57 research outputs found
Spontaneous decay of excited atomic states near a carbon nanotube
Spontaneous decay process of an excited atom placed inside or outside (near
the surface) a carbon nanotube is analyzed. Calculations have been performed
for various achiral nanotubes. The effect of the nanotube surface has been
demonstrated to dramatically increase the atomic spontaneous decay rate -- by 6
to 7 orders of magnitude compared with that of the same atom in vacuum. Such an
increase is associated with the nonradiative decay via surface excitations in
the nanotube.Comment: 8 pages, 3 figure
Quantum tight-binding chains with dissipative coupling
We present a one-dimensional tight-binding chain of two-level systems coupled
only through common dissipative Markovian reservoirs. This quantum chain can
demonstrate anomalous thermodynamic behavior contradicting Fourier law.
Population dynamics of individual systems of the chain is polynomial with the
order determined by the initial state of the chain. The chain can simulate
classically hard problems, such as multi-dimensional random walks
Microscopic theory of quantum dot interactions with quantum light: local field effect
A theory of both linear and nonlinear electromagnetic response of a single QD
exposed to quantum light, accounting the depolarization induced local--field
has been developed. Based on the microscopic Hamiltonian accounting for the
electron--hole exchange interaction, an effective two--body Hamiltonian has
been derived and expressed in terms of the incident electric field, with a
separate term describing the QD depolarization. The quantum equations of motion
have been formulated and solved with the Hamiltonian for various types of the
QD excitation, such as Fock qubit, coherent fields, vacuum state of
electromagnetic field and light with arbitrary photonic state distribution. For
a QD exposed to coherent light, we predict the appearance of two oscillatory
regimes in the Rabi effect separated by the bifurcation. In the first regime,
the standard collapse--revivals phenomenon do not reveal itself and the QD
population inversion is found to be negative, while in the second one, the
collapse--revivals picture is found to be strongly distorted as compared with
that predicted by the standard Jaynes-Cummings model. %The model developed can
easily be extended to %%electromagnetic excitation. For the case of QD
interaction with arbitrary quantum light state in the linear regime, it has
been shown that the local field induce a fine structure of the absorbtion
spectrum. Instead of a single line with frequency corresponding to which the
exciton transition frequency, a duplet is appeared with one component shifted
by the amount of the local field coupling parameter. It has been demonstrated
the strong light--mater coupling regime arises in the weak-field limit. A
physical interpretation of the predicted effects has been proposed.Comment: 14 pages, 7 figure
Spontaneous decay of an emitter's excited state near a finite-length metallic carbon nanotube
The spontaneous decay of an excited state of an emitter placed in the
vicinity of a metallic single-wall carbon nanotube (SWNT) was examined
theoretically. The emitter-SWNT coupling strongly depends on the position of
the emitter relative to the SWNT, the length of the SWNT, the dipole transition
frequency and the orientation of the emitter. In the high-frequency regime,
dips in the spectrum of the spontaneous decay rate exist at the resonance
frequencies in the spectrum of the SWNT conductivity. In the
intermediate-frequency regime, the SWNT conductivity is very low, and the
spontaneous decay rate is practically unaffected by the SWNT. In the
low-frequency regime, the spectrum of the spontaneous decay rate contains
resonances at the antennas resonance frequencies for surface-wave propagation
in the SWNT. Enhancement of both the total and radiative spontaneous decay
rates by several orders in magnitude is predicted at these resonance
frequencies. The strong emitter-field coupling is achieved, in spite of the low
Q factor of the antenna resonances, due to the very high magnitude of the
electromagnetic field in the near-field zone. The vacuum Rabi oscillations of
the population of the excited emitter state are exhibited when the emitter is
coupled to an antenna resonance of the SWNT.Comment: 8 pages, 6 figure
Spontaneous decay dynamics in atomically doped carbon nanotubes
We report a strictly non-exponential spontaneous decay dynamics of an excited
two-level atom placed inside or at different distances outside a carbon
nanotube (CN). This is the result of strong non-Markovian memory effects
arising from the rapid variation of the photonic density of states with
frequency near the CN. The system exhibits vacuum-field Rabi oscillations, a
principal signature of strong atom-vacuum-field coupling, when the atom is
close enough to the nanotube surface and the atomic transition frequency is in
the vicinity of the resonance of the photonic density of states. Caused by
decreasing the atom-field coupling strength, the non-exponential decay dynamics
gives place to the exponential one if the atom moves away from the CN surface.
Thus, atom-field coupling and the character of the spontaneous decay dynamics,
respectively, may be controlled by changing the distance between the atom and
CN surface by means of a proper preparation of atomically doped CNs. This opens
routes for new challenging nanophotonics applications of atomically doped CN
systems as various sources of coherent light emitted by dopant atoms.Comment: 10 pages, 4 figure
van der Waals coupling in atomically doped carbon nanotubes
We have investigated atom-nanotube van der Waals (vdW) coupling in atomically
doped carbon nanotubes (CNs). Our approach is based on the perturbation theory
for degenerated atomic levels, thus accounting for both weak and strong
atom-vacuum-field coupling. The vdW energy is described by an integral equation
represented in terms of the local photonic density of states (DOS). By solving
it numerically, we demonstrate the inapplicability of standard
weak-coupling-based vdW interaction models in a close vicinity of the CN
surface where the local photonic DOS effectively increases, giving rise to an
atom-field coupling enhancement. An inside encapsulation of atoms into the CN
has been shown to be energetically more favorable than their outside adsorption
by the CN surface. If the atom is fixed outside the CN, the modulus of the vdW
energy increases with the CN radius provided that the weak atom-field coupling
regime is realized (i.e., far enough from the CN). For inside atomic position,
the modulus of the vdW energy decreases with the CN radius, representing a
general effect of the effective interaction area reduction with lowering the CN
curvature.Comment: 15 pages, 5 figure
Harmonic generation in ring-shaped molecules
We study numerically the interaction between an intense circularly polarized
laser field and an electron moving in a potential which has a discrete
cylindrical symmetry with respect to the laser pulse propagation direction.
This setup serves as a simple model, e.g., for benzene and other aromatic
compounds. From general symmetry considerations, within a Floquet approach,
selection rules for the harmonic generation [O. Alon Phys. Rev. Lett. 80 3743
(1998)] have been derived recently. Instead, the results we present in this
paper have been obtained solving the time-dependent Schroedinger equation ab
initio for realistic pulse shapes. We find a rich structure which is not always
dominated by the laser harmonics.Comment: 15 pages including 7 figure
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