4,119 research outputs found
Numerical study of the lattice vacancy effects on the single-channel electron transport of graphite ribbons
Lattice vacancy effects on electrical conductance of nanographite ribbon are
investigated by means of the Landauer approach using a tight binding model. In
the low-energy regime ribbons with zigzag boundary provide a single conducting
channel whose origin is connected with the presence of edge states. It is found
that the chemical potential dependence of conductance strongly depends on the
difference () of the number of removed A and B sublattice sites. The
large lattice vacancy with shows zero-conductance dips
in the single-channel region, however, the large lattice vacancy with
has no dip structure in this region. The connection between this
conductance rule and the Longuet-Higgins conjecture is also discussed
The nirSTBM region coding for cytochrome cd1-dependent nitrite respiration of Pseudomonas stutzeri consists of a cluster of mono-, di-, and tetraheme proteins
AbstractGenes for respiratory nitrite reduction (denitrification) of Pseudomonas stutzeri are clustered within 7 kbp. A 4.6-kbp Hind III-Kpn I fragment carrying nirS, the structural gene for cytochrome cd1, was sequenced. An open reading frame immediately downstream of nirScodes for a 22.8-kDa protein with four heme c-binding motifs. Mutagenesis of this gene causes an apparent defect in electron donation to cytochrome cd1. Following this ORF are the structural genes for cytochrome c552, cytochrome c551, and ORF5 that codes for a 11.9-kDa monoheme protein. All cytochromes have a signal sequence for protein export
Avoided crossings in mesoscopic systems: electron propagation on a non-uniform magnetic cylinder
We consider an electron constrained to move on a surface with revolution
symmetry in the presence of a constant magnetic field parallel to the
surface axis. Depending on and the surface geometry the transverse part of
the spectrum typically exhibits many crossings which change to avoided
crossings if a weak symmetry breaking interaction is introduced. We study the
effect of such perturbations on the quantum propagation. This problem admits a
natural reformulation to which tools from molecular dynamics can be applied. In
turn, this leads to the study of a perturbation theory for the time dependent
Born-Oppenheimer approximation
Orbital Ordering Structures in (Nd,Pr)0.5Sr0.5MnO3 Manganite Thin Films on Perovskite (011) Substrates
Structural study of orbital-ordered manganite thin films has been conducted
using synchrotron radiation, and a ground state electronic phase diagram is
made. The lattice parameters of four manganite thin films, Nd0.5Sr0.5MnO3
(NSMO) or Pr0.5Sr0.5MnO3 (PSMO) on (011) surfaces of SrTiO3 (STO) or
[(LaAlO3){0.3}(SrAl0.5Ta0.5O3){0.7}] (LSAT), were measured as a function of
temperature. The result shows, as expected based on previous knowledge of bulk
materials, that the films' resistivity is closely related to their structures.
Observed superlattice reflections indicate that NSMO thin films have an
antiferro-orbital-ordered phase as their low-temperature phase while PSMO film
on LSAT has a ferro-orbital-ordered phase, and that on STO has no
orbital-ordered phase. A metallic ground state was observed only in films
having a narrow region of A-site ion radius, while larger ions favor
ferro-orbital-ordered structure and smaller ions stabilize
antiferro-orbital-ordered structure. The key to the orbital-ordering transition
in (011) film is found to be the in-plane displacement along [0-1 1] direction.Comment: 19pages, 11 figure
Superconductivity and spin-glass like behavior in system with Pd sheet sandwiched between graphene sheets
Pd-metal graphite (Pd-MG) has a layered structure, where each Pd sheet is
sandwiched between adjacent graphene sheets. DC magnetization and AC magnetic
susceptibility of Pd-MG have been measured using a SQUID magnetometer. Pd-MG
undergoes a superconducting transition at ( K). The
superconductivity occurs in Pd sheets. The relaxation of (aging),
which is common to spin glass systems, is also observed below . The
relaxation rate shows a peak at a characteristic time , which is
longer than a wait time . The irreversibility between and
occurs well above . The susceptibility obeys a
Curie-Weiss behavior with a negative Curie-Weiss temperature ( K). The growth of antiferromagnetic order is limited by the
disordered nature of nanographites, forming spin glass-like behavior at low
temperatures in graphene sheets.Comment: 21 pages, 15 figures; submitted to J. Phys.: Condensed Matte
First application of the Trojan Horse Method with a Radioactive Ion Beam: study of the F()O}} reaction at astrophysical energies
Measurement of nuclear cross sections at astrophysical energies involving
unstable species is one of the most challenging tasks in experimental nuclear
physics. The use of indirect methods is often unavoidable in this scenario. In
this paper the Trojan Horse Method is applied for the first time to a
radioactive ion beam induced reaction studying the
F()O process at low energies relevant to astrophysics
via the three body reaction H(F,O)n. The knowledge
of the F()O reaction rate is crucial to understand
the nova explosion phenomena. The cross section of this reaction is
characterized by the presence of several resonances in Ne and possibly
interference effects among them. The results reported in Literature are not
satisfactory and new investigations of the F()O
reaction cross section will be useful. In the present work the spin-parity
assignments of relevant levels have been discussed and the astrophysical
S-factor has been extracted considering also interference effectsComment: 7 pages, 4 figure
Low-frequency modes in the Raman spectrum of sp-sp2 nanostructured carbon
A novel form of amorphous carbon with sp-sp2 hybridization has been recently
produced by supersonic cluster beam deposition showing the presence in the film
of both polyynic and cumulenic species [L. Ravagnan et al. Phys. Rev. Lett. 98,
216103 (2007)]. Here we present a in situ Raman characterization of the low
frequency vibrational region (400-800 cm-1) of sp-sp2 films at different
temperatures. We report the presence of two peaks at 450 cm-1 and 720 cm-1. The
lower frequency peak shows an evolution with the variation of the sp content
and it can be attributed, with the support of density functional theory (DFT)
simulations, to bending modes of sp linear structures. The peak at 720 cm-1
does not vary with the sp content and it can be attributed to a feature in the
vibrational density of states activated by the disorder of the sp2 phase.Comment: 15 pages, 5 figures, 1 tabl
Phonons in random alloys: the itinerant coherent-potential approximation
We present the itinerant coherent-potential approximation(ICPA), an analytic,
translationally invariant and tractable form of augmented-space-based,
multiple-scattering theory in a single-site approximation for harmonic phonons
in realistic random binary alloys with mass and force-constant disorder.
We provide expressions for quantities needed for comparison with experimental
structure factors such as partial and average spectral functions and derive the
sum rules associated with them. Numerical results are presented for Ni_{55}
Pd_{45} and Ni_{50} Pt_{50} alloys which serve as test cases, the former for
weak force-constant disorder and the latter for strong. We present results on
dispersion curves and disorder-induced widths. Direct comparisons with the
single-site coherent potential approximation(CPA) and experiment are made which
provide insight into the physics of force-constant changes in random alloys.
The CPA accounts well for the weak force-constant disorder case but fails for
strong force-constant disorder where the ICPA succeeds.Comment: 19 pages, 12 eps figures, uses RevTex
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