RHIC. In these proceedings, we will discuss recent STAR measurements of heavy
flavor production, to investigate the heavy quark interaction with the medium.
Electromagnetic probes, such as electrons, provide information on the various
stages of the medium evolution without modification by final stage
interactions. Di-electron production measurements by STAR will also be
discussed.Comment: 5 pages, 6 figures, proceedings for CPOD201
Anisotropic superconducting properties of aligned SmLaFeAsOF microcrystalline powder
The SmLaFeAsOF compound is a quasi-2D
layered superconductor with a superconducting transition temperature T = 52
K. Due to the Fe spin-orbital related anisotropic exchange coupling
(antiferromagnetic or ferromagnetic fluctuation), the tetragonal
microcrystalline powder can be aligned at room temperature using the
field-rotation method where the tetragonal -plane is parallel to the
aligned magnetic field B and -axis along the rotation axis.
Anisotropic superconducting properties with anisotropic diamagnetic ratio
2.4 + 0.6 was observed from low field susceptibility
(T) and magnetization M(B). The anisotropic low-field phase diagram
with the variation of lower critical field gives a zero-temperature penetration
depth (0) = 280 nm and (0) = 120 nm. The magnetic
fluctuation used for powder alignment at 300 K may be related with the pairing
mechanism of superconductivity at lower temperature.Comment: 4 pages, 6 figure
Simple Front End Electronics for Multigap Resistive Plate Chambers
A simple circuit for the presentation of the signals from Multi-gap Resistive
Plate Chambers (MRPCs) to standard existing digitization electronics is
described. The circuit is based on "off-the-shelf" discrete components. An
optimization of the values of specific components is required to match the
aspects of the MRPCs for the given application. This simple circuit is an
attractive option for the initial signal processing for MRPC prototyping and
bench- or beam-testing efforts, as well as for final implementations of
small-area Time-of-Flight systems with existing data acquisition systems.Comment: submitted to Nucl. Inst. and Methods, Section
Obvious enhancement of the total reaction cross sections for P with Si target and the possible relavent mechanisms
The reaction cross sections of P and the corresponding isotones on
Si target were measured at intermediate energies. The measured reaction cross
sections of the N=12 and 13 isotones show an abrupt increase at . The
experimental results for the isotones with as well as P can
be well described by the modified Glauber theory of the optical limit approach.
The enhancement of the reaction cross section for P could be explained
in the modified Glauber theory with an enlarged core. Theoretical analysis with
the modified Glauber theory of the optical limit and few-body approaches
underpredicted the experimental data of P. Our theoretical analysis
shows that an enlarged core together with proton halo are probably the
mechanism responsible for the enhancement of the cross sections for the
reaction of P+Si.Comment: 16 pages, 5 figures, to be published in Phys.Rev.
Three dimensionality of band structure and a large residual quasiparticle population in BaKFeAs as revealed by the c-axis polarized optical measurement
We report on a c-axis polarized optical measurement on a
BaKFeAs single crystal. We find that the c-axis
optical response is significantly different from that of high-T cuprates.
The experiments reveal an anisotropic three-dimensional optical response with
the absence of the Josephson plasma edge in R() in the superconducting
state. Furthermore, different from the ab-plane optical response, a large
residual quasiparticle population down to was observed in
the c-axis polarized reflectance measurement. We elaborate that there exist
nodes for the superconducting gap in regions of the 3D Fermi surface that
contribute dominantly to the c-axis optical conductivity.Comment: 4 figure
Effect of electron-electron scattering on spin dephasing in a high-mobility low-density twodimensional electron gas
Utilizing time-resolved Kerr rotation techniques, we have investigated the
spin dynamics of a high mobility, low density two dimensional electron gas in a
GaAs/Al0:35Ga0:65As heterostructure in dependence on temperature from 1.5 K to
30 K. It is found that the spin relaxation/dephasing time under a magnetic
field of 0.5 T exhibits a maximum of 3.12 ns around 14 K, superimposed on an
increasing background with rising temperature. The appearance of the maximum is
ascribed to that at the temperature where the crossover from the degenerate to
the nondegenerate regime takes place, electron-electron Coulomb scattering
becomes strongest, and thus inhomogeneous precession broadening due to
D'yakonov-Perel'(DP) mechanism becomes weakest. These results agree with the
recent theoretical predictions [Zhou et al., PRB 75, 045305 (2007)], verifying
the importance of electron-electron Coulomb scattering to electron spin
relaxation/dephasing.Comment: 4 pages, 2 figure
152 fs nanotube-mode-locked thulium-doped all-fiber laser.
Ultrafast fiber lasers with broad bandwidth and short pulse duration have a variety of applications, such as ultrafast time-resolved spectroscopy and supercontinuum generation. We report a simple and compact all-fiber thulium-doped femtosecond laser mode-locked by carbon nanotubes. The oscillator operates in slightly normal cavity dispersion at 0.055 ps(2), and delivers 152 fs pulses with 52.8 nm bandwidth and 0.19 nJ pulse energy. This is the shortest pulse duration and the widest spectral width demonstrated from Tm-doped all-fiber lasers based on 1 or 2 dimensional nanomaterials, underscoring their growing potential as versatile saturable absorber materials.We acknowledge funding from the Science and Technology Projects of Shenzhen City (JCYJ20150324140036862,
JCYJ20140418095735546), the Natural Science Foundation of Guangdong Province (2015A030310464,
2016A030310049), the Scientific Research Foundation of Shenzhen City (827-000118), the Teknologiateollisuus
TT-100, the European Union’s Seventh Framework Programme (REA grant agreement No. 631610), the Academy
of Finland (No. 284548), Tekes (OPEC) and Aalto University (Finland). TH acknowledges funding from the
Royal Academy of Engineering through a research fellowship (Graphlex).This is the final version of the article. It first appeared from Nature Publishing Group at http://dx.doi.org/10.1038/srep28885
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