273 research outputs found
Infrared spectroscopic studies on unoriented single-walled carbon nanotube films under hydrostatic pressure
The electronic properties of as-prepared and purified unoriented
single-walled carbon nanotube films were studied by transmission measurements
over a broad frequency range (far-infrared up to visible) as a function of
temperature (15 K - 295 K) and external pressure (up to 8 GPa). Both the
as-prepared and the purified SWCNT films exhibit nearly temperature-independent
properties. With increasing pressure the low-energy absorbance decreases
suggesting an increasing carrier localization due to pressure-induced
deformations. The energy of the optical transitions in the SWCNTs decreases
with increasing pressure, which can be attributed to pressure-induced
hybridization and symmetry-breaking effects. We find an anomaly in the
pressure-induced shift of the optical transitions at 2 GPa due to a
structural phase transition.Comment: 13 pages, 15 figure
Chirality distribution and transition energies of carbon nanotubes
From resonant Raman scattering on isolated nanotubes we obtained the optical
transition energies, the radial breathing mode frequency and Raman intensity of
both metallic and semiconducting tubes. We unambiguously assigned the chiral
index (n_1,n_2) of approximately 50 nanotubes based solely on a third-neighbor
tight-binding Kataura plot and find omega_RBM=214.4cm^-1nm/d+18.7cm^-1. In
contrast to luminescence experiments we observe all chiralities including
zig-zag tubes. The Raman intensities have a systematic chiral-angle dependence
confirming recent ab-initio calculations.Comment: 4 pages, to be published in Phys. Rev. Let
Contacting single bundles of carbon nanotubes with alternating electric fields
Single bundles of carbon nanotubes have been selectively deposited from
suspensions onto sub-micron electrodes with alternating electric fields. We
explore the resulting contacts using several solvents and delineate the
differences between Au and Ag as electrode materials. Alignment of the bundles
between electrodes occurs at frequencies above 1 kHz. Control over the number
of trapped bundles is achieved by choosing an electrode material which
interacts strongly with the chemical functional groups of the carbon nanotubes,
with superior contacts being formed with Ag electrodes.Comment: 4 pages, RevTe
Entanglement of distant atoms by projective measurement: The role of detection efficiency
We assess proposals for entangling two distant atoms by measurement of
emitted photons, analyzing how their performance depends on the photon
detection efficiency. We consider schemes based on measurement of one or two
photons and compare them in terms of the probability to obtain the detection
event and of the conditional fidelity with which the desired entangled state is
created. Based on an unravelling of the master equation, we quantify the
parameter regimes in which one or the other scheme is more efficient, including
the possible combination of the one-photon scheme with state purification. In
general, protocols based on one-photon detection are more efficient in set-ups
characterized by low photon detection efficiency, while at larger values
two-photon protocols are preferable. We give numerical examples based on
current experiments.Comment: 12 pages, 6 figure
Influence of endohedral water on diameter sorting of single-walled carbon nanotubes by density gradient centrifugation
Beta-decay of nuclei around Se-90. Search for signatures of a N=56 sub-shell closure relevant the r-process
Nuclear structure plays a significant role on the rapid neutron capture
process (r-process) since shapes evolve with the emergence of shells and
sub-shells. There was some indication in neighboring nuclei that we might find
examples of a new N=56 sub-shell, which may give rise to a doubly magic Se-90
nucleus. Beta-decay half lives of nuclei around Se-90 have been measured to
determine if this nucleus has in fact a doubly-magic character. The
fragmentation of Xe-136 beam at the National Superconducting Cyclotron
Laboratory at Michigan State University was used to create a cocktail of nuclei
in the A=90 region. We have measured the half lives of twenty-two nuclei near
the r-process path in the A=90 region. The half lives of As-88 and Se-90 have
been measured for the first time. The values were compared with theoretical
predictions in the search for nuclear-deformation signatures of a N=56
sub-shell, and its possible role in the emergence of a potential doubly-magic
Se-90. The impact of such hypothesis on the synthesis of heavy nuclei,
particularly in the production of Sr, Y and Zr elements was investigated with a
weak r-process network. The new half lives agree with results obtained from a
standard global QRPA model used in r-process calculations, indicating that
Se-90 has a quadrupole shape incompatible with a closed N=56 sub-shell in this
region. The impact of the measured Se-90 half-life in comparison with a former
theoretical predication associated with a spherical half-life on the
weak-r-process is shown to be strong
Quantum interference from remotely trapped ions
We observe quantum interference of photons emitted by two continuously
laser-excited single ions, independently trapped in distinct vacuum vessels.
High contrast two-photon interference is observed in two experiments with
different ion species, calcium and barium. Our experimental findings are
quantitatively reproduced by Bloch equation calculations. In particular, we
show that the coherence of the individual resonance fluorescence light field is
determined from the observed interference
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