3,188 research outputs found
Quantum and thermal spin relaxation in diluted spin ice: Dy(2-x)MxTi2O7 (M = Lu, Y)
We have studied the low temperature a.c. magnetic susceptibility of the
diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the
frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y
or Lu. We examine a broad range of dilutions, 0 <= x <= 1.98, and we find that
the T ~ 16 K freezing is suppressed for low levels of dilution but re-emerges
for x > 0.4 and persists to x = 1.98. This behavior can be understood as a
non-monotonic dependence of the quantum spin relaxation time with dilution. The
results suggest that the observed spin freezing is fundamentally a single spin
process which is affected by the local environment, rather than the development
of spin-spin correlations as earlier data suggested.Comment: 26 pages, 9 figure
Boundary conditions and the entropy bound
The entropy-to-energy bound is examined for a quantum scalar field confined
to a cavity and satisfying Robin condition on the boundary of the cavity. It is
found that near certain points in the space of the parameter defining the
boundary condition the lowest eigenfrequency (while non-zero) becomes
arbitrarily small. Estimating, according to Bekenstein and Schiffer, the ratio
by the -function, , we compute
explicitly and find that it is not bounded near those points that signals
violation of the bound. We interpret our results as imposing certain
constraints on the value of the boundary interaction and estimate the forbidden
region in the parameter space of the boundary conditions.Comment: 16 pages, latex, v2: typos corrected, to appear in Phys.Rev.
Slow spin relaxation in a highly polarized cooperative paramagnet
We report measurements of the ac susceptibility of the cooperative paramagnet
Tb2Ti2O7 in a strong magnetic field. Our data show the expected saturation
maximum in chi(T) and also an unexpected low frequency dependence (< 1 Hz) of
this peak, suggesting very slow spin relaxations are occurring. Measurements on
samples diluted with nonmagnetic Y3+ or Lu3+ and complementary measurements on
pure and diluted Dy2Ti2O7 strongly suggest that the relaxation is associated
with dipolar spin correlations, representing unusual cooperative behavior in a
paramagnetic system.Comment: Accepted for publication in Physical Review Letter
Quantum-Classical Reentrant Relaxation Crossover in Dy2Ti2O7 Spin-Ice
We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through
measurements of the a.c. magnetic susceptibility. While the characteristic spin
relaxation time is thermally activated at high temperatures, it becomes almost
temperature independent below Tcross ~ 13 K, suggesting that quantum tunneling
dominates the relaxation process below that temperature. As the low-entropy
spin ice state develops below Tice ~ 4 K, the spin relaxation time increases
sharply with decreasing temperature, suggesting the emergence of a collective
degree of freedom for which thermal relaxation processes again become important
as the spins become highly correlated
Geometrical Magnetic Frustration in Rare Earth Chalcogenide Spinels
We have characterized the magnetic and structural properties of the CdLn2Se4
(Ln = Dy, Ho), and CdLn2S4 (Ln = Ho, Er, Tm, Yb) spinels. We observe all
compounds to be normal spinels, possessing a geometrically frustrated
sublattice of lanthanide atoms with no observable structural disorder. Fits to
the high temperature magnetic susceptibilities indicate these materials to have
effective antiferromagnetic interactions, with Curie-Weiss temperatures theta ~
-10 K, except CdYb2S4 for which theta ~ -40 K. The absence of magnetic long
range order or glassiness above T = 1.8 K strongly suggests that these
materials are a new venue in which to study the effects of strong geometrical
frustration, potentially as rich in new physical phenomena as that of the
pyrochlore oxides.Comment: 17 pages, 5 figures, submitted to Phys Rev B; added acknowledgement
Exfoliative cytodiagnosis as a screening test in bladder tumours
A retrospective evaluation of patients afflicted with tumours of the bladder shows that exfoliative cytology of the urinary sediment can be recommended for early diagnosis of latent tumours of the bladder, particularly of malignant papilloma and carcinoma; early diagnosis of malignant degeneration of benign bladder papilloma; and early diagnosis of a recurrence of bladder tumour after a bladder operation. It is a simple method with great diagnostic value both in the clinic and in urological practice
Electrochemical pressure impedance spectroscopy for polymer electrolyte membrane fuel cells: Signal interpretation
Electrochemical pressure impedance spectroscopy (EPIS) is an emerging tool for the diagnosis of polymer electrolyte membrane fuel cells (PEMFC). It is based on analyzing the frequency response of the cell voltage with respect to an excitation of the gas-phase pressure. Several experimental studies in the past decade have shown the complexity of EPIS signals, and so far there is no agreement on the interpretation of EPIS features. The present study contributes to shed light into the physicochemical origin of EPIS features, by using a combination of pseudo-two-dimensional modeling and analytical interpretation. Using static simulations, the contributions of cathode equilibrium potential, cathode overpotential, and membrane resistance on the quasi-static EPIS response are quantified. Using model reduction, the EPIS responses of individual dynamic processes are predicted and compared to the response of the full model. We show that the EPIS signal of the PEMFC studied here is dominated by the humidifier. The signal is further analyzed by using transfer functions between various internal cell states and the outlet pressure excitation. We show that the EPIS response of the humidifier is caused by an oscillating oxygen molar fraction due to an oscillating mass flow rate
Ga-NMR local susceptibility of the kagome-based magnet SrCr_9pGa_(12-9p)O_19. A high temperature study
We report a high- Ga-NMR study in the kagome-based antiferromagnetic
compound SrCrGaO (), and present a
refined mean-field analysis of the high T local NMR susceptibility of Cr
frustrated moments. We find that the intralayer kagome coupling is K,
and the interlayer coupling through non-kagome Cr moments is K. The ratio confirms the common belief that
the frustrated entity is a pyrochlore slab.Comment: 8 pages, 4 figures Conference paper: Highly Frustrated Magnetism
2000, Waterloo (Canada) Submitted to Canadian Journal of Physic
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