3,053 research outputs found
Zero Temperature Phase Transition in Spin-ladders: Phase Diagram and Dynamical studies of Cu(Hp)Cl
In a magnetic field, spin-ladders undergo two zero-temperature phase
transitions at the critical fields Hc1 and Hc2. An experimental review of
static and dynamical properties of spin-ladders close to these critical points
is presented. The scaling functions, universal to all quantum critical points
in one-dimension, are extracted from (a) the thermodynamic quantities
(magnetization) and (b) the dynamical functions (NMR relaxation). A simple
mapping of strongly coupled spin ladders in a magnetic field on the exactly
solvable XXZ model enables to make detailed fits and gives an overall
understanding of a broad class of quantum magnets in their gapless phase
(between Hc1 and Hc2). In this phase, the low temperature divergence of the NMR
relaxation demonstrates its Luttinger liquid nature as well as the novel
quantum critical regime at higher temperature. The general behaviour close
these quantum critical points can be tied to known models of quantum magnetism.Comment: few corrections made, 15 pages, to be published in European Journal
of Physics
Atomic and Electronic Structure of a Rashba - Junction at the BiTeI Surface
The non-centrosymmetric semiconductor BiTeI exhibits two distinct surface
terminations that support spin-split Rashba surface states. Their ambipolarity
can be exploited for creating spin-polarized - junctions at the
boundaries between domains with different surface terminations. We use scanning
tunneling microscopy/spectroscopy (STM/STS) to locate such junctions and
investigate their atomic and electronic properties. The Te- and I-terminated
surfaces are identified owing to their distinct chemical reactivity, and an
apparent height mismatch of electronic origin. The Rashba surface states are
revealed in the STS spectra by the onset of a van Hove singularity at the band
edge. Eventually, an electronic depletion is found on interfacial Te atoms,
consistent with the formation of a space charge area in typical -
junctions.Comment: 5 pages, 4 figure
Charge Order Driven spin-Peierls Transition in NaV2O5
We conclude from 23Na and 51V NMR measurements in NaxV2O5(x=0.996) a charge
ordering transition starting at T=37 K and preceding the lattice distortion and
the formation of a spin gap Delta=106 K at Tc=34.7 K. Above Tc, only a single
Na site is observed in agreement with the Pmmn space group of this first
1/4-filled ladder system. Below Tc=34.7 K, this line evolves into eight
distinct 23Na quadrupolar split lines, which evidences a lattice distortion
with, at least, a doubling of the unit cell in the (a,b) plane. A model for
this unique transition implying both charge density wave and spin-Peierls order
is discussed.Comment: 4 pages, 3 figures, submitted to Phys. Rev. Let
Zigzag Charge Ordering in alpha'-NaV2O5
23Na NMR spectrum measurements in alpha'-NaV2O5 with a single- crystalline
sample are reported. In the charge-ordered phase, the number of inequivalent Na
sites observed is more than that expected from the low-temperature structures
of space group Fmm2 reported so far. This disagreement indicates that the real
structure including both atomic displacement and charge disproportionation is
of lower symmetry. It is suggested that zigzag ordering is the most probable.
The temperature variation of the NMR spectra near the transition temperature is
incompatible with that of second-order transitions. It is thus concluded that
the charge ordering transition is first-order.Comment: 4 pages, 5 eps figures, submitted to J. Phys. Soc. Jp
The electronic structure and the phases of BaVS3
BaVS3 is a moderately correlated d-electron system with a rich phase diagram.
To construct the corresponding minimal electronic model, one has to decide
which d-states are occupied, and to which extent. The ARPES experiment
presented here shows that the behavior of BaVS3 is governed by the coexistence
of wide-band (A_1g) and narrow-band (twofold degenerate E) d-electrons. We
sketch a lattice fermion model which may serve as a minimal model of BaVS3.
This serves foremost for the understanding of the metal-insulator in pure BaVS3
and its absence in some related compounds. The nature of the low temperature
magnetic order differs for several systems which may be described in terms of
the same electron model. We describe several recent experiments which give
information about magnetic order at high pressures. In particular, we discuss
field-induced insulator-to-metal transition at slightly subcritical pressures,
and an evidence for magnetic order in the high-pressure metallic phase. The
phase diagram of Sr-doped BaVS3 is also discussed. The complexity of the phases
of BaVS3 arises from the fact that it is simultaneously unstable against
several kinds of instabilities.Comment: Presented at the International Conference on Magnetism 2006 (Kyoto),
6 pages, 9 figure
Orthorhombic versus monoclinic symmetry of the charge-ordered state of NaV2O5
High-resolution X-ray diffraction data show that the low-temperature
superstructure of alpha-NaV2O5 has an F-centered orthorhombic 2a x 2b x 4c
superlattice. A structure model is proposed, that is characterized by layers
with zigzag charge order on all ladders and stacking disorder, such that the
averaged structure has space group Fmm2. This model is in accordance with both
X-ray scattering and NMR data. Variations in the stacking order and disorder
offer an explanation for the recently observed devils staircase of the
superlattice period along c.Comment: REVTEX, 4 pages including 2 figures, shortened, submitted to PR
Charge-ordering phase transition and order-disorder effects in the Raman spectra of NaV2O5
In the ac polarized Raman spectra of NaV2O5 we have found anomalous phonon
broadening, and an energy shift of the low-frequency mode as a function of the
temperature. These effects are related to the breaking of translational
symmetry, caused by electrical disorder that originates from the fluctuating
nature of the V {4.5+} valence state of vanadium. The structural correlation
length, obtained from comparisons between the measured and calculated Raman
scattering spectra, diverges at T< 5 K, indicating the existence of the
long-range charge order at very low temperatures, probably at T=0 K.Comment: 8 pages, 4 figures, new version, to appear in PR
High field magnetic resonant properties of beta'-(ET)2SF5CF2SO3
A systematic electron spin resonance (ESR) investigation of the low
temperature regime for the (ET)2SF5CF2SO3 system was performed in the frequency
range of ~200-700 GHz, using backward wave oscillator sources, and at fields up
to 25 T. Newly acquired access to the high frequency and fields shows
experimental ESR results in agreement with the nuclear magnetic resonance (NMR)
investigation, revealing evidence that the transition seen at 20 K is not of
conventional spin-Peierls order. A significant change of the spin resonance
spectrum in beta'-(ET)2SF5CF2SO3 at low temperatures, indicates a transition
into a three-dimensional-antiferromagnetic (3D AFM) phase.Comment: 4 pages, 7 figures, minor grammatical change
X-ray anomalous scattering investigations on the charge order in -NaVO
Anomalous x-ray diffraction studies show that the charge ordering in
-NaVO is of zig-zag type in all vanadium ladders. We
have found that there are two models of the stacking of layers along
\emph{c-}direction, each of them consisting of 2 degenerated patterns, and that
the experimental data is well reproduced if the 2 patterns appears
simultaneously. We believe that the low temperature structure contains stacking
faults separating regions corresponding to the four possible patterns.Comment: Submitted to Phys. Rev. Lett., 4 pages, 4 eps figures inserted in the
tex
Anomalous spectral weight in photoemission spectra of the hole doped Haldane chain Y2-xSrxBaNiO5
In this paper, we present photoemission experiments on the hole doped Haldane
chain compound . By using the photon energy dependence of
the photoemission cross section, we identified the symmetry of the first
ionisation states (d type). Hole doping in this system leads to a significant
increase in the spectral weight at the top of the valence band without any
change in the vicinity of the Fermi energy. This behavior, not observed in
other charge transfer oxides at low doping level, could result from the
inhomogeneous character of the doped system and from a Ni 3d-O 2p hybridization
enhancement due to the shortening of the relevant Ni-O distance in the
localized hole-doped regions.Comment: 5 pages, 4 figure
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