935 research outputs found
Detection of coherent magnons via ultrafast pump-probe reflectance spectroscopy in multiferroic Ba0.6Sr1.4Zn2Fe12O22
We report the detection of a magnetic resonance mode in multiferroic
Ba0.6Sr1.4Zn2Fe12O22 using time domain pump-probe reflectance spectroscopy.
Magnetic sublattice precession is coherently excited via picosecond thermal
modification of the exchange energy. Importantly, this precession is recorded
as a change in reflectance caused by the dynamic magnetoelectric effect. Thus,
transient reflectance provides a sensitive probe of magnetization dynamics in
materials with strong magnetoelectric coupling, such as multiferroics,
revealing new possibilities for application in spintronics and ultrafast
manipulation of magnetic moments.Comment: 4 figure
Magnetic properties of the spin-1 chain compound NiClCHCHCHNH
We report experimental results of the static magnetization, ESR and NMR
spectroscopic measurements of the Ni-hybrid compound
NiClCHCHCHNH. In this material NiCl octahedra are
structurally arranged in chains along the crystallographic -axis. According
to the static susceptibility and ESR data Ni spins are isotropic
and are coupled antiferromagnetically (AFM) along the chain with the exchange
constant K. These are important prerequisites for the realization of
the so-called Haldane spin-1 chain with the spin-singlet ground state and a
quantum spin gap. However, experimental results evidence AFM order at K presumably due to small interchain couplings. Interestingly,
frequency-, magnetic field-, and temperature-dependent ESR measurements, as
well as the NMR data, reveal signatures which could presumably indicate an
inhomogeneous ground state of co-existent mesoscopically spatially separated
AFM ordered and spin-singlet state regions similar to the situation observed
before in some spin-diluted Haldane magnets
Direct Observation of the Quantum Energy Gap in S = 1/2 Tetragonal Cuprate Antiferromagnets
Using an electron spin resonance spectrometer covering a wide range of
frequency and magnetic field, we have measured the low energy excitations of
the S=1/2 tetragonal antiferromagnets, Sr_{2}CuO_{2}Cl_{2} and
Sr_{2}Cu_{3}O_{4}Cl_{2}. Our observation of in-plane energy gaps of order 0.1
meV at zero external magnetic field are consistent with a spin wave
calculation, which includes several kinds of quantum fluctuations that remove
frustration. Results agree with other experiments and with exchange anisotropy
parameters determined from a five band Hubbard model.Comment: 4 pages, 3 figure
Magnetization steps in Zn_(1-x)Mn_xO: Four largest exchange constants and single-ion anisotropy
Magnetization steps (MST's) from Mn pairs in several single crystals of
Zn_(1-x)Mn_xO (0.0056<=x<=0.030, and in one powder (x=0.029), were observed.
The largest two exchange constants, J1/kB=-18.2+/-0.5K and J1'/kB=-24.3+/-0.6K,
were obtained from large peaks in the differential susceptibility, dM/dH,
measured in pulsed magnetic fields, H, up to 500 kOe. These two largest J's are
associated with the two inequivalent classes of nearest neighbors (NN's) in the
wurtzite structure. The 29% difference between J1 and J1' is substantially
larger than 13% in CdS:Mn, and 15% in CdSe:Mn. The pulsed-field data also
indicate that, despite the direct contact between the samples and a
superfluid-helium bath, substantial departures from thermal equilibrium
occurred during the 7.4 ms pulse. The third- and fourth-largest J's were
determined from the magnetization M at 20 mK, measured in dc magnetic fields H
up to 90 kOe. Both field orientations H||c and H||[10-10] were studied. (The
[10-10] direction is perpendicular to the c-axis, [0001].) By definition,
neighbors which are not NN's are distant neighbors (DN's). The largest DN
exchange constant (third-largest overall), has the value J/kB=-0.543+/-0.005K,
and is associated with the DN at r=c. Because this is not the closest DN, this
result implies that the J's do not decrease monotonically with the distance r.
The second-largest DN exchange constant (fourth-largest overall), has the value
J/kB=-0.080 K. It is associated with one of the two classes of neighbors that
have a coordination number z=12, but the evidence is insufficient for a
definite unique choice. The dependence of M on the direction of H gives
D/kB=-0.039+/-0.008K, in fair agreement with -0.031 K from earlier EPR work.Comment: 12 pages, 10 figures. Submitted to PR
Long wavelength magnetic and magnetoelectric excitations in the ferroelectric antiferromagnet BiFeO3
We present a terahertz spectroscopic study of magnetic excitations in
ferroelectric antiferromagnet BiFeO3. We interpret the observed spectrum of
long-wavelength magnetic resonance modes in terms of the normal modes of the
material's cycloidal antiferromagnetic structure. We find that the modulated
Dzyaloshinski-Moriya interaction leads to a splitting of the out-of-plane
resonance modes. We also assign one of the observed absorption lines to an
electromagnon excitation that results from the magnetoelectric coupling between
the ferroelectric polarization and the cycloidal magnetic structure of BiFeO3
Magnetic resonance in the antiferromagnetic and normal state of NH_3K_3C_60
We report on the magnetic resonance of NH_3K_3C_60 powders in the frequency
range of 9 to 225 GHz. The observation of an antiferromagnetic resonance below
the phase transition at 40 K is evidence for an antiferromagnetically ordered
ground state. In the normal state, above 40 K, the temperature dependence of
the spin-susceptibilty measured by ESR agrees with previous static measurements
and is too weak to be explained by interacting localized spins in an insulator.
The magnetic resonance line width has an unusual magnetic-field dependence
which is large and temperature independent in the magnetically ordered state
and decreases rapidly above the transition. These observations agree with the
suggestion that NH_3K_3C_60 is a metal in the normal state and undergoes a
Mott-Hubbard metal to insulator transition at 40 K.Comment: 4 pages, 5 figures. Submitted to Phys. Rev.
Magnetization steps in a diluted Heisenberg antiferromagnetic chain: Theory and experiments on TMMC:Cd
A theory for the equilibrium low-temperature magnetization M of a diluted
Heisenberg antiferromagnetic chain is presented. The magnetization curve, M
versus B, is calculated using the exact contributions of finite chains with 1
to 5 spins, and the "rise and ramp approximation" for longer chains. Some
non-equilibrium effects that occur in a rapidly changing B, are also
considered. Specific non-equilibrium models based on earlier treatments of the
phonon bottleneck, and of spin flips associated with cross relaxation and with
level crossings, are discussed. Magnetization data on powders of TMMC diluted
with cadmium [i.e., (CH_3)_4NMn_xCd_(1-x)Cl_3, with 0.16<=x<=0.50 were measured
at 0.55 K in 18 T superconducting magnets. The field B_1 at the first MST from
pairs is used to determine the NN exchange constant, J, which changes from -5.9
K to -6.5 K as x increases from 0.16 to 0.50. The magnetization curves obtained
in the superconducting magnets are compared with simulations based on the
equilibrium theory. Data for the differential susceptibility, dM/dB, were taken
in pulsed magnetic fields (7.4 ms duration) up to 50 T, with the powder samples
in a 1.5 K liquid-helium bath. Non-equilibrium effects, which became more
severe as x decreased, were observed. The non-equilibrium effects are
tentatively interpreted using the "Inadequate Heat Flow Scenario," or to
cross-relaxation, and crossings of energy levels, including those of excited
states.Comment: 16 pages, 14 figure
Magnetism, Critical Fluctuations and Susceptibility Renormalization in Pd
Some of the most popular ways to treat quantum critical materials, that is,
materials close to a magnetic instability, are based on the Landau functional.
The central quantity of such approaches is the average magnitude of spin
fluctuations, which is very difficult to measure experimentally or compute
directly from the first principles. We calculate the parameters of the Landau
functional for Pd and use these to connect the critical fluctuations beyond the
local-density approximation and the band structure.Comment: Replaced with the revised version accepted for publication.
References updated, errors corrected, other change
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