366 research outputs found
On the existence of optimal affine methods for approximating linear functionals
AbstractThe existence of an optimal affine method using linear information is established for the approximation of a linear functional on a convex set. This is a generalization of a result of S. A. Smolyak (“On Optimal Restoration of Functions and Functionals of Them,” Candidate Dissertation, Moscow State University, 1965)
Transport and optical response of molecular junctions driven by surface plasmon-polaritons
We consider a biased molecular junction subjected to external time-dependent
electromagnetic field. The field for two typical junction geometries (bowtie
antennas and metal nanospheres) is calculated within finite-difference
time-domain technique. Time-dependent transport and optical response of the
junctions is calculated within non-equilibrium Green's function approach
expressed in a form convenient for description of multi-level systems. We
present numerical results for a two-level (HOMO-LUMO) model, and discuss
influence of localized surface plasmon polariton modes on transport.Comment: 9 pages, 6 figure
Surface quality and surface waves on subwavelength-structured silver films
We analyze the physical-chemical surface properties of single-slit, single-groove subwavelength-structured silver films with high-resolution transmission electron microscopy and calculate exact solutions to Maxwell’s equations corresponding to recent far-field interferometry experiments using these structures. Contrary to a recent suggestion the surface analysis shows that the silver films are free of detectable contaminants. The finite-difference time-domain calculations, in excellent agreement with experiment, show a rapid fringe amplitude decrease in the near zone (slit-groove distance out to 3–4 wavelengths). Extrapolation to slit-groove distances beyond the near zone shows that the surface wave evolves to the expected bound surface plasmon polariton (SPP). Fourier analysis of these results indicates the presence of a distribution of transient, evanescent modes around the SPP that dephase and dissipate as the surface wave evolves from the near to the far zone
Analysis of surface waves generated on subwavelength-structured silver films
Using transmission electron microscopy (TEM) to analyse the physical-chemical
surface properties of subwavlength structured silver films and
finite-difference time-domain (FDTD) numerical simulations of the optical
response of these structures to plane-wave excitation, we report on the origin
and nature of the persistent surface waves generated by a single slit-groove
motif and recently measured by far-field optical interferometry. The surface
analysis shows that the silver films are free of detectable oxide or sulfide
contaminants, and the numerical simulations show very good agreement with the
results previously reported.Comment: 9 Figure
Optical properties of metal nanoparticles with no center of inversion symmetry: observation of volume plasmons
We present theoretical and experimental studies of the optical response of
L-shaped silver nanoparticles. The scattering spectrum exhibits several plasmon
resonances that depend sensitively on the polarization of the incident
electromagnetic field. The physical origin of the resonances is traced to
different plasmon phenomena. In particular, a high energy band with unusual
properties is interpreted in terms of volume plasmon oscillations arising from
the asymmetry of a nanoparticle.Comment: 14 pages, 5 figures. Physical Review B, 2007, accepte
Vibrational Spectra of a Mechanosensitive Channel
We report the simulated vibrational spectra of a mechanosensitive membrane channel in different gating states. Our results show that while linear absorption is insensitive to structural differences, linear dichroism and sum-frequency generation spectroscopies are sensitive to the orientation of the transmembrane helices, which is changing during the opening process. Linear dichroism cannot distinguish an intermediate structure from the closed structure, but sum-frequency generation can. In addition, we find that two-dimensional infrared spectroscopy can be used to distinguish all three investigated gating states of the mechanosensitive membrane channel.
Об истории открытия и природе алмазов в вулканических породах Камчатки
The history of the discovery of diamonds in the products of Kamchatka volcanic eruptions is briefly described, and the results of comprehensive studies of Tolbachin diamonds including crystallomorphology, faceted sculptures, xenomineral greases and films on the surface, nanomicroswitches, impurity elements, spectroscopic properties, isotopic composition of carbon and nitrogen are summarized. The conclusion is drawn about the natural origin of the Tolbachin diamonds formed directly in the volcanic ash-gas cloud by crystallization from gases stimulated by atmospheric electric discharges.Кратко описана история открытия алмазов в продуктах извержений вулканов Камчатки и обобщены результаты комплексных исследований толбачинских алмазов – кристалломорфологии, гранной скульптуры, ксеноминеральных примазок и пленок на поверхности, наномикровключений, элементов-примесей, спектроскопических свойств, изотопного состава углерода и азота. Сделан вывод о природном происхождении толбачинских алмазов, образовавшихся непосредственно в среде вулканического пеплогазового облака путем кристаллизации из газов, стимулированной атмосферными электрическими разрядами
Measurement of decay rate and parameters at KEDR
Using the inclusive photon spectrum based on a data sample collected at the
peak with the KEDR detector at the VEPP-4M collider, we
measured the rate of the radiative decay as well
as mass and width. Taking into account an asymmetric photon
lineshape we obtained keV, MeV/, MeV.Comment: 6 pages, 3 figure
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