Transport and Noise Characteristics of Submicron High-Temperature Superconductor Grain-Boundary Junctions

We have investigated the transport and noise properties of submicron YBCO bicrystal grain-boundary junctions prepared using electron beam lithography. The junctions show an increased conductance for low voltages reminiscent of Josephson junctions having a barrier with high transmissivity. The voltage noise spectra are dominated by a few Lorentzian components. At low temperatures clear two-level random telegraph switching (RTS) signals are observable in the voltage vs time traces. We have investigated the temperature and voltage dependence of individual fluctuators both from statistical analysis of voltage vs time traces and from fits to noise spectra. A transition from tunneling to thermally activated behavior of individual fluctuators was clearly observed. The experimental results support the model of charge carrier traps in the barrier region.Comment: 4 pages, 4 figures, to be published in Appl. Phys. Let

Two regimes for effects of surface disorder on the zero-bias conductance peak of tunnel junctions involving d-wave superconductors

Impurity-induced quasiparticle bound states on a pair-breaking surface of a d-wave superconductor are theoretically described, taking into account hybridization of impurity- and surface-induced Andreev states. Further a theory for effects of surface disorder (of thin impurity surface layer) on the low-bias conductance of tunnel junctions is developed. We find a threshold $n_c$ for surface impurity concentration $n_S$, which separates the two regimes for surface impurity effects on the zero-bias conductance peak (ZBCP). Below the threshold, surface impurities do not broaden the ZBCP, but effectively reduce its weight and generate impurity bands. For low $n_S$ impurity bands can be, in principle, resolved experimentally, being centered at energies of bound states induced by an isolated impurity on the surface. For larger $n_S$ impurity bands are distorted, move to lower energies and, beginning with the threshold concentration $n_S=n_c$, become centered at zero energy. With increasing $n_S$ above the threshold, the ZBCP is quickly destroyed in the case of strong scatterers, while it is gradually suppressed and broaden in the presence of weak impurity potentials. More realistic cases, taking into account additional broadening, not related to the surface disorder, are also considered.Comment: 9 pages, 7 figure

Electronic depth profiles with atomic layer resolution from resonant soft x-ray reflectivity

The analysis of x-ray reflectivity data from artificial heterostructures usually relies on the homogeneity of optical properties of the constituent materials. However, when the x-ray energy is tuned to an absorption edge, this homogeneity no longer exists. Within the same material, spatial regions containing elements at resonance will have optical properties very different from regions without resonating sites. In this situation, models assuming homogeneous optical properties throughout the material can fail to describe the reflectivity adequately. As we show here, resonant soft x-ray reflectivity is sensitive to these variations, even though the wavelength is typically large as compared to the atomic distances over which the optical properties vary. We have therefore developed a scheme for analyzing resonant soft x-ray reflectivity data, which takes the atomic structure of a material into account by "slicing" it into atomic planes with characteristic optical properties. Using LaSrMnO4 as an example, we discuss both the theoretical and experimental implications of this approach. Our analysis not only allows to determine important structural information such as interface terminations and stacking of atomic layers, but also enables to extract depth-resolved spectroscopic information with atomic resolution, thus enhancing the capability of the technique to study emergent phenomena at surfaces and interfaces.Comment: Completely overhauled with respect to the previous version due to peer revie

Electronic structure of d-wave superconducting quantum wires

We present analytical and numerical results for the electronic spectra of wires of a d-wave superconductor on a square lattice. The spectra of Andreev and other quasiparticle states, as well as the spatial and particle-hole structures of their wave functions, depend on interference effects caused by the presence of the surfaces and are qualitatively different for half-filled wires with even or odd number of chains. For half-filled wires with an odd number of chains N at (110) orientation, spectra consist of N doubly degenerate branches. By contrast, for even N wires, these levels are split, and all quasiparticle states, even the ones lying above the maximal gap, have the characteristic properties of Andreev bound states. These Andreev states above the gap can be interpreted as a consequence of an infinite sequence of Andreev reflections experienced by quasiparticles along their trajectories bounded by the surfaces of the wire. Our microscopic results for the local density of states display atomic-scale Friedel oscillations due to the presence of the surfaces, which should be observable by scanning tunneling microscopy. For narrow wires the self-consistent treatment of the order parameter is found to play a crucial role. In particular, we find that for small wire widths the finite geometry may drive strong fluctuations or even stablilize exotic quasi-1D pair states with spin triplet character.Comment: 21 pages, 20 figures. Slightly modified version as published in PR

Comment on "Raman spectroscopy study of NaxCoO2 and superconducting NaxCoO2 yH2O"

The effect of surface degradation of the thermolectric cobaltite on Raman spectra is discussed and compared to experimental results from Co3O4 single crystals. We conclude that on NaCl flux grown NaxCoO2 crystals a surface layer of Co3O4 easily forms that leads to the observation of an intense phonon around 700 cm-1 [Phys. Rev. B 70, 052502 (2004)]. Raman spectra on freshly cleaved crystals from optical floating zone ovens do not show such effects and have a high frequency phonon cut-off at approximately 600 cm -1 [Phys. Rev. Lett 96, 167204 (2006)]. We discuss the relation of structural dimensionality, electronic correlations and the high frequency phonon cut-off of the thermolectric cobaltite.Comment: 2 pages, 1 figure, to be published in Phys. Rev. B (2007

Anomalous Low Temperature Behavior of Superconducting Nd(1.85)Ce(0.15)CuO(4-y)

We have measured the temperature dependence of the in-plane London penetration depth lambda(T) and the maximum Josephson current Ic(T) using bicrystal grain boundary Josephson junctions of the electron-doped cuprate superconductor Nd(1.85)Ce(0.15)CuO(4-y). Both quantities reveal an anomalous temperature dependence below about 4 K. In contrast to the usual monotonous decrease (increase) of lambda(T) (Ic(T)) with decreasing temperature, lambda(T) and Ic(T) are found to increase and decrease, respectively, with decreasing temperature below 4 K resulting in a non-monotonous overall temperature dependence. This anomalous behavior was found to be absent in analogous measurements performed on Pr(1.85)Ce(0.15)CuO(4-y). From this we conclude that the anomalous behavior of Nd(1.85)Ce(0.15)CuO(4-y) is caused by the presence of the Nd3+ paramagnetic moments. Correcting the measured lambda(T) dependence of Nd(1.85)Ce(0.15)CuO(4-y) for the temperature dependent susceptibility due to the Nd moments, an exponential dependence is obtained indicating isotropic s-wave pairing. This result is fully consistent with the lambda(T) dependence measured for Pr(1.85)Ce(0.15)CuO(4-y).Comment: 4 pages including 4 figures, to appear in Phys. Rev. Let

Possible pseudogap behavior of electron doped high-temperature superconductors

We have measured the low-energy quasiparticle excitation spectrum of the electron doped high-temperature superconductors (HTS) Nd(1.85)Ce(0.15)CuO(4-y) and Pr(1.85)Ce(0.15)CuO(4-y) as a function of temperature and applied magnetic field using tunneling spectroscopy. At zero magnetic field, for these optimum doped samples no excitation gap is observed in the tunneling spectra above the transition temperature Tc. In contrast, below Tc for applied magnetic fields well above the resistively determined upper critical field, a clear excitation gap at the Fermi level is found which is comparable to the superconducting energy gap below Tc. Possible interpretations of this observation are the existence of a normal state pseudogap in the electron doped HTS or the existence of a spatially non-uniform superconducting state.Comment: 4 pages, 4 ps-figures included, to be published in Phys. Rev. B, Rapid Com

Evidence for Surface Andreev Bound states in Cuprate Superconductors from Penetration Depth Measurements

Tunneling and theoretical studies have suggested that Andreev bound states form at certain surfaces of unconventional superconductors. Through studies of the temperature and field dependence of the in-plane magnetic penetration depth lambda_ab at low temperature, we have found strong evidence for the presence of these states in clean single crystal YBCO and BSCCO. Crystals cut to expose a [110] interface show a strong upturn in lambda_ab at around 7K, when the field is oriented so that the supercurrents flow around this surface. In YBCO this upturn is completely suppressed by a field of ~0.1 T.Comment: 4 pages 2 column revtex + 4 postscript figures. Submitted to PR

Evidence for a Nodeless Gap from the Superfluid Density of Optimally Doped Pr_{1.855}Ce_{0.145}CuO_{4-y} Films

We present measurements of the ab-plane magnetic penetration depth, \lambda(T), in five optimally doped Pr_{1.855}Ce_{0.145}CuO_{4-y} films for 1.6 K \leq T \leq T_c \sim 24 K. Low resistivities, high superfluid densities n_s(T)\propto \lambda^{-2}(T), high T_c's, and small transition widths are reproducible and indicative of excellent film quality. For all five films, \lambda^{-2}(T)/\lambda^{-2}(0) at low T is well fitted by an exponential temperature dependence with a gap, \Delta_{min}, of 0.85 k_B T_c. This behavior is consistent with a nodeless gap and is incompatible with d-wave superconductivity.Comment: 5 pages, 4 figures, reorganized for clarit